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Nonlocal Theory of Linear and Nonlinear Optical Responses

Research Project

Project/Area Number 04640368
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 物性一般(含極低温・固体物性に対する理論)
Research InstitutionOsaka University

Principal Investigator

CHO Kikuo  Osaka University, Faculty of Engineering Science, Professor, 基礎工学部, 教授 (60013489)

Co-Investigator(Kenkyū-buntansha) OHFUTI Yasushi  Osaka University, Faculty of Engineering Science, Research assistant, 基礎工学部, 助手 (10201980)
Project Period (FY) 1992 – 1994
Project Status Completed (Fiscal Year 1994)
Budget Amount *help
¥2,000,000 (Direct Cost: ¥2,000,000)
Fiscal Year 1994: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1993: ¥600,000 (Direct Cost: ¥600,000)
Fiscal Year 1992: ¥900,000 (Direct Cost: ¥900,000)
KeywordsNonlocal response / Radiative correction / Size dependence / photon STM / Optical Stark effect / Wave number conservation rule / Mossbauer resonant diffraction / SHG / 非局所応答理論 / 共鳴光学応答 / 半導体薄膜 / 半導体微粒子 / ポンプ・プローブ分光 / サイズ変化 / 近接電磁場 / メスバウアー共鳴回折 / 超微粒子 / 微粒子集合系 / 放射寿命 / 長波長近似 / 内部電場
Research Abstract

Applying the nonlocal response theory developed by us, we have studied the following problems with the results described respectively. [1] Optical response of the assemblies of semiconductor microspheres : Resonant response spectrum was studied as a function of particle number, the way of their arrangements, size, and geometrical configuration. Radiative correction is explicitly included. The same analytical expression of radiative width as in QED is obtained for a single sphere and 1D and 2D infinite lattices. [2] Study of photon STM : By extending the results of [1], we have calculated the near field intensity map of a resonantly irradiated sample and the signal intensity in transmission and reflection geometries. The effect of configurational resonance is predicted, and the breakdown of electric dipole selection rule in reflection mode has been demonstrated. [3] Optical Stark effect of excitons and biexcitons in a slab : A consistent description of nonlinear spectra has been given for the size dependence in the region of 100 A-10000 A thickness. The development of wave number section rule is clearly shown. The calculated spectra show optical Stark shift, resonant broadening and two photon absorption simultaneously. [4] Formulation of Mossbauer diffraction : A nonlocal formulation has been given for a stack of 2D atomic layrs, and the condition of the enhancement of radiative width is studied. [5] SHG from the 2D electronic bands at insulator/semiconductor interface : A nonlocal formulation of resonant SHG due to atomically thin 2D layr has been given without employing the doubtful argument of boundary conditions. The use of 2D periodicity and the long wavelength approximation for the direction of thickness leads to a simple equation to be solved.

Report

(4 results)
  • 1994 Annual Research Report   Final Research Report Summary
  • 1993 Annual Research Report
  • 1992 Annual Research Report
  • Research Products

    (34 results)

All Other

All Publications (34 results)

