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Study of Positronium in Insulating Crystals

Research Project

Project/Area Number 08404018
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionThe University of Tokyo

Principal Investigator

HYODO Toshio  Graduate school of Arts and Sciences, The University of Tokyo, Professor, 大学院・総合文化研究科, 教授 (90012484)

Co-Investigator(Kenkyū-buntansha) SAITO Haruo  Graduate school of Arts and Sciences, The University of Tokyo, Research Associate, 大学院・総合文化研究科, 助手 (60235059)
NAGASHIMA Yasuyuki  Graduate school of Arts and Sciences, The University of Tokyo, Research Associate, 大学院・総合文化研究科, 助手 (60198322)
Project Period (FY) 1996 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥40,500,000 (Direct Cost: ¥40,500,000)
Fiscal Year 1999: ¥5,600,000 (Direct Cost: ¥5,600,000)
Fiscal Year 1998: ¥6,400,000 (Direct Cost: ¥6,400,000)
Fiscal Year 1997: ¥9,200,000 (Direct Cost: ¥9,200,000)
Fiscal Year 1996: ¥19,300,000 (Direct Cost: ¥19,300,000)
KeywordsPositron annihilation / Positron / Positronium / 2D-ACAR / Insulator / Alkali halide / Quartz / Spin-crossover salt / 合成石英 / 四重極相互作用 / スピン偏極 / 偏極率 / 局在ポジトロニウム / トンネル効果 / 陽電子ビーム / ライナック / 仕事関数 / 2光子角相関 / 拡散定数 / スルカリハライド / スビンクロスオーバー錯塩 / スピン転移 / スピン交換 / 非局在ポジトロニウム
Research Abstract

A positron injected in insulating material form a hydrogen-like bound state with an electron called positronium. Behavior of ositronium in insulating materials has attracted interests in relation with the properties of excitions. It is also realized as a probe of the spin states of materials.
The present study revealed various aspects of the positronium interactions with materials by using 2D-ACAR apparatus recently developed by us, the high intensity slow positron beam line at KEK, and conventional positron annihilation techniques including 1D-ACAR, positron lifetime ,Doppler broadening of annihilation radiation, positron age-momentum correlation.
New results have been obtained for the following subjects :
(1) Wave functions of delocalized positronium in alkali halides at low temperatures.
(2) Effect of the phonon scattering on the momentum distribution of positronium in quartz and MgFィイD22ィエD2.
(3) Tunneling transition of delocalized positronium to a self-localized state.
(4) Positronium emission from quartz single crystal and fused silica.
(5) Positronium lifetime in quartz single crystal.
(6) Study of spin-crossover material and related material by using positronium.
(7) Positronium quadrupole interactions in anistoropic crystals.
(8) Development of positron spin polarimeter by using positronium in solids.

Report

(5 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • 1996 Annual Research Report
  • Research Products

    (59 results)

All Other

All Publications (59 results)

