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Artificial fabrication and magnetic properties of non-equilibrium ordered alloys by monatomic layr control

Research Project

Project/Area Number 08455316
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Structural/Functional materials
Research InstitutionTohoku University

Principal Investigator

TAKANASHI Koki  Tohoku Univ., Inst.Mater.Res.Associate Professor, 金属材料研究所, 助教授 (00187981)

Co-Investigator(Kenkyū-buntansha) SATO Katsuaki  Tokyo Univ.Agr.& Tech., Fac.Eng.Professor, 工学部, 教授 (50170733)
FUJIMORI Hiroyasu  Tohoku Univ., Inst.Mater.Res.Professor, 金属材料研究所, 教授 (60005866)
MITANI Seiji  Tohoku Univ., Inst.Mater.Res.Research Associate, 金属材料研究所, 助手 (20250813)
Project Period (FY) 1996 – 1997
Project Status Completed (Fiscal Year 1997)
Budget Amount *help
¥8,800,000 (Direct Cost: ¥8,800,000)
Fiscal Year 1997: ¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 1996: ¥6,600,000 (Direct Cost: ¥6,600,000)
Keywordsmonatomic layr control / ordered alloys / magnetic superlattices / perpendicular magnetic anisotropy / magnetooptical Kerr effect / 磁気力一効果 / 磁気力-効果
Research Abstract

We have compared structural and magnetic properties of the Ll_0-type FeAu ordered alloy fabricated by monatomic layr control to those of Fe (x ML) /Au (x ML) superlattices, where ML represents monatomic layr thickness. X-ray diffraction peaks corresponding to the superlattice period of x+x=2x ML have been observed definitely both for x=integers and non-integers. The X-ray diffraction patterns can be simulated by the model assuming a complete layr-by-layr growth with strucutural coherence throughout the sample, indicating the formation of coherent layred structure. The perpendicular magnetic anisotropy energy has been estimated from the in-plane and perpendicular magnetization curves. The product of the perpendicular anisotropy energy K_* and the Fe layr thickness t_<Fe>, K_*・t_<Fe>, for x=integers, decreases linearly with increasing t_<Fe> as seen in many magnetic superlattices. The interface anisotorpy energy K_s evaluated from the linear relationship increases with x for 1<less than … More or equal>x<less than or equal>3, and saturates for x<greater than or equal>4, which is explained by an extended Neel model. For x=non-integers, on the other hand, K_*・t_<Fe> vs.t_<Fe> deviates from the linear relationship, and shows oscillatory behavior with a period of 1 ML.We consider that this is a consequence associated with the reduction in K_s due to the interface roughness for x=non-integers. This study provides the first discovery of the oscillatory perpendicular anisotropy in magnetic superlattices. Furthermore, FMR measurements have indicated that the in-plane fourfold anisotropy also oscillates as a function of t_<Fe> with a period of 1.ML.In order to elucidate the origin for the oscillatory magnetic anisotropies, more precise structure analyzes including high resolution TEM,EXAFS and in situ STM are necessary. Magnetooptical measurements also indicate the oscillation of the Kerr rotation for the photon energy less than 2.5 eV.For 1<less than or equal>x<less than or equal>8, in addition, prominent structure around 3-4 eV has been observed, suggesting the formation of quantum well states of 3d electrons in Fe layrs. Less

Report

(3 results)
  • 1997 Annual Research Report   Final Research Report Summary
  • 1996 Annual Research Report
  • Research Products

    (28 results)

All Other

All Publications (28 results)

