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NMR Study of the New Antiferromagnetic Heavy Fermion Superconductors UM_2Al_3 (M=Ni and Pd)

Research Project

Project/Area Number 04452051
Research Category

Grant-in-Aid for General Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 物性一般(含極低温・固体物性に対する理論)
Research InstitutionOsaka University

Principal Investigator

ASAYAMA Kunisuke  Osaka Univ., Faculty of Eng.Sci., Prof., 基礎工学部, 教授 (20029416)

Co-Investigator(Kenkyū-buntansha) ZHENG Guo-qing  Osaka Univ., Faculty of Eng.Sci., Res.Assoc., 基礎工学部, 助手 (50231444)
KITAOKA Yoshio  Osaka Univ., Faculty of Eng.Sci., Assoc.Prof., 基礎工学部, 助教授 (70110707)
Project Period (FY) 1992 – 1993
Project Status Completed (Fiscal Year 1993)
Budget Amount *help
¥6,300,000 (Direct Cost: ¥6,300,000)
Fiscal Year 1993: ¥1,300,000 (Direct Cost: ¥1,300,000)
Fiscal Year 1992: ¥5,000,000 (Direct Cost: ¥5,000,000)
KeywordsNMR / Heavy Fermion / Superconductor / Magnetic Transition / NQR / UPd_2Al_3 / UNi_2Al_3 / CePd_2Al_3 / 重い電子系超伝導 / 核磁気共鳴
Research Abstract

NMR and NQR studies on two newly-discovered antiferromagnetic heavy-fermion superconductors, UNi_2Al_3 and UPd_2Al_3 with T_c = 1 and 2K and T_N =4.2K and 14K, respectively, have revealed that the type of magnetic fluctuation and spin structure of these two compounds belong to different classes. UNi_2Al_3 possesses a unique feature where the low-energy spin fluctuations survive in a low-T region, keeping a strong wave-number dependence. This is the first case in the magnetic actinide system. The spin structure is presumably of a helical spin type where the magnetic field causes a partial canting of an assembly of spins to the direction of the magnetic easy plane. In UPd_2Al_3, there emerges a partial energy gap on the Fermi surface below T_N, while the low temperature properties are governed by the Fermi liquid excitation associated with the residual density of states. The spin structure is of a commensurate type where the ferromagnetic sheets directed in the magnetic easy plane couple antiferromagnetically along the hexagonal caxis. It should, however, be noted that the magnetic moments, 0.85mu_B for UPd_2Al_3 is by one order of magnitude larger than 0.03mu_B for URu_2Si_2, while the magnetic or electronic energy gap is rather by one-half smaller.
The unstablesuperconducting property of UNi_2Al_3 in powder sample in comparison with UPd_2Al_3 may be related to the unique magnetic nature of UNi_2Al_3. The superconductivity in UPd_2Al_3 is in a clean limit with dominant singlet pairing. This means that the impurity scattering plays a minor role and hence the pseudo-spin momentum is preserved in the pairing state. The superconducting energy gap is of an anisotropic type where the gap vanishes on lines at the Fermi surface. Apparently, the unique relaxation behavior in the heavy fermion superconductors is consistently described in terms of a universal gapless model, irrespective of the variety of the magnetic and normal state properties.

Report

(3 results)
  • 1993 Annual Research Report   Final Research Report Summary
  • 1992 Annual Research Report
  • Research Products

    (21 results)

All Other

All Publications (21 results)

  • [Publications] Y.KITAOKA: "NMR study of weak magnetism and superconductivity in heavy-fermion systems" Physica B. 186-188. 229-235 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Kyogaku: "^<27>Al NMR study of the new heavy-fermion superconductors UM_2Al_3(M=Ni,Pd)" Physica B. 186-188. 285-287 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Y.Kitaoka: "NMR investigations of the ground state in the gap-type Kondo lattice CeNiSn and the low carrier system Yb_4As_3" Physica B. 186-188. 431-433 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] K.Asayama: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series.8. 205-214 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Kyogaku: "NMR and NQR Studies of Magnetism and Superconductivity in the Antiferromagnetic Heavy Fermion Superconductivity UM_2Al_3(M=Ni and Pd)" J.Phys.Soc.Jpn. 62. 4016-4030 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] H.TOU: "Al NMR Study of the Antiferromagnetic Heavy Fermion Antiferromagnet CePd_2Al_3" J.Phys.Soc.Jpn.63(発表予定). (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Y.Kitaoka et al.: "NMR study of weak magnetism and superconductivity in heavy-fermion systems" Physica. B186-188. 229-235 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Kyogaku et al.: "Al^<27>N NMR study of the new heavy-fermion superconductors UM_2Al_3 (M = Ni, Pd)" Physica. B186-188. 285-287 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Y.Kitaoka et al.: "NMR investigations of the ground state in the gap-type Kondo lattice CeNiSn and the low carrier system Yb_4As_3" Physica. B186-188. 431-433 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] K.Asayama et al.: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series 8. 205-214 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Kyogaku et al.: "NMR and NQR Studies of Magnetism and Superconductivity in the Antiferromagnetic Heavy Fermion superconductivity UM_2Al_3 (M=Ni and Pd)" J.Phys.Soc.Jpn.62. 4016-4030 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] H.Toh et al.: "Al NMR Study of the Antiferromagnetic Heavy Fermion Antiferromagnet CePd_2Al_3" J.Phys.Soc.Jpn.(to be published).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] Y.KITAOKA: "NMR study of weak magnetism and superconductivity in heavy-fermion systems" Physica B. 186-188. 229-235 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] M.Kyogaku: "^<27>Al NMR study of the new heavy-fermion superconductors UM_2Al_3(M=Ni,Pd)" Physica B. 186-188. 285-287 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] Y.Kitaoka: "NMR investigations of the ground state in the gap-type Kondo lattice CeNiSn and the low carrier system Yb_4As_3" Physica B. 186-188. 431-433 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] K.Asayama: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series.8. 205-214 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] M.Kyogaku: "NMR and NQR Studies of Magnetism and Superconductivity in the Antiferromagnetic Heavy Fermion Superconductivity UM_2Al_3(M=Ni and Pd)" J.Phys.Soc.Jpn. 62. 4016-4030 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] H.TOU: "Al NMR Study of the Antiferromagnetic Heavy Fermion Antiferromagnet CePd_2Al_3" J.Phys.Soc.Jpn.63(発表予定). (1994)

    • Related Report
      1993 Annual Research Report
  • [Publications] K.ASAYAMA: "NMR Measurements on Cerium and Uranium Compounds" Jpn.J.Appl.Phys.Series. 8. 205-214 (1993)

    • Related Report
      1992 Annual Research Report
  • [Publications] M.KYOGAKU: "Magnetic Instability of the Gap State in CeNiSn at Very Low Temperature" J.of.Physical Socity of Japan. 61. 43-46 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Y.KITAOKA: "NMR Study of Weak Magnetism and Superconductivity in Heavy Fermion Systems" Physica B. (1993)

    • Related Report
      1992 Annual Research Report

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Published: 1992-04-01   Modified: 2016-04-21  

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