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Fermi surface and anti-ferromagnetic order in 2D organic condutors

Research Project

Project/Area Number 04640322
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 固体物性
Research InstitutionInstitute for Materials Research, Tohoku University

Principal Investigator

TOYOTA Naoki  Instirite for Materials Research, Associate Prof., 金属材料研究所, 助教授 (50124607)

Co-Investigator(Kenkyū-buntansha) WATANABE Yosuke  Institute for Materials Research, Assistant, 金属材料研究所, 助手 (00167181)
SASAKI Takahiko  Institute for Materials Research, Assistant, 金属材料研究所, 助手 (20241565)
LANG Michael  東北大学, 金属材料研究所, 助手 (60240397)
Project Period (FY) 1992 – 1993
Project Status Completed (Fiscal Year 1993)
Budget Amount *help
¥2,400,000 (Direct Cost: ¥2,400,000)
Fiscal Year 1993: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1992: ¥1,600,000 (Direct Cost: ¥1,600,000)
KeywordsOrganic conductor / BEDFTTF Salt / (BEOT-TTF)_2KHg(SCN)_4 / anti-ferromagnetic metal, quantum oscillation / 量子振動効果 / スピン密度波
Research Abstract

This research aims to study an organic conductor (BEDT-TTF) 2KHg-(SCN)4 which takes a phase transition from paramagnetic normal metal to antiferromagnetic metal at about 10K.This material, a typical quasi-two-dimensional conductor as well as other BEDT-TTF salts, shows quite unique properties such as, anomalous magnetoresistance below the transition point, splitting in the de-Haas quantum oscillations, and the reentrance to the normal metallic state above twenty several Tesla at low temperatures. We have studied these properties from the viewpoint of low-dimensional electronic states where closed 2D and open 1D Fermi surfaces coexist. We summarize the results as follows.
1. We have found sharp increase in the Hall coefficient below the transition temperature. This suggests that the significant amount of carriers disappears, being not inconsistent with the appearance of spin- or charge-density-wave.
2. We have systematically explained the origin of the splitting of de-Haas oscillations in terms of the positive (ferromagnetic) exchange interaction acting between the lower and upper Zeeman levels.
3. Detailed studies for the in-plane current-direction dependence and the angular dependent oscillations of the magnetoresistance suggests that a new open orbit appears in the low temperature phase, pointing to the possible lattice displacement accompanied with the transition. We have pointed out the model on a basis of the coexistent SDW and CDW.

Report

(3 results)
  • 1993 Annual Research Report   Final Research Report Summary
  • 1992 Annual Research Report
  • Research Products

    (21 results)

All Other

All Publications (21 results)

