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Plasma-Surface Interactions during Plasma Etching for Next-Generation Nanoscale Device Fabrication

Planned Research

Project AreaCreation of Science of Plasma Nano-Interface Interactions
Project/Area Number 21110008
Research Category

Grant-in-Aid for Scientific Research on Innovative Areas (Research in a proposed research area)

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionKyoto University

Principal Investigator

ONO Kouichi  京都大学, 工学(系)研究科(研究院), 教授 (30311731)

Co-Investigator(Kenkyū-buntansha) ERIGUCHI Koji  京都大学, 工学研究科, 准教授 (70419448)
TAKAO Yoshinori  京都大学, 工学研究科, 助教 (80552661)
Project Period (FY) 2009-07-23 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥69,030,000 (Direct Cost: ¥53,100,000、Indirect Cost: ¥15,930,000)
Fiscal Year 2013: ¥15,210,000 (Direct Cost: ¥11,700,000、Indirect Cost: ¥3,510,000)
Fiscal Year 2012: ¥15,210,000 (Direct Cost: ¥11,700,000、Indirect Cost: ¥3,510,000)
Fiscal Year 2011: ¥15,210,000 (Direct Cost: ¥11,700,000、Indirect Cost: ¥3,510,000)
Fiscal Year 2010: ¥15,210,000 (Direct Cost: ¥11,700,000、Indirect Cost: ¥3,510,000)
Fiscal Year 2009: ¥8,190,000 (Direct Cost: ¥6,300,000、Indirect Cost: ¥1,890,000)
Keywordsプラズマ加工 / プラズマ化学 / 表面・界面物性 / 半導体超微細化 / 超微細加工技術 / 反応粒子輸送 / プラズマエッチング / プラズマ・表面過程揺動 / 超微細加工形状
Research Abstract

Nanometer-scale surface roughness has become an important issue to be resolved in the fabrication of nanoscale devices, because the roughness at the feature bottom and sidewalls affects the variability in transistor performance. We have developed a three-dimensional atomic-scale cellular model (ASCeM-3D) based on the Monte Carlo algorithm, to simulate plasma-surface interactions and the nanoscale feature profile evolution during plasma etching of Si in Cl-based plasmas. Numerical results exhibited nanoscale surface roughening and rippling in response to ion incidence angle onto substrate surfaces. The mechanisms for such surface roughening and rippling of etched surfaces were investigated through a comparison with experiments, with the help of a classical molecular dynamics simulation. Based on these understanding, the pulse-bias etching through a repetitive on/off of the rf bias power was demonstrated to be one promising way of reducing the surface roughness during plasma etching.

Report

(6 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • 2010 Annual Research Report
  • 2009 Annual Research Report
  • Research Products

    (49 results)

All 2014 2013 2012 2011 2010 2009 Other

All Journal Article (21 results) (of which Peer Reviewed: 20 results) Presentation (21 results) (of which Invited: 9 results) Book (4 results) Remarks (1 results) Patent(Industrial Property Rights) (2 results)

  • [Journal Article] Surface roughening and rippling during plasma etching of Si : Numerical investigations and a comparison with experiments2014

    • Author(s)
      H.Tsuda, N.Nakazaki, Y.Takao, K.Eriguchi, and K.Ono
    • Journal Title

      J. Vac. Sci. Technol.

      Volume: B 32 Issue: 3

    • DOI

      10.1116/1.4874309

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Molecular dynamics simulations of silicon chloride ion incidence during Si etching in Cl-based plasmas2014

    • Author(s)
      N.Nakazaki, Y.Takao, K.Eriguchi, and K.Ono
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 53 Issue: 5 Pages: 056201-056201

    • DOI

      10.7567/jjap.53.056201

    • NAID

      210000143754

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Surface roughening and rippling during plasma etching of Si: Numerical investigations and a comparison with experiments2014

    • Author(s)
      H. Tsuda, N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Journal Title

      J. Vac. Sci. Technol. B

      Volume: 32

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] プラズマナノ加工における表面ラフネスとリップル形成機構2013