  • [Publications] Y. Nagai: "A new two-dimensional angvlar correlation of annihilation radiation apparatus using positron-sensitive photomultiolier tubes"Nucl. Instr. Meth. A. 378. 629-632 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Two-dimensional Lr angular correlation study of delocalized positronium in alkali halids"J. Phys : Condens. Matter. 9. 11239-11246 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Saito: "Effect of ultraviolet on axide fine grains studied with positron annihilation and ESR"Mat. Sci. Forum. 255-257. 463-465 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Hyodo: "Use of newly developed compact LD-ACAR spectrometer for the study of positronium in solids"Mat. Sci. Forum. 255-257. 488-490 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Study of delocolized positronium in alkali halides by LD-ACAR"Mat. Sci. Forum. 255-257. 569-571 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Analyses of momentum distribution of Bloch-positronium in solids"Mat. Sci. Forum. 255-257. 596-598 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Morinaka: "Time-of-flight spectroscopy of positronium emitted from SiO<@D22@>D2 surface"Mat. Sci. Forum. 255-257. 689-691 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] I. V. Bonderev: "Positronium in alkali halides : Tunneling from the delocalized to the self-trapped state"Phys. Rev. B. 57. 11341-11348 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Local structural deformation in[Zn(ptz)<@D26@>D2](BF<@D24@>D2)<@D22@>D2 and [Fe(ptz)<@D26@>D2](BF<@D24@>D2)<@D22@>D2 crystals observed by positron onnibilation spectroscopy"Phys. Rev. B. 57. 14119-14122 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagashima: "Origins of positronium emitted from SiO<@D22@>D2"Phys. Rev. B. 58. 12676-12679 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J. Yamaura: "X-ray diffraction study of[Zn(1-propyltetrazole)<@D22@>D2)](BF<@D24@>D2)<@D22@>D2 single crystal"Phys. Rev. B. 58. 14098-14101 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Saito: "Positron annihilation in [Fe(ptz)<@D2n@>D2](BF<@D2n@>D2) and [Zn(ptz)<@D2n@>D2](BF<@D2n@>D2)<@D2n@>D2 single crystals studied with one-dimensional angular correlation of annihilation radiation"Jpn. J. Appl. Phys. Part I. 37. 111-112 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Saito: "Quencing of Positronium by surface paramagnetic centers in ultraviolet and positron-irradiated fine oxide grains"Phys. Rev. B. 60. 11070-11077 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Lifetime of delocalized positronium in a-SiO<@D22@>D2"Phys. Rev. B. 60. 7677-7679 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Suvegh: "Positronium as a sensitive detector of changes in molecular structure"Advances in Molecular Structure Research. 313-357 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Temperature dependence of momentum distribution of positronium in MeF<@D22@>D2, SiO<@D22@>D2, and H<@D22@>D2O"To be published in Phys. Rev. B.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Measurement of positron spin polarization by using the Doppeler"To be published in Nucl. Instr. A.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 兵頭 俊夫: "ポジトロニウムを用いた材料研究"まてりあ(日本金属学会誌). 35. 103-109 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 森中 康弘: "絶縁体表面のポジトロニウム放出"PF低速陽電子源建設報告(KEK Report). 2. 27 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 兵頭 俊夫: "AMOC法(寿命-運動量相関測定)"放射線. 24. 13-20 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 兵頭 俊夫: "陽電子を用いた物性研究"放射光. 11. 11-23 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, H. Saito, T. Iwata, Y. Nagashima, T. Hyodo, H. Uchida, and T. Omura: "A new two-dimensional angular Correlation of annihilation radiation apparatus using Position-sensitive photomultiplier tubes"Nucl. Instr. Meth. A. 378. 629-632 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, H. Saito, Y. Nagashima, N. Kobayashi, and T. Hyodo: "Two-dimensional 2 γ angular correlation study of delocalized positronium in alkali halides"J. Phys. ; Condens. Matter. 9. 11239-11246 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Saito and T. Hyodo: "Effect of ultraviolet irradiation on oxide fine grains studied with positron annihilation and ESR"Mat. Sci. Forum. 255-257. 463-465 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Hyodo, Y. Nagai, H. Saito, Y. Nagashima, A. Vertes, and K. Suvegh: "Use of newly developed compact 2D-ACAR spectrometer for the study of positronium in solids"Mat. Sci. Forum. 255-257. 488-490 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, H. Saito, Y. Nagashima, N. Kobayashi, and T. Hyodo: "Study of delocalized positronium in alkali halides by 2D-ACAR"Mat. Sci. Forum. 255-257. 569-571 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, M. Kakimoto, H. Ikari, and T. Hyodo: "Analysis of momentum distribution of Bloch-positronium in solids"Mat. Sci. Forum. 255-257. 596-598 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Morinaka, Y. Nagashima, Y. Nagai, T. Hyodo, T. Kurihara, T. shidara, and K. Nakahara: "Time-of-flight spectroscopy of positronium emitted from SiOィイD22ィエD2 surface"Mat. Sci. Forum. 255-257. 689-691 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] I. V. Bondarev and T. Hyodo: "Positronium in alkali halides : Tunneling from the delocalized to the self-trapped state""Phys. Rev. B. 57. 11341-11348 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, H. Saito, T. Hyodo, A. Vertes, and K. Suvegh: "Local structural deformation in [Zn(ptz)ィイD26ィエD2](BFィイD24ィエD2)ィイD22ィエD2 [Fe(ptz)ィイD26ィエD2](BFィイD24ィエD2)ィイD22ィエD2 crystals observed by positron annihilation spectroscopy"Phys. Rev. B. 57. 14119-14122 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagashima, Y. Morinaka, T. Kurihara, Y. Nagai, T. Hyodo, T. Shidara, and K. Nakahara: "Origins of positronium emitted from SiOィイD22ィエD2"Phys. Rev. B. 58. 12676-12679 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J. Yamaura, R. Kato, Y. Nagai, H. Saito, and T. Hyodo: "X-ray diffraction study of [Zn(1-propyltetrazole)ィイD26ィエD2](BFィイD24ィエD2)ィイD22ィエD2 single crystal"Pys. Rev. B. 58. 14098-14101 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. saito, Y. Nagai, T. Hyodo, K. Suvegh, and A. Vertes: "Positron annihilation in [Fe(ptz)ィイD26ィエD2](BFィイD24ィエD2)ィイD22ィエD2 and [Zn(ptz)ィイD26ィエD2](BFィイD24ィエD2)ィイD22ィエD2 single crystals studied with one-dimensional angular correlation of annihilation radiation""Jpn. J. Appl. Phys. Part 1. 37. 111-112 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Saito and T. Hyodo: "Quenching of positronium by surface paramagnetic centers in ultraviolet- and positron-irradiated fine oxide grains""Pys. Rev. B. 60. 11070-11077 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, Y. Nagashima, and Hyodo: "Lifetime of delocalized positronium in α-SiOィイD22ィエD2"Phys. Rev. B. 60. 7677-7679 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Suvegh, A. Vertes, and T. Hyodo: "Positronium as a sensitive detector of changes in molecular structure""Advances in Molecular Structure Research" edited by M. Hargittai and I.. Hargittai, (JAI Press, Stanford). 313-357 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, M. Kakimoto, T. Hyodo, K. Fujiwara, . Ikari, M. Eldrup, and A.T. Stewart: "Temperature dependence of momentum distribution of positronium in MgFィイD22ィエD2, SiO,ィイD22ィエD2, and HィイD22ィエD2O"Phys. Rev. B. To be published.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai, Y. Nagashima, J. Kim, Y. Itoh, and T. Hyodo: "Measurement of positron spin polarization by using the Doppler broadening method"Nucl. Instr. Meth. A. To be published.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Hyodo: ""Materials research using positronium" (in Japanese)"Materia (Bulletin of the Japan Institute of Metals). 35. 103-109 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Morinaka and Y. Nagashima: ""Positoronium emission from insulator surface" (in Japanese)"KEK Report. 27. 97-12 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Hyodo: ""AMOC (Age-momentum correlation measurement)" (in Japanese)"Hoshasen. 24. 13-20 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Hyodo: ""Materials research using positrons" (in Japanese)"Hoshako (Journal of the Japanese Society for Synchrotron Radiation Research). 11. 11-23 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Nagai: "Lifetime of delocalozed positronium in α-SiO_2"Phys. Rev. B. 60. 11070-11077 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K. Suregh: "Positron as a sensitive detector of changes in molecular structure""Advances in Molecular Structure Reserch" edited by M. Hargittai and I. Hargittai (JAI Press, Stanford). 313-357 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y. Nagai: "Temperature dependence of momentum distribution of positronium in MgF_2, SiO_2, and H_2O"To be published in Phys. Rev. B.

