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Dynamical Study of Photoexcited States in Semiconductors by Means of Femtosecond Pump-and-Probe Spectroscopy

Research Project

Project/Area Number 03402007
Research Category

Grant-in-Aid for General Scientific Research (A)

Allocation TypeSingle-year Grants
Research Field 固体物性
Research InstitutionUniversity of Tsukuba

Principal Investigator

MASUMOTO Yasuaki  Institute of Physics, University of Tsukuba, Professor, 物理学系, 教授 (60111580)

Co-Investigator(Kenkyū-buntansha) MISHINA Tomobumi  Institute of Physics, University of Tsukuba, Research Associate, 物理学系, 助手 (10209744)
Project Period (FY) 1991 – 1992
Project Status Completed (Fiscal Year 1992)
Budget Amount *help
¥25,900,000 (Direct Cost: ¥25,900,000)
Fiscal Year 1992: ¥10,300,000 (Direct Cost: ¥10,300,000)
Fiscal Year 1991: ¥15,600,000 (Direct Cost: ¥15,600,000)
KeywordsFemtosecond / Pump-and-Probe Spectroscopy / Nonequilibrium Electron Distribution / Exciton / Coherent Phonon / Quantum Beat / Type-II Quantum Well / Excitonic Polariton / ZnP_2 / フェムト秒時間分解分光 / ワニエ励起子 / ポラリトン / チタンサファイアレーザー / ポラリトン量子ビート / 光学非線形性 / AlGaAsーAlAs / 超高速光非線形素子 / BiI_3 / 層状結晶 / ポンプ・プロ-ブ / コヒ-レントフォノン効果
Research Abstract

<Observation of nonequilibrium electrons in CdSe> Femtosecond pump-and-probe spectroscopy was applied to highly excited CdSe. Nonequilibrium distribution of electrons was observed for 50 fs. <Exciton-hole collision in type-II AlGaAs-AlAs quantum wells> Exciton-hole collision rate was measured by means of time-resolved degenerate four-wave mixing. Phase relaxation of excitons is dominated by the collision between the excitons and long-lived holes. <Observation of coherent optical phonons in BiI_3> Resonant coherent lattice vibrations in the vicinity of the indirect absorption edge in a BiI_3 lattice crystal are observed in a femtosecond pump-and-probe experiment. The coherent transverse optical lattice vibration, which has a period of 300 fs, continues for more than 100 cycles. <Quantum beats of Wannier excitons and excitonic polaritons> Quantum beats of Wannier excitons and excitonic polaritons were observed in ZnP_2. Qunatum beat originates from Wannier excitons whose principal quantum numbers n are 2,3 and 4. Polariton quantum beat was also observed as a result of interference of both upper and lower polaritons around the n =1 resonance.

Report

(3 results)
  • 1992 Annual Research Report   Final Research Report Summary
  • 1991 Annual Research Report
  • Research Products

    (24 results)

All Other

All Publications (24 results)

  • [Publications] Y.Masumoto: "Intraband Energy Relaxation of Hot Carriers in CdSe" Journal of Luminescence. 48&49. 189-192 (1991)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Mishina: "Exciton-Hole Collision in Staggered Type-II AL_<0.34>Ga_<0.66>As/AlAs Multiple Quantum Wells" Physical Review B. 44. 5664-5667 (1991)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.Masumoto: "Band Gap Renormalization and Optical Gain Formation in Highly Excited CdSe" Journal of Crystal Growth. 117. 732-737 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Mishina: "Observation of Coherent Optical Phonons in BiI_3" Physical Review B. 46. 4229-4232 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] F.Sasaki: "Ultrafast Pump-and-Probe Spectroscopy in CdSe:Hot Carrier and Exciton Dynamics" Physical Review B. 46. 6750-6759 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Kawazoe: "Spin Relaxation Process of Holes in Type II Al_<0.34>Ga_<0.66>As/AlAs Multiple Quantum Wells" Physical Review B. 47. (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.Masumoto and F.Sasaki: "Intraband Energy Relaxation of Hot Carriers in CdSe" J.Lumin. 48 & 49. 189 (1991)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Mishina and Y.Masumoto: "Exciton-Hole Collision in Staggered Type-II Al_<0.34>Ga_<0.66>As/AlAs Multiple Quantum Wells" Phy.Rev.B 44. 5664 (1991)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.Masumoto, B.Fluegel, K.Meissner, S.W.Koch, R.Binder, A.Paul and N.Peyghambarian: "Band Gap Renormalization and Optical Gain Formation in Highly Excited CdSe" J.Crystal Growth. 117. 732 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Mishina, Y.Masumoto, B.Fluegel, K.Meissner and N.Peyghambarian: "Observation of Coherent Optical Phonons in BiI_3" Phys.Rev.B 46. 4229 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] F.Sasaki, T.Mishina and Y.masumoto: "Ultrafast Pump-and-Probe Spectroscopy in CdSe: Hot Carrier and Exciton Dynamics" Phys.Rev.B 46. 6750 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] T.Kawazoe, Y.Masumoto and T.Mishina: "Spin Relaxation Process of Holes in Type II Al_<0.34>Ga_<0.66>As/AlAs Multiple Quantum Wells" Phys.Rev.B 47,April 15. (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.Masumoto: "Band Gap Renormalization and Pptical Gain Formation in Highly Excited CdSe" Journal of Crystal Growth. 117. 732-737 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] T.Mishina: "Observation of Coherent Optical Phonons in Bil3" Physical Review B. 46. 4229-4232 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] T.Mishina: "Picosecond Repetitive Optical Switching Using Type II Multiple Quantum well Structures" Japanese Journal of Applied Physics. 31. 343-345 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] F.Sasaki: "Ultrafast Pump-and-Probe Spectroscopy in CdSe:Hot-Carrier and Exciton Dynamics" Physical Review B. 46. 6750-6759 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] B.D.Fluegel: "Experimental and Theoretical Investigation of Femtosecond Carrier Relaxation in CdSe" Solid State Communications. 83. 17-19 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] T.Kawazoe: "Spin Relaxation Process of Holes in Type II Al0.34Ga0.66As/AlAs Multiple Quantum Wells" Physical Review B.

    • Related Report
      1992 Annual Research Report
  • [Publications] Yasuaki Masumoto: "Intraband Enargy Relaxation of Hot Carriers CdSe" Journal of Luminescence. 48&49. 189-192 (1991)

    • Related Report
      1991 Annual Research Report
  • [Publications] Tomobumi Mishina: "ExcitonーHole Collision in Staggered TypeーII Al_0 _<34>Ga_0 _<66>As/AlAs Multiple Quantum Wells" Phisical Review B. 44. 5664-5667 (1991)

    • Related Report
      1991 Annual Research Report
  • [Publications] Fumio Sasaki: "Nonequilibrium Distribution of Hot Carriers in a CdSe Thin Film" Superlattices and Microstructures.

    • Related Report
      1991 Annual Research Report
  • [Publications] Tetsuro Wamura: "SizeーDependent Homogeneous Linewidth of Z_3 Exciton Absorption Spectra in CuCl Microcrystals" Applied Phisics Letters. 59. 1758-1760 (1991)

    • Related Report
      1991 Annual Research Report
  • [Publications] Tomobumi Mishina: "Observation of Coherent Optical Phonons in BiI_3" Physical Review B.

    • Related Report
      1991 Annual Research Report
  • [Publications] Fumio Sasaki: "Ultrafast PumpーandーProbe Spectroscopy in Cdse:Hot Carrier and Exciton Dynamics" Physical Review B.

    • Related Report
      1991 Annual Research Report

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Published: 1991-04-01   Modified: 2016-04-21  

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