    • Author(s)
      斧 高一, 津田博隆, 中崎暢也, 鷹尾祥典, 江利口浩二
    • Journal Title

      表面科学

      Volume: 34 Pages: 528-534

    • NAID

      10031202796

    • URL

      https://www.jstage.jst.go.jp/browse/jsssj/34/10/_contents/-char/ja/

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of capacitive coupling in a miniature inductively coupled plasma source2012

    • Author(s)
      Y.Takao, K.Eriguchi, and K.Ono
    • Journal Title

      J. Appl. Phys

      Volume: 112 Issue: 9 Pages: 93306-93306

    • DOI

      10.1063/1.4764333

    • NAID

      120004920433

    • URL

      http://hdl.handle.net/2433/161047

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Modeling and Simulation of Nanoscale Surface Rippling during Plasma Etching of Si under Oblique Ion Incidence2012

    • Author(s)
      Hirotaka Tsuda, Yoshinori Takao, Koji Friguchi Kouichi Onc
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 51 Issue: 8S1 Pages: 08HC01-08HC01

    • DOI

      10.1143/jjap.51.08hc01

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular Dynamics Analysis of the Formation of Surface Roughness during Si Etching in Chlorine-based Plasmas2011

    • Author(s)
      Hirotaka Tsuda, Yoshinori Takao, Koji Eriguchi, Kouichi Ono
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 50 Issue: 8S2 Pages: 08KB02-08KB02

    • DOI

      10.1143/jjap.50.08kb02

    • Related Report
      2013 Final Research Report 2011 Annual Research Report 2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Three-dimensional Atomic-scale Cellular Model and Feature Profile Evolution during Si Etching in Chlorine-based Plasmas : Analysis of Profile Anomalies and Surface Roughness2011

    • Author(s)
      Hirotaka Tsuda, Hiroki Miyata, Yoshinori Takao, Koji Eriguchi, Kouichi Ono
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 50 Issue: 8S1 Pages: 08JE06-08JE06

    • DOI

      10.1143/jjap.50.08je06

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Particle Simulations of Sheath Dynamics in Low Pressure Capacitively Coupled Argon Plasma Discharges2011

    • Author(s)
      Y.Takao, K.Matsuoka, K.Eriguchi, and K.Ono
    • Journal Title

      Jpn. J. Appl. Phys

      Volume: 50 Issue: 8S1 Pages: 08JC02-08JC02

    • DOI

      10.1143/jjap.50.08jc02

    • NAID

      210000071066

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Modeling of plasma-induced damage and its impacts on parameter variations in advanced electronic devices2011

    • Author(s)
      K.Eriguchi, Y.Takao, and K.Ono
    • Journal Title

      J. Vac. Sci. Technol

      Volume: A29 Issue: 4 Pages: 41303-41303

    • DOI

      10.1116/1.3598382

    • NAID

      120003133618

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-scale cellular model and profile simulation of Si etching : Analysis of profile anomalies and microscopic uniformity2010

    • Author(s)
      H.Tsuda, M.Mori, Y.Takao, K.Eriguchi, and K.Ono
    • Journal Title

      Jpn. J. Appl. Phys

      Volume: 49 Issue: 8S1 Pages: 08JE01-08JE01

    • DOI

      10.1143/jjap.49.08je01

    • NAID

      210000069057

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] 先端プラズマエッチングプロセスのモデリングと体系化2010

    • Author(s)
      斧 高一
    • Journal Title

      化学工業

      Volume: 61 Pages: 457-465

    • NAID

      40017136560

    • URL

      http://www.kako-sha.co.jp/2010contentskagaku.htm

    • Related Report
      2013 Final Research Report
  • [Journal Article] Atomic-scale cellular model and profile simulation of Si etching : Formation of surface roughness and residue2010

    • Author(s)
      H.Tsuda, M.Mori, Y.Takao, K.Eriguchi, and K.Ono
    • Journal Title

      Thin Solid Films

      Volume: 518 Issue: 13 Pages: 3475-3480

    • DOI

      10.1016/j.tsf.2009.11.043

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Plasma-surface interactions for advanced plasma etching processes in nanoscale ULSI device fabrication : A numerical and experimental study2010

