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"Neutron Scattering Study on Photosensitive Magnetic Clusters in Semimagnetic Semiconductors"

Research Project

Project/Area Number 07455417
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionTOHOKU UNIVERSITY

Principal Investigator

KAJITANI Tsuyoshi  TOHOKU UNIVERSITY,School of Engineering, Professor, 大学院・工学研究科, 教授 (80134039)

Co-Investigator(Kenkyū-buntansha) MIYAZAKI Yuzuru  TOHOKU UNIVERSITY,School of Engineering, Research Associate, 大学院・工学研究科, 助手 (40261606)
ONO Yasuhiro  TOHOKU UNIVERSITY,School of Engineering, Research Associate, 大学院・工学研究科, 助手 (30211832)
SHAMOTO Shin-ichi  TOHOKU UNIVERSITY,School of Engineering, Associate Professor, 大学院・工学研究科, 助教授 (90235698)
ITO Tadashi  TOHOKU UNIVERSITY,School of Engineering, Professor, 大学院・工学研究科, 教授 (60004503)
Project Period (FY) 1995 – 1997
Project Status Completed (Fiscal Year 1997)
Budget Amount *help
¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 1997: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1996: ¥1,100,000 (Direct Cost: ¥1,100,000)
KeywordsSEMIMAGNETIC SEMICONDUCTOR / II-VI-TYPE COMPOUND / MAGNETIC CLUSTER / SPIN GLASS / NEUTRON DIFFRACTION / COLD NEUTRON SCATTERING / PPC / 磁気クラスター / 中性子散乱 / 磁気準弾性散乱 / 反強磁性 / 常磁性 / 磁的化測定 / 単結晶
Research Abstract

Present study was aimed to obtain structural characteristics of optically sennsitive magnetic clusters and its related physical properties of magnetic clusters in the II-VI-type semiconductors deped with magnetic metal atoms. Single crystals of Zn_<1-x>Mn_xTe with x=0.3-0.6 were prepared by the standard Bridgeman method. Structural study on the average lattice was done by means of powder x-ray diffraction measurement in the temperature range from 20K to the ambient. Magnetic susceptibility measurements were performed by means of SQUID manetometer in the range from the ambient to 4.2K.The spin glass temperatures, Tg, were determined accordingly. In the course of the present study, diffuse intensities due to the short range magnetic ordering was found by the powder neutron diffraction measurement below 100K.The magnetic structure-type of the magnetic clusters, which is responsible for the diffuse scatterings, has been determined by means of single crystal neutron diffraction study. The s … More ingle crystal neutron diffraction measurement was performed in the magnetic field up to 5-Tesla by the use of high resolution neutron diffractometers, HRPD and HERMES installed in the JRR3M reactor hall and the thermal guide hall, respectively. Two dimensional neutron diffraction intensity measurement was performed in the 001 reciprocal plane simultaneously by many neutron counters set in the instruments. Brillouin scattering measurement was tried to study the spin dynamics in the low temperature range. Brillouin scattering measurement, i.e., an optical inelastic scattering measurement, is suitable to measure the excitation levels in the range below 0.5meV with the resolution of 0.01meV.A new Ar-gas laser was purchased with the aid of present financial support and a 5-pass high resolution Fabry-Perot interferrometer was made from an old 3-pass interferrometer, and then a 5-pass Brillouin scattering system was assembled. Brillouin scattering measurement at low temperatures in the magnetic field up to 4000 Oe was successfully performed for the complicated ferromagnetic metallic compound. A part of the magnon dispersion relationship consistent with the neutron scattering data was determined by this instrument. Neutron inelastic scattering measurement has been performed for Zn_<0.6>Mn_<0.4>Te sample using the cold neutron spectrometer AGNES.Critical scattering, associated with the spin glass transition has been observed for the first time in this semimagnetic semiconductor. The critical scattering was observed at temperatures in the vicinity of the spin glass transition temperature, 17K.Photo conductivity has been found also for the first time below 150K in Zn_<0.6>Mn_<0.4>Te sample. The electric AC conductivity has been increased dramaticaly under the laser light with the wave lengths of lambda=6328,5145 and 4880A,respectively. The conductivity was reduced to the original level after the light was darkened, but it took very long, i.e.2000 second at 50K,being above the Less

Report

(4 results)
  • 1997 Annual Research Report   Final Research Report Summary
  • 1996 Annual Research Report
  • 1995 Annual Research Report
  • Research Products

    (20 results)

All Other

All Publications (20 results)