    • Related Report
      1999 Annual Research Report
  • [Publications] Y. Nagai: "Measurement of positron spin polarization by using the Doppler broadening method"To be published in Nuel. Instr. Meth. A.

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Saito: "Position Annihilation in 〔Fe(ptz)_6〕(BF_4)_2 and 〔Zn(ptz)_6〕(BF_4)_2 Single Crystals Studied with One-dimensional Angular Correlation of Annihilation Padiation" Jpn.J.Appl.Phys.Part 1. 37. 111-112 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] I.Bondorev: "Positronium in Alkali Hakides : Tunneling from the Delocalized to the Self-trapped state" Phys.Rev.B. 57. 11341-11348 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Nagai: "Local Structural Deforemation in 〔Zn(ptz)_6〕_2 and 〔Fe(ptz)_6〕(BF_4)_2 Crystals Observed by Positron Annihilation Spectrofcopy" Phys.Rev.B. 57. 14119-14122 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Nagashima: "Origin of Positronium Emitted from SiO_2" Phys.Rev.B. 58. 12676-12679 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] J.Yamaura: "X-ray Difftraction Study of 〔Zn(1-propyltetrazole)_6〕(BF_4)_2 Single Crystal" Phys.Rev.B. 58. 14098-14101 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 兵頭俊夫: "陽電子を用いた物性研究" 放射光(日本放射光学会誌). 11. 11-23 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 兵頭俊夫: "AMOC法(寿命-運動量相関測定)" 放射線. 24(No.3). 13-20 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Nagai: "Two-dimensional 2γ Angular Correlation Study of Delocalised Positromium in Alkal : Halides" journal of physics : Condensed matter. Vol.9. 11239-11246 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] H.Saito: "positron Amihilation in [Fe(Dtζ)_6](BF)_2 and [Zn(PC_2)_6](BF_4)_2 Single Crystals Studied with One-dimensional Argulcr Correlation of Annihilation Racliation" Japanese Journal of Applied Physics. Vol.27. 111-112 (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Morinaka: "Time-of-Flight Spectroscopy of Positronium Emission from SiO_2 Surface" Materials Science Forum. 255-257. 689-691 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Nagai: "Analysis of Momentum Distribution of Bloch-Positronium in Solids" Materials Science Forum. 255-257. 596-598 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] T.Hyodo: "Use of a Newly Developed Compact 2D-ACAR Spectrometer for the Study of Positronium in Solids" Materials Science Forum. 255-257. 488-490 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Nagai: "A new two-dimemsionnal angular correlation of ammihilation radiation apparatus using position-sensitive photomultiplier tubes" Nuclear Instruments & Methods in Physics Research. A378. 629-632 (1996)

    • Related Report
      1996 Annual Research Report

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Published: 1996-04-01   Modified: 2020-05-15  

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