    • Author(s)
      K.Ono, H.Ohta, and K.Eriguchi
    • Journal Title

      Thin Solid Films

      Volume: 518 Issue: 13 Pages: 3461-3468

    • DOI

      10.1016/j.tsf.2009.11.030

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Two-dimensional particle-in-cell Monte Carlo simulation of a miniature inductively coupled plasma source2010

    • Author(s)
      Y.Takao, N, Kusaba, K.Eriguchi, and K.Ono
    • Journal Title

      J. Appl. Phys

      Volume: 108 Issue: 9

    • DOI

      10.1063/1.3506536

    • NAID

      120005553877

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-scale cellular model and profile simulation of Si etching : Analysis of profile anomalies and microscopic uniformity2010

    • Author(s)
      H.Tsuda, M.Mori, Y.Takao, K.Eriguchi, K.Ono
    • Journal Title

      Jpn.J.Appl.Phys

      Volume: Vol.49, No.8

    • NAID

      210000069057

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Two-dimensional particle-in-cell Monte Carlo simulation of a miniature inductively coupled plasma source2010

    • Author(s)
      Y.Takao, N, Kusaba, K.Eriguchi, K.Ono
    • Journal Title

      J.Appl.Phys.

      Volume: Vol.108, No.9

    • NAID

      120005553877

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Plasma-surface interactions for advanced plasma etching processes in nanoscale ULSI device fabrication : A numerical and experimental study2010

    • Author(s)
      K.Ono, H.Ohta, K.Eriguchi
    • Journal Title

      Thin Solid Films Vol.518

      Pages: 3461-3468

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-scale cellular model and profile simulation of Si etching : Formation of surface roughness and residue2010

    • Author(s)
      H.Tsuda, M.Mori, Y.Takao, K.Friguchi, K.Ono
    • Journal Title

      Thin Solid Films Vol.518

      Pages: 3475-3480

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular-Dynamics-Based Profile Evolution Simulation for Sub-10-nm Si Processing Technology2009

    • Author(s)
      H.Tsuda, K.Eriguchi, K.Ono, and H.Ohta
    • Journal Title

      Appl. Phys. Express

      Volume: 2 Issue: 11 Pages: 116501-116501

    • DOI

      10.1143/apex.2.116501

    • NAID

      10027012154

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Molecular-Dynamics-Based Profile Evolution Simulation for Sub-10-nm Si Processing Technology2009

    • Author(s)
      H.Tsuda, K.Eriguchi, K.Ono, H.Ohta
    • Journal Title

      Appl.Phys.Express Vol.2, No.11

    • NAID

      10027012154

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] Plasma Etch Challenges for Nanoscale Device Fabrication : Modeling, Analysis, and Control of Plasma-Surface Interactions2013

    • Author(s)
      K.Ono
    • Organizer
      9th Asian-European International Conference on Plasma Surface Engineering (AEPSE2013)
    • Place of Presentation
      Jeju, South Korea (韓国,済州島)
    • Year and Date
      2013-08-30
    • Related Report
      2013 Final Research Report
  • [Presentation] Surface Roughening during Si Etching in Inductively Coupled Cl2 Plasmas: Experimental Investigations and a Comparison with Numerical Simulations2013

    • Author(s)
      (H. Tsuda), N. Nakazaki, D. Fukushima, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      6th International Conference on Plasma-Nanotechnology Science (IC-PLANTS2013)
    • Place of Presentation
      Gero, Gifu, Japan
    • Year and Date
      2013-02-03
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Formation Mechanisms of Nanoscale Surface Roughness and Rippling during Plasma Etching and Sputtering of Si under Oblique Ion Incidence2012

    • Author(s)
      (H. Tsuda), Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      American Vacuum Society 59th International Symposium (AVS2012)
    • Place of Presentation
      Tampa, Florida, USA
    • Year and Date
      2012-10-30
    • Related Report
      2012 Annual Research Report
  • [Presentation] Molecular Dynamics Analysis of Si Etching with Cl and Br Beams: Ion Incident Angle and Neutral Radical Flux Dependence2012

    • Author(s)
      (N. Nakazaki), H. Tsuda, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      American Vacuum Society 59th International Symposium (AVS2012)
    • Place of Presentation
      Tampa, Florida, USA
    • Year and Date
      2012-10-30
    • Related Report
      2012 Annual Research Report
  • [Presentation] Plasma Etching for Nanofabrication : Fundamentals, Current Status, and Future Prospects2012

