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Measurements of the vertical distributions of ozone and related species using high resolution FTIR

Research Project

Project/Area Number 08640559
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Space and upper atmospheric physics
Research InstitutionNagoya University

Principal Investigator

NAKAJIMA Hideaki  Nagoya Univ., Solar-Terr.Env.Lab., Research Associate, 太陽地球環境研究所, 助手 (20217722)

Co-Investigator(Kenkyū-buntansha) MURATA Isao  Tohoku Univ., Dep.of Science, Research Associate, 理学研究科, 助手 (00291245)
TAGUCHI Makoto  National Institute of Polar Research, Associate Professor, 助教授 (70236404)
KOIKE Makoto  Nagoya Univ., Solar-Terr.Env.Lab., Research Associate, 太陽地球環境研究所, 助手 (00225343)
KONDO Yutaka  Nagoya Univ., Solar-Terr.Env.Lab., Professor, 太陽地球環境研究所, 教授 (20110752)
Project Period (FY) 1996 – 1997
Project Status Completed (Fiscal Year 1997)
Budget Amount *help
¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 1997: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 1996: ¥1,300,000 (Direct Cost: ¥1,300,000)
Keywordsinfrared spectroscopy / FTIR / vertical profile / retrieval / stratosphere / ozone / trace constituents / laser-heterodyne / 大気化学
Research Abstract

We installed the Tunable Diode Laser Heterodyne Spectrometer (TDLHS) at Moshiri Observatory, Nagoya University in October, 1996. Measurement of Solar infrared spectra using TDLHS and Fourier-Transform Infrared Spectrometer (FTIR) were made for two weeks simultaneously. Absorption spectra of several trace molecules such as O3, N2O,HCl, HF,and HNO<@D23@>D2 were taken. Also ozonesonde measurements were conducted at Moshiri Observatory. Vertical profiles of volume mixing ratios (VMRs) of O3 were retrieved from these high-resolution solar spectra. The VMR profile retrieval is based on an iterative inversion algorithm, which utilizes line-by-line, layr-by-layr calculations. Eighty ozone vertical profiles were retrieved from the two spectral regions from 40 spectra and were compared with 17 ozonesonde measurements from a nearby station. Average differences between 18 and 34 km were less than (]SY.+-。[) 12%. The standard deviation of the average differences between 18 and 34 km were less than 20%. Effects of several different factors on errors of profile retrievals, such as initial guess, temperature profiles, and instrument line shape functions, were evaluated by numerical simulation. The estimated errors were extremely consistent with the observed errors between 18 and 34 km, suggesting that the FTIR was optically well adjusted. In general, it was found that retrieval of the O3 profile gives VMRs in an accuracy better than 40% at 14 km, improving to 10-15% between 18 and 30 km, with precision of 30% and 20% for these altitude ranges, respectively.

Report

(3 results)
  • 1997 Annual Research Report   Final Research Report Summary
  • 1996 Annual Research Report
  • Research Products

    (11 results)

All Other

All Publications (11 results)

  • [Publications] Nakajima, H., et al.: "Retrieval of vertical profiles of ozone from high-resolution infrared solar spectra at Rikubetsu,Japan" J.Geophys.Res.102. 29,981-29,990 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Nakajima, H., et al.: "Accuracy of total ozone column amounts observed with solar infrared spectroscopy" Geophys.Res.Lett.24. 77-80 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Nakajima, H., et al.: "Carbon monoxide column abundances and tropospheric concentrations retrieved from high resolution graund-based infrared solar spectra at 43.5°N over Japan" J.Gephys.Res.102. 23,403-23,411 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Nakajima, H., X.Liu, I.Murata, Y.Kondo, F.J.Murcray, M.Koike, Y.Zhao, and H.Nakane: "Retrieval of vertical profiles of ozone from high-resolution infrared solar spectra at Rikubetsu, Japan" J.Geophys.Res.102. 29981-29990 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Murata, I., Y.Kondo, H.Nakajima, M.Koike, Y.Zhao, W.A.Matthews, and K.Suzuki: "Accuracy of total ozone column amounts observed with solar infrared spectroscopy" Geophys.Res.Lett.24. 77-80 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Zhao, Y., Y.Kondo, F.J.Murcray, X.Liu, M.Koike, K.Kita, H.Nakajima, I.Murata, and K.Suzuki: "Carbon monoxide column abundances and tropospheric concentrations retrieved from high resolution ground-based infrared solar spectra at 43.5゚N over Japan" J.Geophys.Res.102. 23403-23411 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1997 Final Research Report Summary
  • [Publications] Nakajima,H., et al.: "Retrieval of vertical profiles of ozone from high-resolution infrared solar spectra at Rikubetsu,Japan" J.Geophys.Res.102. 29,981-29,990 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Nakajima,H., et al.: "Accuracy of total ozone column amounts observed with solar infrared spectroscopy" Geophys.Res.Lett.24. 77-80 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Nakajima,H., et al.: "Carbon monoxide column abundances and tropospheric concentrations retrieved from high resolution ground-based infrared solar spectra at 43.5° N over Japan" J.Geophys.Res.102. 23,403-23,411 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] I.Murata: "Accuracy of total ozone column amounts observed with sdar infrared spectroscopy" Geophysical Research Letters. 24. 77-80 (1997)

    • Related Report
      1996 Annual Research Report
  • [Publications] H.Nakajima: "Retrieval of height profiles of stratospheric ozone from ground-based infrared solar spectra obtained at Rikubetsu,Japan" Proceedings of 18th Ozone Symposium-96 (L'Aquila). (1997)

    • Related Report
      1996 Annual Research Report

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Published: 1996-04-01   Modified: 2016-04-21  

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