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NMR Study of Magnetic Property in Heavy Fermion Superconductor CeCu_2Si_2

Research Project

Project/Area Number 03452041
Research Category

Grant-in-Aid for General Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 固体物性
Research InstitutionOsaka University

Principal Investigator

KITAOKA Yoshio  Osaka Univ., Faculty of Eng. Sci., Assoc. Prof., 基礎工学部, 助教授 (70110707)

Co-Investigator(Kenkyū-buntansha) ASAYAMA Kunisuke  Osaka Univ., Faculty of Eng. Sci., Prof., 基礎工学部, 教授 (20029416)
Project Period (FY) 1991 – 1992
Project Status Completed (Fiscal Year 1992)
Budget Amount *help
¥5,900,000 (Direct Cost: ¥5,900,000)
Fiscal Year 1992: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 1991: ¥4,800,000 (Direct Cost: ¥4,800,000)
KeywordsHeavy Fermion / Superconductivity / Magnetic Transition / CeCu_2Si_2 / NMR / NQR
Research Abstract

The magnetic correlation in the heavy fermion superconductor, CeCu<@D22.02@>D2Si<@D22@>D2 and Th-doped Ce<@D21-x@>D2Th<@D2x@>D2Cu<@D22.2@>D2Si<@D22@>D2, has been investigated by Cu nuclear magnetic resonance (NMR) and nuclear quadrupoleresonance (NQR). For CeCu<@D22.02@>D2Si<@D22@>D2 with T<@D2c@>D2 = 0.72KJ, a "magnetic transition" has been found at around 0.8 K in applied fields up to 3.5T. Below the transition temperature, Cu NMR loses the intensity suddenly without any broadening and shift of the spectrum, and the spin-echo decay rate, 1/T<@D22@>D2, at H = 13.3kOe, increases with decreasing temperature, which is different from the behavior expected in a static magnetically ordered state. The "magnetic transition" just above T<@D2c@>D2 is quite unusual in a sense that the ordered state may not be in a completely static regime, but possesses some dynamic aspect. We have constructed a magnetic phase diagram in the field-temperature plane for CeCu<@D22.02@>D2Si<@D22@>D2. To ensure the magnetic instability in CeCu<@D22@>D2 we have investigated a magnetic and superconducting phase diagram of Th-doped Ce<@D21-x@>D2Th<@D2x@>D2Cu<@D22.2@>D2Si<@D22@>D2. Static magnetic ordering with T<@D2n@>D2 = 2.4K and 4.5K for x=0.08 and 0.12, respectively, is evidenced by a pronounced broadening of the <@D163@>D1Cu-NQR and -NMR spectra and a mean-field type of anomaly in the specific heat. In contrast, for the lightly Th-doped compounds with x (] SY.ltoreq.[) 0.064, there has been observed neither any signature of a broadening of the NQR and NMR spectra nor an anomaly of the specific heat, but a dramatic reduction of the NMR and NQR intensities below a temperature ranging from 0.9 K to 1.3 K upon increasing Th-content. It is emphasized that the unusual "magnetic transition" found in undoped and lightly Th-doped CeCu<@D22.2@>D2Si<@D22@>D2 should be distinguished from the static magnetic ordering in the heavily Th-doped systems.

Report

(3 results)
  • 1992 Annual Research Report   Final Research Report Summary
  • 1991 Annual Research Report
  • Research Products

    (15 results)

All Other

All Publications (15 results)

  • [Publications] Y.KITAOK: "Magnetic and Superconducting Phase Diagram of Heavy Fermion Superconductors Ce_<1->xThxCu_<2.2>Si_2-Cu NMR and NQR Study-" J.of Physical Socity of Japan. 60. 2122-2126 (1991)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] H.NAKAMURA: "Nuclear magnetic resonance study of magnetic correlation in the heavy-fermion superconductor CeCu_2Si_2" J.Phys.Condens Matter. 4. 473-486 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] K.ASAYAMA: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series. 8. 205-214 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.KITAOKA: "NMR Study of Weak Magnetism and Superconductivity in Heavy Fermion Systems" Physica B. (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y. Kitaoka: "Magnetic and Superconducting Phase Diagram of Heavy Fermion Superconductors Ce_<1-x>Th_xCu_<2.2>Si_2 --Cu NMR and NQR Study--" J. Phys. Soc. Jpn.60. 2122-2126 (1991)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] H. Nakamura: "Nuclear magnetic resonance study of magnetic correlation in the heavy-fermion superconductor CeCu_2Si_2" J. Phys. Condens Matter. 4. 473-486 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] K. Asayama: "NMR Measurements on Cerium and Uranium Compounds" Jpn. J. Appl. Phys. Series. 8. 205-214 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y. Kitaoka: "NMR Study of Weak Magnetism and Superconductivity in Heavy Fermion Systems" Physica B.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1992 Final Research Report Summary
  • [Publications] Y.KITAOKA: "Magnetic and Superconducting Phase Diagram of Heavy Fermion Supercon ductors Ce_<1-x>ThxCu_<2.2>Si_2ーCu NMR and NQR Studyー" J.of Physical Society of Japan. 60. 2122-2126 (1991)

    • Related Report
      1992 Annual Research Report
  • [Publications] K.NAKAMURA: "Nuclear magnetic resonance study of magnetic correlation in the heavy-fermion superconductor CeCu_2Si_2" J.Phys. Condens Matter. 4. 473-486 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] K.ASAYAMA: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series. 8. 205-214 (1993)

    • Related Report
      1992 Annual Research Report
  • [Publications] Y.KITAOKA: "NMR Study of Weak Magnetism and Superconductivity in Heavy Fermion Systems" Physica B. (1993)

    • Related Report
      1992 Annual Research Report
  • [Publications] 北岡 良雄: "Magnetic and Superconducting Phase Diagram of Heavy Fermion Superconductors Ce_<1ーX>Th_XCu_<2.2>Si_2 ーCu NMR and NOR Studyー" Journal of the Physical Society of Japan. 60. 2122-2126 (1991)

    • Related Report
      1991 Annual Research Report
  • [Publications] 中村 裕之: "NMR Study of Magnetic Correlation in Heavy Fermion Superconductor CeCu_2Si_2" Journal of Physics:Condens.Matter. (1992)

    • Related Report
      1991 Annual Research Report
  • [Publications] 教学 正文: "Magnetic Instability of the Gap State in CeNiSn at Very Low Temperature" Journal of the Physical Society of Japan. 61. 43-46 (1992)

    • Related Report
      1991 Annual Research Report

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Published: 1991-04-01   Modified: 2016-04-21  

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