    • Author(s)
      K.Ono
    • Organizer
      11th Asia Pacific Conference on Plasma Science and Technology (APCPST 2012) and 25th Symposium on Plasma Science for Materials SPSM25)
    • Place of Presentation
      Kyoto, Japan (京都市)
    • Year and Date
      2012-10-02
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Plasma Etching for Nanofabrication: Fundamentals, Current Status, and Future Prospects2012

    • Author(s)
      (K. Ono)
    • Organizer
      11th Asia Pacific Conference on Plasma Science and Technology (APCPST2012) and 25th Symposium on Plasma Science for Materials (SPSM25)
    • Place of Presentation
      Kyoto University, Kyoto, Japan
    • Year and Date
      2012-10-02
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Surface Roughening and Rippling during Plasma Etching2012

    • Author(s)
      K.Ono
    • Organizer
      International Union of Materials Research Societies - International Conference on Electronic Materials (IUMRSICEM 2012)
    • Place of Presentation
      Yokohama, Japan (横浜市)
    • Year and Date
      2012-09-25
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Surface Roughening and Rippling during Plasma Etching2012

    • Author(s)
      (K. Ono)
    • Organizer
      International Union of Materials Research Societies - International Conference on Electronic Materials (IUMRS-ICEM 2012)
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan
    • Year and Date
      2012-09-25
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Plasma-Surface Interactions for Materials Nanofabrication and Space Propulsion : A Unified Study for Technology Developments and Future Progress2011

    • Author(s)
      K.Ono
    • Organizer
      Plasma Conference 2011 (PLASMA 2011)
    • Place of Presentation
      Kanazawa, Japan (金沢市)
    • Year and Date
      2011-11-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Plasma-Surface Interactions for Materials Nanofabrication and Space, Propulsion : A Unified Study for Technology Developments and Future2011

    • Author(s)
      K.Ono
    • Organizer
      Plasma Conference 2011 (PLASMA 2011)
    • Place of Presentation
      Kanazawa, Japan(招待講演)
    • Year and Date
      2011-11-22
    • Related Report
      2011 Annual Research Report
  • [Presentation] Plasma-surface interactions in plasma etching processes for nanometer-scale microelectronic devices2010

    • Author(s)
      K.Ono
    • Organizer
      63rd Annual Gaseous Electronics Conference (GEC2010) and 7th International Conference on Reactive Plasmas (ICRP-7)
    • Place of Presentation
      Paris, France (フランス,パリ市)
    • Year and Date
      2010-10-07
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Plasma-surface interactions in plasma etching processes for nanometer-scale microelectronic devices2010

    • Author(s)
      K.Ono
    • Organizer
      63rd Gaseous Electronics Conference (GEC2010) and 7th International Conference on Reactive Plasmas (ICRP-7)
    • Place of Presentation
      Paris, France(招待講演)
    • Year and Date
      2010-10-07
    • Related Report
      2010 Annual Research Report
  • [Presentation] Plasma-surface interactions in plasma etching of high-k dielectrics and metal electrode materials2010

    • Author(s)
      K.Ono
    • Organizer
      10th Asia-Pacific Conference on Plasma Science and Technology (APCPST2010) and 23rd Symposium on Plasma Science for Materials (SPSM23)
    • Place of Presentation
      Jeju, South Korea [韓国,済州島]
    • Year and Date
      2010-07-05
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Plasma Nano-Surface Engineering for Advanced Gate Etch Process in ULSI Device Fabrication2009

    • Author(s)
      K.Ono
    • Organizer
      7th Asian-European International Conference on Plasma Surface Engineering (AEPSE2009)
    • Place of Presentation
      Busan, Korea (韓国,釜山市)
    • Year and Date
      2009-09-23
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Plasma Nano-Surface Engineering for Advanced Gate Etch Process in ULSI Device Fabrication2009

    • Author(s)
      K.Ono
    • Organizer
      7th Asian-European International Conference on Plasma Surface Engineering (AEPSE2009), Busan, South Korea.
    • Place of Presentation
      Busan, South Korea
    • Year and Date
      2009-09-23
    • Related Report
      2009 Annual Research Report
  • [Presentation] Plasma Etch Challenges for Nanoscale Device Fabrication: Modeling, Analysis, and Control of Plasma-Surface Interactions