  • [Publications] T.Sasaki: "Magnetic Phase Diagram of the Organic Conductor α-(BEDT-TTF)_2KHg(SCN)_4" Solid State Commun.82. 447-451 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Lang: "Magnetic Penetration Depth of k-(BEDT-TTF)_2 CuN(CN)_2Br determined by the Reuersible Magnetization" Phys.Rev.B. 46. 5822-5825 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Lang: "Magnetic Penetration Depth of k-(BEDT-TTF)_2 Cu(NCS)_2:Strong Euidence for Conuentional Cooper Paining" Phys.Rev.Lett. 69. 1443-1446 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki: "Hall Effect in the Organic conductor α-(BEDT-TTF)_2KHg(SCN)_4 where BEDT-TTF is bis(ethylenedithio) tetrgthiafulvalene" Phys.Rev.B. 48. 1928-1931 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki: "Splitting Wave Form of the Maguetic Quantum Oscillations in α-(BE-DT-TTF)_2KHg(SCN)_4,where BEDT-TTF is bis(ethylene) dithio tetrathiafulualem" Phys.Rev.B. 48. 11457-11460 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki: "Anisotropic Galvanomagnetic Effect in the Quasi-Two-Dimensional Organic Conductor α-(BEDT-TTF)_2KHg(SCN)_4" Phys.Rev.B. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki et al.: "Magnetic Phase Diagram of the Organic Conductors alpha-(BEDT-TTF)_2KHg(SCN)_4" Solid State Commun. 82. 477-451 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Lang et al.: "Magnetic Penetration Depth of kappa-(BEDT-TTF)_2 CuN(CN)_2Br, determined by the reversible magnetization" Phys.rev.B46. 5822-5825 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] M.Lang et al.: "Magnetic Penetration Depth of kappa-(BEDT-TTF)_2 Cu(NCS)_2 : Strong Evidence for Conventional Cooper Pairing" Phys.Rev.Lett.69. 1443-1446 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki et al.: "Hall Effect in the Organic Conductor alpha-(BEDT-TTF)_2KHg(SCN)_4 where BEDT-TTF is bis(ethylene) dithiotetrathisfulvalene" Phys.Rev.B48. 1928-1931 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki et al.: "Splitting Wave Form of the Magnetic Quantum Osci-lattions in alpha-(BEDT-TTF)_2KHg(SCN)_4, where BEDT-TTF is bis(ethylene) dithiotetrathiafulvalene" Phys.Rev.B48. 11457-11460 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki et al.: "Anisotropic Galvanomagnetic Effect in the Quasi-Two-Dimensional Organic Conductor alpha-(BEDT-TTF)_2KHg(SCN)_4, where BEDT-TTF is bis(ethylene) dithiotetrathiafulvalene" Phys.Rev.B. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1993 Final Research Report Summary
  • [Publications] T.Sasaki: "Magnetic Phase Diagram of the Organic Conductor α-(BEDT-TTF)_2KHg(SCN)_4" Solid State Commun.82. 447-451 (1992)

    • Related Report
      1993 Annual Research Report
  • [Publications] M.Lang: "Magnetic Penetration Depth of κ-(BEDT-TTF)_2CuN(CN)_2Br determined by the Reversible Magnetization" Phys.Rev.B. 46. 5822-5825 (1992)

    • Related Report
      1993 Annual Research Report
  • [Publications] M.Lang: "Magnetic Penetration Depth of κ-(BEDT-TTF)_2Cu(NCS)_2:Strong Evidence for Conventional Cooper Pairing" Phys.Rev.Lett. 69. 1443-1446 (1992)

    • Related Report
      1993 Annual Research Report
  • [Publications] T.Sasaki: "Hall Effect in the Organic conductor α-(BEDT-TTF)_2KHg(SCN)_4 where BEDT-TTF is bis(ethylenedithio)tetrathiafulvalene" Phys.Rev.B. 48. 1928-1931 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] T.Sasaki: "Splitting Wave Form of the Magnetic Quantum Oscillations in α-(BEDT-TTF)_2KHg(SCN)_4,where BEDT-TTF is bis(ethylene)dithio tetrathiafulvalene" Phys.Rev.B. 48. 11457-11460 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] T.Sasaki: "Anisotropic Galvanomagnetic Effect in the Quasi-Two-Dimensional Organic Conductor α-(BEDT-TTF)_2KHg(SCN)_4" Phys.Rev.B. (印刷中).

    • Related Report
      1993 Annual Research Report
  • [Publications] T.Sasaki,N.Toyota: "Magnetic Phase Diagram of the Organic Gonductor α-(BEDT-TTF)_2KHg(SCN)_4" Solid State Commun.82. 447-451 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] M.Lang,N.Toyota T.Sasaki,H.Sato: "Magnetic Penetration Depth of K-(BEDT-TTF)_2Cu〔N(CN)_2〕Br,determined by the recersible magnetization" Phys.Rev.B. 46. 5822-5825 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] M.Lang,N.Toyota T.Sasaki,H.Sato: "Magnetic penetration depth of K-(BEDT-TTF)_2Cu(NCS)_2:Strong evidence for conventional cooper pairing" Phys.Rev.Lett. 69. 1443-1446 (1992)

    • Related Report
      1992 Annual Research Report

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Published: 1992-04-01   Modified: 2016-04-21  

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