  • [Publications] Y.Ohfuti: "Nonlocal formulation of optical response of an assembly of fine particles" Proc.Int.Symp.on Science and Technology of Mesoscopic Structures(Springer Verlag). 457-463 (1992)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Ohfuti: "Spontaneous emission rate of 0 to 3D systmes by nonlocal formulation" Jpn.J.Appl.Phys.Series 9. 197-200 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Resonant size enhancement of induced polarization with particular spatial distribution in optical response of mesoscopic systems" Solid State Commun.87. 1105-1108 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Nonlocal aspects of optical responses of mesoscopic Systems" Proc.Int.Conf.on Dynamical Processes in the Excited States of Solids(invited),J.Luminescence. 58. 95-99 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Nonlocal response of size quantized excitons in a semiconductor microsphere" Proc.Int.Conf.on Luminescence,J.Luminescence. 60/61. 330-332 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] H.Ishihara: "Nonlocal theory of the third order nonlinear optical response of confined excitons" Phys.Rev.B. 48. 7960-7974 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Z.K.Tang: "Optical selection rule and oscillator strength of confined exciton system in CuC1 thin films" Phys.Rev.Letters. 71. 1431-1434 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] H.Ishihara: "A new type of nonlinear optical response in a thin film owing to 'nonlocality induced double resonance in energy and size' of internal field" Solid State Commun.89. 837-841 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] N.Matsuura: "Nonlocal theory of the optical Stark effect on the size quantized excitons in a slab" J.Phys.Soc.Jpn.64. 651-662 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Effect of selective pumping of polaritons on the optical spectra of a thin layer of CuC1:Result of nonlocal response theory" Proc.Int.Conf.on Excitonic Processes in Condensed Matter (invited) SPIE Proc.Series 2362. 151-161 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Study of scanning near-field optical microscopy (SNOM)by nonlocal response theory" Proc.Int.Conf.on Optical Properties of Nanostructures (invited),Jpn.J.Appl.Phys.Suppl.34. 267-270 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Ohfuti: ""Nonlocal formulation of optical response of an assembly of fine particles"" Proc.Int.Symp.on Science and Technology of mesoscopic structures (Springer Verlag). 457-463 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Ohfuti: ""Spontaneous emission rate of 0 to 3D systems by nonlocal formulation"" Jpn.J.Appl.Phys.Series. 9. 197-200 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: ""Resonant size enhancement of induced polarization with particular spatial distribution in optical response of mesoscopic systems"" Solid State Commun.87. 1105-1108 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: ""Nonlocal aspects of optical responses of mesoscopic systems"" Proc.Int.Conf.on dynamical Processes in the Excited States of Solids (invited), J.Luminescence. 58. 95-99 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: ""Nonlocal response of size quantized excitons in a semiconductor microsphere"" Proc.Int.Conf.on Luminescence, J.Luminescence. 60/61. 330-332 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] H.Ishihara: ""Nonlocal theory of the third order nonlinear optical response of confined excitons"" Phys.Rev.B48. 7960-7974 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Z.K.Tang: ""Optical selection rule and oscillator strength of confined exciton system in CuCl thin films"" Phys.Rev.Letters. 71. 1431-1434 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] H.Ishihara: ""A new type of nonlinear optical response in a thin film owing to 'nonlocality induced double resonance in energy and size' of internal field"" Solid State Commun.89. 837-841 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] N.Matsuura: ""Nonlocal theory of the optical Stark effect on the size quantized excitons in a slab"" J.Phys.Soc.Jpn.64. 651-662 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: ""Effect of selective pumping of polaritons on the optical spectra of a thin layr of CuCl : Result of nonlocal respons theory"" Proc.Int.Conf.on Excitonic Processes in Condensed Matter (invited) SPIE Proc.Series. 2362. 151-161 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: ""Study of scanning near-field optical microscopy (SNOM) by nonlocal response theory"" Proc.Int.Conf.on Optical Properties of Nanostructures (invited), Jpn.J.Appl.Phys.Suppl.34-1. 267-270 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] K.Cho: "Effect of selective pumping of polaritons on the optical spectra of CuCl:Result of nonlocal response theory" Proc.Int.Conf.on Excitonic Processes in Condensed Matter,Darwin,1994(The International Society of Optical Engineering). (in print). (1995)

    • Related Report
      1994 Annual Research Report
  • [Publications] N.Matsuura: "Nonlocal theory of the optical Stark effect on the size quantized excitons in a slab" J.Phys.Soc.Jpn.64(in print). (1995)

    • Related Report
      1994 Annual Research Report
  • [Publications] K.Cho: "Study of scanning near-field optical microscopy (SNOM) by nonlocal response theory" Proc.Int.Conf.on Optical Properties of Nanostructures,Sendai,1994,(Jpn.J.Appl.Phys.Suppl.). (in print). (1995)

    • Related Report
      1994 Annual Research Report
  • [Publications] Y.Ohfuti: "Spontaneous Emission Rate of 0 to 3D Systems by Nonlocal Formulation" J.Appl.Phys.Series. 9. 197-200 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] K.Cho: "Resonant Size Enhancement of Induced Polarization with Particular Spatial Distribution in Optical Response of Mesoscopic Systems" Solod State Commun.87. 1105-1108 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] K.Cho: "Nonlocal Aspects of the Optical Responses of Mesoscopic Systems" J.Luminesc.623(in print). (1994)

    • Related Report
      1993 Annual Research Report
  • [Publications] K.Cho: "Nonlocal Response of Size-quantized Excitons in a Semiconductor Microsphere" J.Luminesc.(in print). (1994)

    • Related Report
      1993 Annual Research Report
  • [Publications] Z.K.Tang: "Optical Selection Rule and Oscillator Strength of Confined Exciton System in CuCl Thin Films" Phys.Rev.Letters. 71. 1431-1434 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] Y.Ohfuti: "Spontaneous Emission Rate of 0 to 3D Systems Nonlocl Formulation" Japan.J.Appl.Phys.Series 9. 5- (1993)

    • Related Report
      1992 Annual Research Report
  • [Publications] H.Ishihara: "Resonant Enhancement of Internal Field as a Function of Mesoscopic System Size:An Unoticed Source of Large Optical Nonlinearity in Nonlocal Response" Proc.Int.Conf.on Science and Technology of Mesoscopic Structures,ed.by S.Namba,C.Hamaguchi,and T.Ando(Springer Verlag,1992). 464-469 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] Y.Ohfti: "Nonlocal Formulation of Optical Response of an Assembly of Fine Particles" Proc.Int.Conf.on Science and Technology of Mesoscopic Structures,ed.by S.Namba,C.Hamaguchi,and T.Ando(SpringerVerlag,1992). 457-463 (1992)

    • Related Report
      1992 Annual Research Report
  • [Publications] 張紀 久夫: "線形・非線形の共鳴光学応答における非局所性" 数理科学(サイエンス社). 10. 22-27 (1992)

    • Related Report
      1992 Annual Research Report

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Published: 1992-04-01   Modified: 2016-04-21  

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