    • Author(s)
      K. Ono
    • Organizer
      9th Asian-European International Conference on Plasma Surface Engineering (AEPSE2013)
    • Place of Presentation
      Jeju, South Korea
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Molecular dynamics analysis of Si etching in HBr-based Plasmas: Effects of neutral radicals

    • Author(s)
      N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      35th International Symposium on Dry Process (DPS 2013)
    • Place of Presentation
      Jeju, South Korea
    • Related Report
      2013 Annual Research Report
  • [Presentation] Molecular dynamics simulation of etch by-product ion incidence during Si etching in Cl-based plasmas

    • Author(s)
      N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      26th Symposium on Plasma Science & Materials (SPSM26)
    • Place of Presentation
      Fukuoka, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Molecular Dynamics Analysis of Surface Reaction Kinetics during Si Etching in Cl-based Plasmas

    • Author(s)
      N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      66th Annual Gaseous Electronics Conference (GEC2013)
    • Place of Presentation
      Princeton, NJ, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Molecular Dynamics Analysis of Si Etching in HBr-based Plasmas: Ion Incident Energy and Angle Dependence

    • Author(s)
      N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      AVS 60th International Symposium (AVS2013)
    • Place of Presentation
      Long Beach, CA, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Surface roughening during Si etching in inductively coupled Cl2 plasmas

    • Author(s)
      N. Nakazaki, Y. Takao, K. Eriguchi, and K. Ono
    • Organizer
      8th International Conference on Reactive Plasmas and 31st Symposium on Plasma Processing (ICRP-8/SPP-31)
    • Place of Presentation
      Fukuoka, Japan
    • Related Report
      2013 Annual Research Report
  • [Book] High-k 膜のドライエッチング ナノエレクトロニクスにおける絶縁超薄膜技術-成膜技術と膜・界面の物性科学-, 第5編, 第4章2012

    • Author(s)
      斧 高一(分担執筆)
    • Publisher
      エヌ・ティー・エス社
    • Related Report
      2013 Final Research Report
  • [Book] "High-k 膜のドライエッチング", 「ナノエレクトロニクスにおける絶縁超薄膜技術-成膜技術と膜・界面の物性科学-」, 第5編, 第4章 (分担執筆).2012

    • Author(s)
      斧 高一
    • Publisher
      エヌ・ティー・エス社
    • Related Report
      2012 Annual Research Report
  • [Book] プラズマエッチングにおける表面反応機構 マイクロ・ナノデバイスのエッチング技術 式田光宏 他 監修, 第二編, 第2章2009

    • Author(s)
      斧 高一(分担執筆)
    • Publisher
      シーエムシー出版
    • Related Report
      2013 Final Research Report
  • [Book] 「マイクロ・ナノデバイスのエッチング技術」,式田光宏・佐藤一雄・田中浩監修 第二編,第2章"プラズマエッチングにおける表面反応機構"2009

    • Author(s)
      斧高一[分担執筆]
    • Publisher
      シーエムシー出版
    • Related Report
      2009 Annual Research Report
  • [Remarks]

    • URL

      http://www.propulsion.kuaero.kyoto-u.ac.jp/

    • Related Report
      2013 Final Research Report
  • [Patent(Industrial Property Rights)] 半導体処理装置のクリーニング方法およびシリコン基板のエッチング方法2011

    • Inventor(s)
      斧 高一,北川智洋,井上 實,大沢正典
    • Industrial Property Rights Holder
      京都大学,太陽日酸株式会社
    • Industrial Property Rights Type
      特許
    • Acquisition Date
      2011-10-07
    • Related Report
      2013 Final Research Report
  • [Patent(Industrial Property Rights)] ワイヤー状構造をもつ半導体の製造方法及び製造装置2009

    • Inventor(s)
      太田裕朗,斧 高一
    • Industrial Property Rights Holder
      京都大学
    • Industrial Property Rights Type
      特許
    • Filing Date
      2009-06-23
    • Related Report
      2013 Final Research Report

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Published: 2009-04-01   Modified: 2018-03-28  

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