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Generation of radicals by laser-ablation and their application to beam source

Research Project

Project/Area Number 05555009
Research Category

Grant-in-Aid for Developmental Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 表面界面物性
Research InstitutionKYUSHU UNIVERSITY

Principal Investigator

OKADA Tatsuo  Kyushu University, Associate Professor, 工学部, 助教授 (90127994)

Co-Investigator(Kenkyū-buntansha) MAEDA Mitsuo  Kyushu University, Professor, 工学部, 教授 (80037910)
Project Period (FY) 1993 – 1994
Project Status Completed (Fiscal Year 1994)
Budget Amount *help
¥4,000,000 (Direct Cost: ¥4,000,000)
Fiscal Year 1994: ¥1,000,000 (Direct Cost: ¥1,000,000)
Fiscal Year 1993: ¥3,000,000 (Direct Cost: ¥3,000,000)
KeywordsRadical / Particle beam / Ablation / LIF / Imaging / Ceramics / Particulate / レーザーアブレーション / レーザー誘起蛍光法 / セラミック / ポリマー
Research Abstract

A variety of radicals was generated directly from solid targets by laser abation. Characteristics of the radicals were investigated by laser-induced fouorescence spectroscopy, in order to access the applicability for the radical sources. The results are summarized as follows.
(1) Ba, Y,YO and BaO radicals were generated from a laser-ablated YBa_2Cu_3O_<7-x> target.
(2) It was found that the kinetic energy of YO molecules reached upto 10eV.On the other hand, the rotational energy distribution was measured to be arount 0.2eV.It is shown that the most of the energy of the ejected molecules was transported as a kinetic energy.
(3) Atomic species were mainly ejected from laser-ablated Al_2O_3, Si_3N_4 and BaTiO_3 targets
(4) It was found that velocity distribution of ejected atoms were well described by a two-components shifted Maxwellian distribution.
(5) Al atomic beam was generated by slitting the Al plume produced by the ablation and temporal developments of its density distribution were visualized by imaging laser-induced fluorescence spectroscopy. It was clearly demonstrated that high-density and high-energy neutral beam can be easily produced by the present technique.
(6) The effect of the cumulative ablation of the targets on the ejection of radicals were investigated. It was found that more particulates and less radicals were ejected, as the target was ablated cumulative by. An empirical fomula which described the degradation of the target was proposed.

Report

(3 results)
  • 1994 Annual Research Report   Final Research Report Summary
  • 1993 Annual Research Report
  • Research Products

    (19 results)

All Other

All Publications (19 results)

  • [Publications] T. Okada他: "Piezoelectric Sensing of Particles Produced by Pulsed-Laser Ablation of YBa_2Cu_3O_<7-σ>" Jpn. J. Appl. Phys.32. 1535-1537 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] 岡田龍雄他: "Laser-spectroscopic investigation of behavior of particles ejected by laser ablation" 応用物理. 32. 1221-1224 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W. K. A. Kumuduni他: "Transport of YO molecules produced by ArF Laser ablation of YBa_2Cu_3O_<7-σ> in ambient oxygen gas" J. Appl. Phys.74. 7510-7516 (1993)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y. Nakata他: "Plume-substrates interaction in pulsed-laser deposition of high-temperature superconducting thin films" Appl. Phys. Lett.64. 2599-2601 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W. K. A. Kumuduni他: "Spatial Distribution of YO Molecules Ejected from Laser-Ablated YBa_2Cu_3O_<7-x>" Appl. Phys. B. 58. 289-294 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y. Nakata他: "Radical Beams Produced by Laser Ablation and Their Application" Jpn. J. Appl. Phys.33. 4316-4319 (1994)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W. K. A. Kumuduni他: "Effect of cumulative ablation on the ejection of particular and molecular species from YBa_2Cu_3O_<7-x> Target" Jpn.J.Appl.Phys.(to be published.). (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Okada et al.: ""Piezoelectric Sensing of Particles Produced by Pulsed-Laser Ablation of YBa_2Cu_3O_<7-sigma>"" Jpn.J.Appl.Phys. Vol.32-No.10B. 1535-1537 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] T.Okada et al.: ""Laser-spectroscopic investigation of behavior of particles ejected by laser ablation"" Oyo Buturi. Vol.62-No.12. 1221-1224 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W.K.A.Kumuduni et al.: ""Transport of YO molecules produced by ArF laser ablation of YBa_2Cu_3O_<7-sigma> In ambient oxygen gas"" J.Appl.Phys.Vol.74-No.12. 7510-7516 (1993)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Nakata et al.: ""Plume-substrates interaction in pulsed-laser deposition of high-temperature superconducting thin films"" Appl.Phys.Lett.Vol.64-No.19. 2599-2601 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W.K.A.Kumuduni et al.: ""Spatial Distribution of YO Molecules Ejected from Laser-Ablated YBa_2Cu_3O_<7-x>"" Appl.Phys.B. Vol.58. 289-294 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Nakata et al.: ""Radical Beams Produced by Laser Ablation and Their Application"" Jpn.J.Appl.Phys. Vol.33-No.7B. 4316-4319 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] W.K.A.Kumuduni et al.: ""Effect of cumulative ablation on the ejection of particular and molecular species from YBa_2Cu_3O_<7-x> target"" Jpn.J.Appl.Phys. (to be published). (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1994 Final Research Report Summary
  • [Publications] Y.Nakata他: "Plume-substrate interacition in pulsed-laser deposition of high-temperature super conducting thin film" Applied Physics Letters. 64. 2599-2601 (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] W.K.A.Kunuduni他: "Spatial distribution of YO molecules ejected from laser-ablated YBa_2Cu_3O_<7-x>" Applied Physics B. 58. 289-294 (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] Y.Nakata他: "Radical beams produced by laser ablation and thin dpplication" Japanes Journal of Applied Physics. 33. 4316-4319 (1994)

    • Related Report
      1994 Annual Research Report
  • [Publications] T.Odaka 他: "Radical Beams Produced by Laser Ablation and Their Application to Radical-Surface Interaction" Proc.2nd Inter. Reactive Plasmas. 431-434 (1993)

    • Related Report
      1993 Annual Research Report
  • [Publications] Y.Nakata: "Radical beaem produced by laser ablation and their application" Jpn. J. Appl. Phys.(印刷中).

    • Related Report
      1993 Annual Research Report

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Published: 1993-04-01   Modified: 2016-04-21  

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