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Development and Application of the Polymerization System with Fuzzy Temperature Control for Highly Viscous and Eexothermal Polymerization

Research Project

Project/Area Number 07555550
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section試験
Research Field 反応・分離工学
Research InstitutionYokohama National University

Principal Investigator

KAMIWANO Mitsuo  Yokohama Nat.Unv., Faculty of Engineering, Professor, 工学部, 教授 (70017896)

Co-Investigator(Kenkyū-buntansha) TARUMOTO Jun  Soken Chem.& Eng.Co.Ltd., Research Center, Investigator, 研究開発センター, 副主任研究員
YAMAMOTO Kazumi  Soken Chem.& Eng.Co.Ltd., Research Center, Head Investigator, 研究開発センター, 主任研究員
NISHI Kazuhiko  Yokohama Nat.Unv., Faculty of Engineering, Assistant, 工学部, 助手 (20262412)
KAMINOYAMA Meguru  Yokohama Nat.Unv., Faculty of Engineering, Assistant Professor, 工学部, 助教授 (50233945)
Project Period (FY) 1995 – 1996
Project Status Completed (Fiscal Year 1996)
Budget Amount *help
¥5,600,000 (Direct Cost: ¥5,600,000)
Fiscal Year 1996: ¥5,600,000 (Direct Cost: ¥5,600,000)
Keywordspolymerization system / fuzzy control / model prediction control / viscous fluids / high exothermal polymerization / Stirred tank reactor / numerical simulation / 撹拌槽型重合反応器 / 温度むら / 重合物物性 / リアルタイム多点温度計測装置 / 重合シミュユレーション / ラジカル付加重合 / 熱伝達係数 / 重合反応槽 / 温度分布 / 分子量分布 / レオロジー / 攪拌槽
Research Abstract

In this study, We developed a batch polymerization reactor which have five cooling coils in the vertical direction. There are sixteen thermocouples to measure temperature distribution in the reactor. The temperature value from each thermocouples are sent microcomputer. The microcomputer calculated operation values for each cooling coils based on a suitable control theory, which is 'fuzzy' or 'model prediction' etc..
We investigated the relationship temperature distribution in the polymerization reactor and the properties of produced polymers at first.
As a result, We found that on-off control reactor and PID control reactor could not temperature control when reaction fluid was high viscosity. But the fuzzy control reactor and the model prediction reacter had control capacity through the reaction time. And produced polymers from the fuzzy control reactor and the model prediction reactor had a narrower molecular weight distributions then the other control reactor. In the case of compared the fuzzy control reactor with the model prediction control, the latter one was better. Because model prediction control was not necessary adjustment of fuzzy constants which is indispensable operation in fuzzy control.
In this study, we developed the numerical simulator for batch polymerization reactor with several control system. This simulator was calculated three dimensional velocity, temperature distribution, monomer conversion distribution in reactor and molecular weight distribution of produced polymer at any time.

Report

(3 results)
  • 1996 Annual Research Report   Final Research Report Summary
  • 1995 Annual Research Report
  • Research Products

    (18 results)

All Other

All Publications (18 results)

  • [Publications] 上和野 満雄 他: "リアルタイム多点温度計測器の試作-高粘度撹拌槽における伝熱状態の測定-" 化学工学論文集. 21. 760-765 (1995)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 山本 一巳 他: "各種翼付重合反応槽における温度むらと重合物物性" 化学工学論文集. 22. 882-890 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 山本 一巳 他: "重合槽内における反応進行に伴う冷却コイルの境膜熱伝達係数の経時変化" 化学工学論文集. 22. 1250-1254 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 上ノ山 周 他: "二重らせん帯翼付撹拌槽におけるスチレン塊状重合反応過程の数値解析" 化学工学論文集. 23. 835-843 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 上和野 満男: "撹拌、混合におけるトラブル発生要因と防止対策" 上和野 満男監修、(株)技術情報協会, 265 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] Mitsuo Kamiwano et.al.: "Trial Manufacture of a Real-Time and Multi-Point Temperature Measuring Instrument-Application for Measyring the Heat Transfer Condition of High Viscous Fluids in a Stirred Vessel-" J.Chem.Eng.Japan. 21. 760-765 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] Kazumi Yamamoto et.al.: "Relation of Polymer Properties and Local Temperature Distribution in a Stirred-Type Batch Reactor using Several Types of Impellers" J.Chem.Eng.Japan. 22. 882-890 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] Kazumi Yamamoto et.al.: "Measurement of Cooling Coil Film Heat Transfer Coefficient with Polymer Reaction Proceeding in a Stirred Batch Reactor" J.Chem.Eng.Japan. 22. 1250-1254 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] Meguru Kaminoyama et.al.: "Numerical Analysis of Bulk Thermal Stirene Polymerization in Stirred Vesssl with Helical Ribbon Impeller" J.Chem.Eng.Japan. 23. 835-843 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] Mitsuo Kamiwano: "The Cause of Troubles and Prevention in Agitating and Mixing Process" Kagaku Joho kyoukai. 265 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 上和野満雄ら: "各種凡用翼付重合反応槽内における温度むらと重合物物性" 化学工学論文集. 22. 882-890 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 上和野満雄ら: "重合槽内における反応進行にともなう冷却コイルの境膜熱伝達係数の経時変化" 化学工学論文集. 22. 1250-1254 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 上和野満雄ら: "数値解析による撹拌槽内における槽壁側局所熱伝達係数の算出法"" 化学工学シンポジウムシリーズ. 51. 109-114 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 上和野満雄ら: "二重らせん帯翼付き撹拌槽型反応器におけるスチレン塊状重合反応の数値解析法" 化学工学シンポジウムシリーズ. 51. 115-120 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 上和野満雄: "リアルタイム多点温度計測器の試作-高粘度攪拌槽における伝熱状態の測定-" 化学工業論文集. 21. 760-765 (1995)

    • Related Report
      1995 Annual Research Report
  • [Publications] 上和野満雄: "Relation of Polymer Properties and Local Temperature Distribution in a Stirred-Type Batch Reactor Using Several Types of Impeller" Proc. of 7th Congress of Asian Pacific Confederation of Chemical Engneering. 2. 704-708 (1996)

    • Related Report
      1995 Annual Research Report
  • [Publications] 上ノ山周: "変貌するミキシング技術-数値シミュレーションの問題点-" 化学工学. 59. 626-629 (1995)

    • Related Report
      1995 Annual Research Report
  • [Publications] 上和野満雄: "攪拌槽のスケールアップ" 化学工学. 60. 162-165 (1996)

    • Related Report
      1995 Annual Research Report

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Published: 1996-04-01   Modified: 2016-04-21  

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