  • [Publications] 小野 康弘: "X-ray Diffraction Study of LaBiO5" Journel of the Phisical Society of Japan. 65. 3224-3227 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] B.P.Zang: "Naturally formed ZuCdSe Quantum dots on ZuSe(110)Surfaces" Applied Physics Letters. 70. 2413-2415 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] B.P.Zang: "Spontaueous formation and Photolumiuesceuce of ZuSe dot arrays" Applied Physics Letters. 71. 3370-3372 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 梶谷 剛: "Cold neutron scattering study on quasi-1D metal cowplexes" Actiuiry Report ou Neutron Scattering Resecuch ISSP Univ-Tokyo. 2. 76-77 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 高山 一也: "Inelastic Neutron Scattering Study of the Holdanegap System Ni(C5H_<14>N_2)_2N_3CLO_3" Activity Report on Neutron Scattering Research ISSP Univ.Tokyo. 3. 113- (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 小野 康弘: "Single Craystal Neutron Diffraction Study of Dilutod M&guetic Semicouductor Z<nM>___<1-x>M<nT>___xe with x=0.432" Activity Report on Neutron Scattering Research ISSP Univ.Tokyo. 4. 68- (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 小野 康弘: "Cokd Neutron Scattering Study of Diluted Maguetic Seniconduetor Z<nM>___<1-x>M<nT>___xe with x=0.432" Activity Report on Neutron Scattering Research ISSP Univ.Tokyo. 4. 69- (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 梶谷 剛: "Cold Neutron Scattering Study on BEDT-TTF Salts" Activity Report on Neutron Scattering Research ISSP Univ.Tokyo. 4. 79- (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 小野 康弘: "X-raydiffraction Study of Sm_2(F<eA>___<1-x>l)17 Single crystals with x=0.058,0.081" Journal of Maguetism and Magunetic Materials. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Y.Ono, K.Takayama and T.Kajitani: ""X-ray Diffraction Study of LaBSiO_5"" Jornal of the Physical Society of Japan. 65. 3224-3227 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] B.P.Zang, T.Yasuda, Y.Segawa, H.Yaguchi, K.Onabe, E.Edamatsu and T.Itoh: ""Naturally formed ZnCdSe quantum dots on ZnSe (110) surfaces"" Applied Physics Letters. 70. 2413-2415 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] B.P.Zang, T.Yasuda, Y.Segawa, K.Edamatsu and T.Itoh: ""Spontaneous formation and photoluminescence of ZnSe dot arrays"" Applied Physics Letters. 71. 3370-3372 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] T.Kajitani, Y.Tsubakino, H.Okamoto, N.Kuroda and H.Yamashita: ""Cold neutron scattering study on quasi-1D metal complexes"" Activity Report on Neutron Scattering Research, ISSP Univ.Tokyo. Vol.2. 76-77 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Takayama, M.Yamashita and T.Kajitani: ""Inelastic Neutron Scattering Study of the Haldane-gap System Ni (C_5H_<14>N_2) _2N_3ClO_3"" Activity Report on Neutron Scattering Research, ISSP Univ.Tokyo. Vol 3. 113 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Y.Ono, K.Sato, S.Shamoto, T.Sato, Y.Oka and T.Kajitani: ""Single Crystal Neutron Diffraction Study of Diluted Magnetic Semiconductor Zn_<1-x>Mn_xTe with x=0.432"" Activity Report on Neutron Scattering Research, ISSP Univ.Tokyo. Vol 4. 68 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Y.Ono, K.Sato, S.Shamoto, T.Sato, Y.Oka and T.Kajitani: ""Cold Neutron Scattering Study of Diluted Magnetic Semiconductor Zn_<1-x>Mn_xTe with x=0.432"" Activity Report on Neutron Scattering Research, ISSP Univ.Tokyo. Vol 4. 69 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] T.Kajitani, Y.Ono, Y.Miyazaki, T.Sasaki and N.Toyota: ""Cold Neutron Scattering Study on BEDT-TTF Salts"" Activity Report on Neutron Scattering Reseach , ISSP Univ.Tokyo. Vol4. 79 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Y.Ono, J.Shimoji, H.Kato, T.Iriyama and T.Kajitani: ""X-ray diffraction study of Sm_2(Fe_<1-x>Al)_<17>single crystals with x=0.058,0.081"" Jounal of Magnetism and Magnetic Materials. (accepted on). (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] B.P.Zang et al.: "Self-assembled ZnCdSe quantum dots on ZnSe(110) surface" Applied Physics Letters. 71. 3370-3372 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] B. P. Zhang: "Self-assembled ZnCdSe quantum dots on ZnSe (110) siuface" Applied Physics Letters,. (印刷中). (1997)

    • Related Report
      1996 Annual Research Report

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Published: 1996-04-01   Modified: 2016-04-21  

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