• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Intra-Spur Reactions Studied by Using Positronium Formation

Research Project

Project/Area Number 01540360
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 物理化学一般
Research InstitutionUniversity of Tokyo

Principal Investigator

ITO Yasuo  Research Center for Nuclear Science and Technology, Associate Professor, 原子力研究総合センター, 助教授 (40011150)

Co-Investigator(Kenkyū-buntansha) ZHICHENG Zhang  Fac. Engin. Univ. of Tokyo, Visiting Research Fellow (on leave from Univ. Sci. a
Project Period (FY) 1989 – 1990
Project Status Completed (Fiscal Year 1990)
Budget Amount *help
¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 1990: ¥300,000 (Direct Cost: ¥300,000)
Fiscal Year 1989: ¥1,300,000 (Direct Cost: ¥1,300,000)
KeywordsPositronium / Radiation spur / Excited States / Electron Scavengers / ポジトロン / 放射線化学 / スパ-反応 / 共鳴反応
Research Abstract

Positronium (Ps) is a hydrogen-like atom which is formed between positron (e^+) and electron (e^-). The mechanism of Ps formation is not yet made clear. There are two models of Ps formation. The Ore model assumes that energetic (epithermal) e^+ picks up an electron from the medium, and the spur model assumes that e^+ is nearly thermalized in its own terminal radiation spur and combines with e^- (excess electron) that is ejected by ionization.
The head investigator has long been involved in the research of this problem, and has a conclusion that the spur model is a better model than the former at least regarding Ps formation in condensed molecular substances. The precious study aims to advance this viewpoint and hopefully make the "Ps formation experiment" a research tool to study fast intra-spur reactions.
The experiments have been to measure Ps yield in various mixtures inert and electrophilic molecules. The importance of the spur process has been confirmed. Moreover a new aspect of Ps formation, namely "Ps formation from excited molecular states" has been found. By the discovery of this new process, the picture of Ps formation has been improved substantially, and we have published a thesis titles "A New Model of Positronium formation".
There still remains problems concerning evaluation of mutual relative importance of the Ore model and the spur model. These problems have been summarized in a review article.

Report

(3 results)
  • 1990 Annual Research Report   Final Research Report Summary
  • 1989 Annual Research Report
  • Research Products

    (20 results)

All Other

All Publications (20 results)

  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneko Tabata: "Antiーinhibition effect of Ckolrinated Benzenes on Positronium Formation in Ccla/C_6H_<12> mixtures" Rodiat. Phys. Chem.36. 273-277 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito: "Competitive effects of Electron Scavenger CH_2cl_2 with C_6F_6, C_6F_5H and CS_2 on Positronium Formation in Cychehexane" Radiat. Phys. Chem.36. 267-272 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneko Tabata: "Positronium Formation in CS_2 and C_6F_6 Mixtures with Triethylamine or Tetrahydrofurane" Radiat. Phys. Chem.36. 253-257 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneko Tabata: "The role of Excited States in Antiーinhibition Effects of Positronium Formation" Radiat. Phys. Chem.36. 285-290 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito: "A new model of Positrovium Formation Resonant Positronium Formation" J. Chem. Phys.93. 1021-1029 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneho Tabata: "Anti-inhibition Effect of Chlorinated Benzenes on Positronium Formation in CC1_4/C_6H_<12>" Radiat. Phys. Chem.36. 273-277 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito: "Competitive Effects of electron Scavenger CH_2Cl_2 with C_6F_6, C_6H_5F and CS_2 on Positronium Formation in Cyclohexane" Radiat. Phys. Chem.36. 267-272 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneho Tabata: "Positronium Formation in CS_2 and C_6F_6 mixtures with Triethylamine or Tetrahydrofurane" Radiat. Phys. Chem.36. 253-257 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito, Yoneho Tabata: "The role of Excited States in anti-inhibition Effects of Positronium formation" Radiat. Phys. Chem.36. 285 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng, Yasuo Ito: "A New Model of Positronium Formation --Resonant Positronium Formation ---" J. Chem. Phys.93. 1021-1029 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Yasuo ITO: "Hot Atom Chemistry and Positronium Chemistry" Handbook of Hot Atom Chemistry ed. by T. Matsuura.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1990 Final Research Report Summary
  • [Publications] Zhang Zhicheng,Yasuo Ito,Yoneho Tabata: "Antiーinhibition Effect of chlorinated Benzenes on Positronium Formation in CCl_4/C_6H_<12> mixtues" Radiat.Phup.Chem.36. 273-277 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo Ito: "Competitive Effects of Electron Scavenger CH_2 Cl_2 with C_6F_6,C_6F_5H and CS_2 on Positronium Formation in Cyclehexane" Radiat.Phys.Chem.36. 267-272 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo Ito,Yoneho Tabata: "Positronium Formation in CS_2 and C_6F_6 Mixtures with Triethylamine or Tetranydrofurane" Radiat.Phys.Chem.36. 253-257 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo Ito,Yoneho Tabata: "The role of Excited States in Antiーinhibition Effects of Positronium Formetion" Radiat.Phys.Chem.36. 285-290 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo Ito: "A new model of Positronium Formation Resonant Positronium Formation" J.Chem.Phys.93. 1021-1029 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo ITO: "The role of excited states in anti-inhibition effects of fluorinated benzenes." J.Radation Physics and Chemistry.

    • Related Report
      1989 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo ITO: "Positronium Formation in CS_2 and C_6F_6 mixtures with triethylamine or tetrahydrofurane" J.Radat.Phys.Chem.

    • Related Report
      1989 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo ITO: "Competitive effects of electron scavenger CH_2Cl_2 with C_6F_<6′> C_6H_5F and CS_2 on positronium formation in cyclohexane." J.Radiat.Phys.Chem.

    • Related Report
      1989 Annual Research Report
  • [Publications] Zhang Zhicheng,Yasuo ITO: "A New model of positronium formation--Resonant Positronium Formation--" J.Phys.Chem.

    • Related Report
      1989 Annual Research Report

URL: 

Published: 1989-04-01   Modified: 2016-04-21  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi