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Optical Microscopic Faraday Rotation Study on Magnetization Relaxation in the Spin Systems Having Ordered Structures with Non-trivial Degeneracy

Research Project

Project/Area Number 03452034
Research Category

Grant-in-Aid for General Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 固体物性
Research InstitutionTOKYO INSTITUTE OF TECHNOLOGY

Principal Investigator

IIO Katsunori  Tokyo Institute of Technology, Faculty of Science, Professor, 理学部, 教授 (20016132)

Co-Investigator(Kenkyū-buntansha) KATO Tetsuya  Tokyo Institute of Technology, Faculty of Science, research associate, 理学部, 助手 (00224519)
NAGATA Kazukiyo  Tokyo Institute of Technology, Faculty of Science, Professor, 理学部, 教授 (00013491)
Project Period (FY) 1991 – 1993
Project Status Completed (Fiscal Year 1993)
Budget Amount *help
¥6,800,000 (Direct Cost: ¥6,800,000)
Fiscal Year 1993: ¥200,000 (Direct Cost: ¥200,000)
Fiscal Year 1992: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1991: ¥5,800,000 (Direct Cost: ¥5,800,000)
KeywordsSlow dynamics / Faraday rotation / Spin glass / Optical microscopic study / Magnetic phase diagram / magneto optics / competing system / Ferroelectricity / フアラデー効果 / 磁気相転移 / ランダム磁場効果 / フアラデ-効果
Research Abstract

In condensed matter with competing interactions, inhomogeneity in specimens disturbs observation of true feature of dynamic and static properties of their multi-degenerate ordered states. To remove this difficulty, we have developed a new experimental system measuring magnetization and its long time decay on a homogeneous region extracted by means of a microscope. For the term of this research project over three years, the main task was to construct an apparetus equiped with a superconducting magnet for optical access for measuring magneto-optical effects, such as Faraday rotation and optical birefringence and to do that with an optical microscope. The final aim was to link those two systems together. Although the former system has already been operated, the latter is just settled recently.
On the other hand, a couple of research programs associated with this study bring about important results. In a mixed compound with Ising -like interaction, Fe_<1-x>MG_xCl_2, long time decay of remanent magnetization due to the random field effect and spin glass behavior could be characterized. Furthermore, as new problems inherent to competing systems, the successive phase transition accompanied with the first order transition in hexagonal layr type MnX_2(X=Br, I)were clarified with respect to magnetic structures of each phase and a mechanism of successive transition. Ferroelectricity was found in the KNICl_3 type lattice with the space group P6_3cm. The latter finding opened a new paradigm in which the physics reflecting coexistence of antiferromagnetism and ferroelectricity is attracted considerable attention. Experimental system with superconducting magnet was succeeded in measuriong the magnetic phase diagram of a triangular lattice antiferromagnet RbMnBr_3 and a layr type magnet with competing interactions NiBr_2. In this way, it takes further effort to fulfilll our project. However the prospect of the present project is rather widely opened.

Report

(4 results)
  • 1993 Annual Research Report   Final Research Report Summary
  • 1992 Annual Research Report
  • 1991 Annual Research Report
  • Research Products

    (34 results)

All Other

All Publications (34 results)

  • [Publications] Yasuaki Oohara: "Birefringence Study of the Criticality of the Magnetic Phase Transition in RbNiCl_3" J.Phys.Soc.Jpn.60[12]. 4282-4287 (1991)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Katsunori Iio: "Time-Dependent Magnetic Phenomena in Dilute Antiferromagnets Fe_<1-x>Mg_xCl_2 Exhibiting Random Field Ising Model and Spin Glass behaviour" ATP Conference Proceedings{Slow dynamics in Condensed Matter,Eds.:K.Kawasaki,M.Tokuyama & T.Kawakatsu}. 421-422

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Tetsuya Kato: "Birefringence Study on Structural and Magnetic Phase Transitions of RbMnBr_3" J.Phys.Soc.Jpn.61[1]. 275-285 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] 飯尾勝矩: "磁気複屈折;スピン短距離秩序を捉える光技術" 日本物理学会誌. 47[5]. 383-387 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] 飯尾勝矩: "中性子回折による六方晶AX_2型競合磁気系の一次転移を伴う逐次相転移の研究" 原研施設利用共同研究成果報告書. G21. 366-368 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Toshiharu Mitsui: "Thermal Expansion Measurement in CsNiBr_3 by Rotating Mirror Method" J.Magn.Magn.Mat.104-107. 819-820 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Kazuhisa Kakurai: "Magnetic Correlation in the quasi one-dimensional Antiferro-magnetic ABX_3 Systems" J.Magn.Magn.Mat.104-107. 856-857 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Kenji Nakajima: "Quasielastic and inelastic Neutron Scattering on RbNiCl_3" J.Phys.Soc.Jpn.6[9]. 3355-3360 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Taiju Tsuboi: "Time Resolved Luminescence Spectra of Rb_2MnCl_4" Phys.Stat.Sol.b170. K55-K59 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Taiju Tsuboi: "Inter-Sublattice Energy transfer in Rb_2MnCl_4 AntiferroMagnetic Crystal" Phys.Stat.Sol.b179. K47-K51 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Tetsuya Kato: "Neuton Diffraction Study of the Magnetic Phase Diagram of RbMnBr_3-Observation of the Critical line of Field-Induced Phase Transition" J.Phys.Soc.Jpn.62[10]. 3384-3387 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Toshiharu Mitsui: "Ferroelectric phase Transition in Hexagonal Antiferromagnet RbFeBr_3 with Linear Chains of Face Sharing Octahedra(FeBr_6)^4" J.Phys.Soc.Jpn.63[3]. 839-842 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Yasuaki Oohara: "Birefringence Study of the Criticality of the Magnetic Phase Transition in RbNiCl_3" J.Phys. Soc. Jpn.60[12]. 4282-4287 (1991)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Katsunori Iio: "Time-Dependent Magnetic Phenomena in Dilute Antiferromagnets Fe_<1-x>Mg_xCl_2 Exhibiting Random Field Ising Model and Spin Glass behavior" ATP Conference Proceedings {Slow dynamics in Condensed Matter, Eds. : K.Kawasaki, M.Tokuyama & T.Kawakatsu}. 421-422