  • [Publications] K, Sato: "Magneto-Optical Spectra in Fe(xML)/Au(xML)Artificially Ordered Superlattices" 日本応用磁気学会誌. 20(2). 197-200 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 中澤 弘実: "単原子層蒸着によるAu(111)上[Fe(nML)/Au(nML)](n=1,2,3)多層膜の作製と垂直磁気異方性" 日本応用磁気学会誌. 20(2). 353-356 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] S, Mitani: "Structural and Magnetic properties of Fe/noble metal monatomic multilayers equivalent to L1_0 ordered alloys" J.Magn.Magn.Mater. 156. 7-10 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K, Sato: "Magneto-Optical Characterization of FeAu Artificial Ordered Alloy" J.Mag.Soc.Jpn. 20(S1). 35-40 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 高梨 弘毅: "単原子層積層制御によるL1_0型FeAu規則合金の構造と磁性" 固体物理. 31(10). 37-43 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 高梨 弘毅: "金属人工格子積層構造の極限への挑戦-単原子層積層制御による人工規則合金合成の試み" 日本金属学会報(まてりあ). 35(11). 1204-1207 (1996)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] S, Mitani: "Coherent Layered Structures in Fe/Au Monatomic Multilayers with Addition of Fractional Atomic Layers" Jpn.J.Appl.Phys.36・8A Part2. L1045-L1047 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K, Takanashi: "Oscillatory perpendicular magnetic anisotropy and lattice place spacing in Fe/Au superlattices" Appl.Phys.Lett.72・6. 737-739 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K, Takanashi: "Magenetooptical Kerr effect in Fe/Au superlattices modulated by integer atomic layers" J.Magn.Magn.Mater. 177-181. 1199-1200 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] 氷見 清和: "非整数原子層原子層交互蒸着Fe/Au人工格子の構造と垂直磁気異方性" 日本応用磁気学会誌. 22・4-2 印刷中. (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Sato: "Magneto-Optical Spectra in Fe (x ML) /Au (x ML) Artificially Ordered Superlattices" J.Man.Soc.Jpn.20 (2). 197-200 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] H.Nakazawa: "Fabrication of [Fe (n Ml) /Au (n Ml) ] (n=1,2,3) on Au (111) by Monatomic Layr Deposition and Perpendicular Magnetic Anisotropy [in Japanese]" J.Man.Soc.Jpn.20 (2). 353-356 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] S.Mitani: "Structural and magnetic properties of Fe/noble metal monatomic multilayrs equivalent to L1_0 ordered alloys" J.Magn.Magn.Mater.156. 7-10 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Sato: "Magnto-Optical Characterization of FeAu Artificial Ordered Alloy" J.Magn.Soc.Jpn.20 (S1). 35-40 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Takanashi: "Structural and Magnetic Properties of an L1_0-Type Ordered FeAu Alloy Fabricated by Alternate Monatomic Layr Deposition (Review) [in Japanese]" Kotaibutsuri. 31 (10). 37-43 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Takanashi: "A Challenge to the Limit of the Layred Structure in Metallic Superlattices - Fabrication of Artificial Ordered Alloys by Monatomic Layr Control (Review) [in Japanese]" Materia. 35 (11). 1204-1207 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] S.Mitani: "Coherent Layred Structure in Fe/Au Monatomic Multilayrs with Addition of Fractional Atomic Layrs" Jpn.J.Appl.Phys.36 (8A). L1045-L1047 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Takanshi: "Oscillatory perpendicular magnetic anisotropy and lattice plane spacing in Fe/Au superlattices" Appl.Phys.Lett.72 (6). 737-739 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Takanashi: "Magnetooptical Kerr effect in Fe/Au superlattices modulated by integer atomic layrs" J.Magn.Magn.Mater.177-181. 1199-1200 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] K.Himi: "Structure and Perpendicular Magnetic Anisotropy in Fe/Au Superlattices Modulated by Non-integer Atomic Layrs [in Japanese]" J.Magn.Soc.Jpn.22 (4-2) (in press). (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] S.Mitani: "Coherent Layered Structures in Fe/Au Monatomic Multilayers with Addition of Fractional Atomic Layers" Jpn.J.Appl.Phys.36・8A Part2. L1045-L1047 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] K.Takanashi: "Oscillatory perpendicular magnetic anisotropy and lattice plane apacing in Fe/Au superlattices" Appl.Phys.Lett.72・6. 737-739 (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] K.Takanashi: "Magenetooptical Kerr effect in Fe/Au superlattices" J.Magn.Magn.Mater.(印刷中). (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] 氷見清和: "非整数原子層原子層交互蒸着Fe/Au人工格子の構造と垂直磁気異方性" 日本応用磁気学会誌. 22・4-2(印刷中). (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] S. Mitani: "Structural and magnetic properties of Fe/noble metal monatomic multilayers equivalent to L10 ordered alloys" Journal of Magnetism and Magnetic Materials. 156. 7-10 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 高梨 弘毅: "単原子層積層制御によるL1_0型FeAl人工規則合金の構造と磁性" 固体物理. 31巻・10号. 37-43 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] 高梨 弘毅: "金属人工格子積層構造の極限への挑戦-単原子積層制御による人工規則合金合成の試み-" まてりあ(日本金属学会報). 31巻・11号. 1204-1207 (1996)

    • Related Report
      1996 Annual Research Report
  • [Publications] K. Sato: "MAGNETO-OPTICAL CHARACTERIZATION OF FeAl ARTIFICIALLY ORDERED ALLOY" Journal of Magnetics Society of Japan, Suppl.Vol. 20 No. S1. 35-40 (1996)

    • Related Report
      1996 Annual Research Report

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Published: 1996-04-01   Modified: 2016-04-21  

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