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Measurements of delta^<13>C of atmospheric CO_2 and its application to the carbon cycle

Research Project

Project/Area Number 05452076
Research Category

Grant-in-Aid for General Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field Meteorology/Physical oceanography/Hydrology
Research InstitutionTohoku University

Principal Investigator

NAKAZAWA Takakiyo  Tohoku University, Faculty of Science, Professor, 理学部, 教授 (30108451)

Co-Investigator(Kenkyū-buntansha) AOKI Shuji  National Institute of Polar Research, Assistatant Professor, 助手 (00183129)
KAWAMURA Hiroshi  Tohoku University, Faculty of Science, Professor, 理学部, 教授 (40169769)
Project Period (FY) 1993 – 1994
Project Status Completed (Fiscal Year 1994)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,900,000)
Fiscal Year 1994: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 1993: ¥2,400,000 (Direct Cost: ¥2,400,000)
KeywordsCarbon dioxide / Carbon isotopic ratio / Global carbon cycle / 同位体比
Research Abstract

The concentration of atmospheric CO_2 has been increasing steadily for the last 200 years, due to human activities such as fossil fuel combustion and deforestation. In order to elucidate the causes of such an increase of the concentration quantitatively, it is necessary to figure out the carbon cycle on the earth's surface. However, the roles of the biosphere and the oceans in the carbon cycle are not yet well understoond. To solve this difficulty, measurements are requireed for the carbon isotopic ratio delta^<13>C of atmospheric CO_2 as well as for its concentration.
In this study, CO_2 samples collected in the troposphere over Japan and in the western Pacific and the Antarctic regions were analyzed for delta^<13>C with a precision of better than 0.02*. The seasonal cycle of delta^<13>C was clearly found at northern latitudes and the equator, due to the seasonal change in the biospheric activities, but it was hardly observable in the southern hemisphere. It was found that values of delta^<13>C decreased seculary at a rate of about 0.03*, due mainly to fossil fuel combustion. Interannual variations in the long-term trend of delta^<13>C were also found in association with ENSO event and other factors, which were almost opposite in phase with those of the CO_2 concentration. The analyzes of delta^<13>C and the CO_2 concentration with a box diffusion model and a 2-D atmospheric transport model showed that an imbalance of the CO_2 exchange between the atmosphere and the biosphere could be responsible for such interannual variations and that the biosphere does not act as a strong net source for atmospheric CO_2.

Report

(3 results)
  • 1994 Annual Research Report   Final Research Report Summary
  • 1993 Annual Research Report
  • Research Products

    (13 results)

All Other

All Publications (13 results)

  • [Publications] T.Nakagawa: "Time and space variations of the carbon isotopic ratio of tropospherio carbon dioxide over Japan" Tellus. 45B. 258-274 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakagawa: "Temporal and spatial variations of carbon isotopic ratio of atmospheric CO_2 in the western Pacific region" J.Geophys.Res.99(印刷中). (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Gamo: "Long-term monitoring of carbon and oxygen isfope ratios of stratospheric CO_2 over Japan" Geophys.Res.Lett、. 21(印刷中). (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakamura: "Seasonat variations in ^<14>C concertrations of Stratospheric CO_2 measured with accelerator mass spectrewelor" Nucl.Inst.Meth.Phys.Res. 392. 413-416 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakazawa: "Time and space variations of the carbon isotopic ratio of the tropospheric carbon dioxide over Japan" Tellus. 45B. 258-274 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakazawa: "Temporal and spatial variations of carbon isotopic ratio of atmospheric carbon dioxide in the western Pacific region" J.Geophys.Res.99 (in press). (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Gamo: "Long-term monitoring of carbon and oxygen isotope ratios of stratospheric carbon dioxide over Japan" Geophys.Res.Lett.21(in press). (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakamura: "Seasonal variations in ^<14>C concentrations of stratospheric carbon dioxide measured with accelerator mass spectrometer" Nucl.Inst.Meth.Phys Res.B92. 413-416 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Nakazawa: "Time and space variations of the carbou isotopic ratio of tropospheric Carbon dioxide over Japan" Tellus. 45B. 258-274 (1993)

    • Related Report
      1994 Annual Research Report
  • [Publications] T.Nakazawa: "Temporal and spatial variationsof carbon isotopic ratio of atmospheric CO_2 in the western Pacific regron" J.Geophys.Res.99(印刷中). (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] T.Gamo: "Long-term monitoring of carbon and oxygen istope ratios of stratospheric CO_2 over Japan" Geophys.Res.Lett.21(印刷中). (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] T.Nakamura: "Seasonal variations in ^<14>C concentrations of stratospheric CO_2 measured with a ccelerafor mass spectrometer" Nucl.Inst.Mcth.phys.Res.B92. 413-416 (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] T.Nakazawa: "Time and space variations of the carbon isotopic ratio of tropospheric carbon dioxide over Japan" Tellus. 45B. 258-274 (1993)

    • Related Report
      1993 Annual Research Report

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Published: 1993-04-01   Modified: 2016-04-21  

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