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Mechanism of Oxygen Effect on Solid State Nuclear Track Detectors

Research Project

Project/Area Number 02680185
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field Nuclear engineering
Research InstitutionKobe University of Mercantile Marine

Principal Investigator

MIYAKE Hiroshi  Kobe Univ. Mer. Mar., Fac. Mer., Prof., 商船学部, 教授 (00031443)

Co-Investigator(Kenkyū-buntansha) YAMAUCHI Tomoya  Kobe Univ. Mer. Mar., Fac. Mer. Mar., Instruct., 商船学部, 助手 (40211619)
ODA Keiji  Kobe Univ. Mer. Mar., Fac. Mer. Mar., Ass. Prof., 商船学部, 助教授 (40169305)
Project Period (FY) 1990 – 1991
Project Status Completed (Fiscal Year 1991)
Budget Amount *help
¥2,000,000 (Direct Cost: ¥2,000,000)
Fiscal Year 1991: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1990: ¥1,500,000 (Direct Cost: ¥1,500,000)
KeywordsTrack Detector / Oxygen Effect / Latent Track / CR-39 / Dissolved-Oxygen Concentration / Diffusion Coeffcient / Life Time of Radicals
Research Abstract

Solid state nuclear track detectors, especially CR-39 plastic ones, are a useful tool to detect heavy charged particles and applied to many fields, such as radiation protection measurements, nuclear fusion study, space science, etc. However, the storage of these detectors in vacuum causes severe effects on the registration sensitivity. The oxygen dissolved in a detector plays an important role in the latent track formation. The purpose of this project is to clarify the mechanism of the "Oxygen Effect" and to develop improved detectors.
The oxygen concentration and the diffusion coefficient in CR-39 plastic were measured, and the relation between the oxygen concentration and the sensitivity of the detector was ascertained. Outgas rates of oxygen and some other components from CR-39 sheets commercially available were measured at room temperature with a quadrupole mass specrometer. Diffusion coefficients and oxygen concentrations dissolved at atmospheric pressure were evaluated to be(4-9)x10^<-9>cm^2/sec and(1-8)x10^<19>molecules/cm^3, respectively. The reduction rates of etch rate ratios through the storage in vacuum were given by a function of local pressures of oxygen dissolved in CR-39. These results supported the "oxygen setting model", quantitatively.
The life time of the radicals formed by alpha-particle irradiation in the sufficiently outgassed CR-39 was evaluated on the basis of the examination for etch pit recovery in radius due to the air exposure after the storage in vacuum. Radicals with a life time of about 40 minutes were found to be formed as well as radicals with a life time of less than a few minutes after irradiation. It was also found that the fractions of radicals with different life times depended on the lots of CR-39, the time of storage after production and the energy of incident particles.

Report

(3 results)
  • 1991 Annual Research Report   Final Research Report Summary
  • 1990 Annual Research Report
  • Research Products

    (7 results)

All Other

All Publications (7 results)

  • [Publications] 三宅 寛,山内 知也,小田 啓二: "CRー39飛跡検出器中の酸素濃度と拡散係数" 放射線. 16. 59-70 (1990)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1991 Final Research Report Summary
  • [Publications] T.Yamauchi,K.Oda and H.Miyake: "An Evaluation of the Radical Life-Time in CR-39 Track Detectors Outgassed under Vacuum" Nuclear Tracks and Radiation Measurements. 20. (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1991 Final Research Report Summary
  • [Publications] H. Miyake, K. Oda and T. Yamauchi: "Diffusion Coefficient and Concentration of Oxygen in CR-39 Track Detector" Hoshasen. Vol. 16, No. 3. 59-69 (1990)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1991 Final Research Report Summary
  • [Publications] T. Yamauchi, K. Oda and H. Miyake: "An Evaluation of the Radical Life-Time in CR-39 Track Detector Suffciently Outgassed Under Vacuum" Nucl. Tracks and Radiat. Meas.Vol. 20. (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1991 Final Research Report Summary
  • [Publications] T.Yamauchi,K.Oda and H.Miyake: "An Evaluation of the Radical LifeーTime in CRー39 Track Detectors Outgassed under Vacuum" Nuclear Tracks and Radiation Measurements. 20. (1992)

    • Related Report
      1991 Annual Research Report
  • [Publications] 三宅 寛、山内 知也、小田 啓二: "CRー39飛跡検出器中の酸素濃度と拡散係数" 放射線. 16,No.3. 59-70 (1990)

    • Related Report
      1990 Annual Research Report
  • [Publications] Tomoya YAMAUCHI,Keiji ODA and Hiroshi MIYAKE: "Oxygen Setting and Life Radicals in DRー39 Track Detector" Nuclear Tracks and Radication Measurements.

    • Related Report
      1990 Annual Research Report

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Published: 1990-04-01   Modified: 2016-04-21  

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