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Crystal Growth and Characterization of Bi_4Si_3O_<12> Systems for Radiation Detectors

Research Project

Project/Area Number 07650791
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionShonan Institute of Technology

Principal Investigator

ISHII Mitsuru  Shonan Institute of Technology, Faculty of Engineering, Professor, 工学部, 教授 (80212827)

Co-Investigator(Kenkyū-buntansha) KOBAYASHI Masaaki  National Laboratory for High Energy Physics, Associate Professor, 物理系, 助教授 (40013388)
Project Period (FY) 1995 – 1996
Project Status Completed (Fiscal Year 1996)
Budget Amount *help
¥1,700,000 (Direct Cost: ¥1,700,000)
Fiscal Year 1996: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1995: ¥900,000 (Direct Cost: ¥900,000)
KeywordsBismuth Sillcate / Crystal growth / Brigman Technique / Transmittance / Scintillation / radiation hardness / セリウム添加ビスマスシリケート
Research Abstract

The aim of this study is to development of new scintillation crystal of BSO (Bi_4Si_3O_<12>) for radiation etectors in high energy physics experiments by Bridgman method.
1) Growth and Characterization of pure BSO.Single crystal of BSO were grown to small crystals (25mm in dia by 70mm length) of various growth conditions, using such high purity raw materials of Bi_2O_3 and SiO_2 for searching of the growth technique for large BSO crystals. Applying the results of these experiments, we manufctured 3 pos of ingots each with 35mm in dia and 20cm in length for trial purpose of detector of high energy particles. Yield of segregation phase was observation on the surface of grown crystals but the inside was clear without any defects. From these ingots, we manufactured Scintillator 190mm in length and evaluated can be used as scintillator practically. Evaluation was made with transmission, scintillation performance as well as radiation hardness by ^<60>Co.
2) Growth and characterization of Ce doped BSO.The segregation coefficients of Ce to BSO is nearly 1.Up to addition of 0.2% Ce, single crystal could be grown same to pure BSO.As for the performance of scintillator of BSO by Ce doping the light output was decreased and no improvement was made on the decay time of florescence but it was found that radiation hardness was improved markedly.
3) Growth and characterization of Pr doped BSO.As for doping of Pr to BSO,the absorption wave length was at 470nm and it was confirmed closed to the emission wave length of this crystals. Therefore, these is a small possibility that Pr doped BSO will become a high performance scintillator.
Based on the above mentioned studies, we confimed that the high purity BSO crystal not including any dopants or including Ce up to 0.2% is best suited for scintillation materials for the radiation detector of high energy particles. The trial manufacture of scintillation crystals of practical scale in underway as an appliation of it

Report

(3 results)
  • 1996 Annual Research Report   Final Research Report Summary
  • 1995 Annual Research Report
  • Research Products

    (24 results)

All Other

All Publications (24 results)

  • [Publications] M.Kobayashi et al,: "Bismuth Silicate Bi_4Si_3O_<12>,A Faster Scimtillator than Bismuth Geromanate Bi_4Ge_3O_<12>" Nucl.Instr.and Meth.A372. 45-50 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Mechamical Properties of PbWO_4 Scintillating Crystals." Nucl.Instr.and Meth.A376. 203-207 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Scintillation and Phashoresonce of PbWO_4 Crystuls." Nucl.Instr.and Meth.A373. 333-346 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Niki et al.: "Radiation Induced Formation of Color Centers in PbWO_4 Single Crystals." J.Appl.Physics.(in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Improvement in Transonittance and Decay Time or PbWO_4 Scintillating Crystul by La doping" Nucl.Instr.and Meth.(in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] 石井満、小林正明: "結晶成長ハンドブック 2.7 シンチレーション結晶" 共立出版(株), 8 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Bismuth Silicate Bi_4Si_3O_<12> A Faster Scintillator than Bismuth Gemanate Bi_4Ge_3O_<12>" Nucl.Instr.Meth.in Physis Res.A372. 45-50 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Improvement in Transmittance and Decay Time of PbWO_4 Scintillating Crystals by La-doping" Nucl.Instr.Meth.in Physis Res.(in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Mechanical Properties if PbWO4 Scintillating Crystals." Nucl.Instr.Meth.in Physis Res.A37. 203-207 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Scintillation and Phosphorescence of PbWO_4 Crystals." Nucl.Instr.Meth.in Physis Res.A373. 333-346 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Further Studies on Excitation-Emission Spectra, Radiation Damages and Mechanical Properties of PbWO_4" Proc.Inter.Conf on INORGANIC SCINTILLATORS and THIER APPRICATIONS/p286-288.Delft, .The Netherlands, August 28-Sept 1. (1995)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Crystal Growth of BSO (Bi_4Si_3O_<12>) by Bridgman Method." Inter.Conf on Crystal Growth, June 18-23 1995, The Hauge. 716

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Growth Mechanism of BSO (Bi_4Si_3O_<12>) by Bridgman Technique." The Tenth American Conf on Crystal Growth, August 4-9,1996, Vail, Colorado.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Crystal Growth of Lange BSO (Bi_4Si_3O_<12>) for Radiation Detectors." The Tenth American Conf on Crystal Growth, August 4-9,1996, Vail, Colorado.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Crystal growth of Large BSO for Radiation Detectors" The 7^<th>china Japan Symposium on Science and Technology of Crystal Growth and Materials. Shanghai November 1-2. 83-84 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] K.Harada et al.: "Growth of BSO (Bi_4Si_3O_<12>) Single Crystal by Bridgman Technique." NCCG-26, AUG.8-10,1995, Morioka. 138

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Crystal Growth of Large BSO (Bi_4S_<13>O_<12>) Bridgman Technique." Proc.Of 41^<st> Symposium on Synthetic Crystals.Oct 6-7,1996, Fukuoka. 55-56

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: "Temperature Change Duning Crystal Growth of Oxides by Vertical Bridgman Technique." ibid. 79-80

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Ishii et al.: Handbook of Crystal Growth Scintillation Crystals. Kyouritsu Shuppansha, 8 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1996 Final Research Report Summary
  • [Publications] M.Kobayashi et al.: "Bismuth Silicate Bi_4Si_3O_<12>,A Faster Scintillatex thau Bismuth Geomanate Bi_4Ge_3O_<12>." Mucle Instr.and Meth.A372. 45-50 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] M.Ishii et al.: "Mechanical Properties of PbWO_4 Scintillating Crystals." Nucl.Instr.and Meth.A376. 203-207 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] M.Kobayashi et al.: "Scintillation and Phashorescence of PbWO_4 Crystal" Nucl.Instr.and Meth.A373. 333-346 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] M.Nikl et al.: "Radiation Induced Formation of Color Centers in PbWO_4 Single Crystals" J.Appl.Physics.(in press).

    • Related Report
      1996 Annual Research Report
  • [Publications] M.Kobayashi et al.: "Improvenent in Transmittance and Decay Time of PbWO_4 Scintillating Crystals by La-doping" Nucl.Instr.and Meth.(in press).

    • Related Report
      1996 Annual Research Report

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Published: 1995-04-01   Modified: 2016-04-21  

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