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Tetsuya Kato: "Birefringence Study on Structural and Magnetic Phase Transitions of RbMnBr_3" J.Phys. Soc. Jpn.61[1]. 275-285 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Toshiharu Mitsui: "Thermal Expansion Measurement in CsNiBr_3 by Rotating Mirror Method" J.Magn. Magn. Mat.104-107. 819-820 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Kazuhisa Kakurai: "Magnetic Correlation in the quasi one-dimensional Antiferromagnetic ABX_3 Systems" J.Magn. Magn. Mat.104-107. 856-857 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Kenji Nakajima: "Quasielastic and inelastic Neutron Scattering on RbNiCl_3" J.Phys. Soc. Jpn.6[9]. 3355-3360 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Taiju Tsuboi: "Time Resolved Luminescence Spectra of Rb_2MnCl_4" Phys. Stat. Sol.(b)170. K55-K59 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Taiju Tsuboi: "Inter-Sublattice Energy transfer in Rb_2MnCl_4 Antiferro-Magnetic Crystal" Phys. Stat. Sol.(b)179. K47-k51 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Tetsuya Kato: "Neuton Diffraction Study of the Magnetic Phase Diagram of RbMnBr_3-Observation of the Critical line of Field-Induced Phase Transition" J.Phys. Soc. Jpn.62[10]. 3384-3387 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Toshiharu Mitsui: "Ferroelectric phase Transition in Hexagonal Antiferromagnet RbFeBr_3 with Linear Chains of Face Sharing Octahedra (FeBr_6)^4" J.Phys. Soc. Jpn.63[3]. 839-842 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Taiju Tsuboi: "Inter-Sublattice Energy Transfer in Rb_2MnCl_4 Antiferromagnetic Crystal" Phys,stat.Sol.(b)179. K47-K51 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] Tetsuya Kato: "Neutron Diffraction Study of the Magnetic Phase Diagram od RbMnBr_3" J.Phys.Soc.Jpn.62. 3384-3387 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] Toshiharu Mitsui: "Ferroelectric Phase Transition in Hexagonal Antiferromaagnet RbFeBr_3 with Linear Chains of Face Sharing Octahedra(FeBr6)^4" J.Phys.Soc.Jpn.63. 839-842 (1994)

    • Related Report
      1993 Annual Research Report
  • [Publications] 飯尾 勝矩: "磁気複屈析:スピン短矩離秩序を捉える光技術" 日本物理学会誌. 47. 383-387 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Toshiharu Mitsui: "Thermal Expansion Measurement in CsNiCl_3 by a New Rotating-Mirror Method" J. Magn. Magn. Mat.104-107. 819-820 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Tetsuya Kato: "Birefringence Study on Structural and Magnetic phase Tnansitions of Rb Mn Br_3" J.Phy. Soc. Jpn.61. 275-285 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Hidekazu Tanaka: "Successive Magnetic Phase Tnansitions in RBVBr_3" J. Phy. Soc. Jpn.61. 3292-3302 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Hidekazu Tanaka: "Magnetic Properties of Rb_<1-X> Kx Nicl_3,RbVBr_3,CsNiI_3" J. Magn. Magn. Mat.104-107. 829-830 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Kenji Nakajima: "Quasielastic and lnelastic Neutron Scattering on RbNicl_3" J. Phy. Soc. Jpn.61. 3355-3360 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Yasuaki Oohara: "Birefringence Study of the Criticality of the Magnetic Phase Transition in RbNiCl_3" J.Phys.Soc.Jpn.60. 4280-4285 (1991)

    • Related Report
      1991 Annual Research Report
  • [Publications] Tetsuya Kato: "Birefringence Study on Struatural and Magnetic Phase Transitions of RbMnBr_3" J.Phys.Soc.Jpn.61. 275-285 (1992)

    • Related Report
      1991 Annual Research Report
  • [Publications] Katsunori Iio: "TimeーDependent Magnetic Phenomena in Dilute Antirerromagnets Fe_<1-x>Mg_xCl_2 Exhibiting Random Field Ising Model and Spin Glass Behaviours" Slow Dynamics in Condensed Matter(1st Tohwa University International Symposium). 93 (1991)

    • Related Report
      1991 Annual Research Report

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Published: 1991-04-01   Modified: 2016-04-21  

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