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Effects of Aerosol Particles on Atmospheric Environment

Research Project

Project/Area Number 09044161
Research Category

Grant-in-Aid for Scientific Research (B).

Allocation TypeSingle-year Grants
Section一般
Research Field 環境影響評価(含放射線生物学)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

KASAHARA Mikio  Kyoto Univ., Graduate School of Energy Science, Professor, エネルギー科学研究科, 教授 (80027143)

Co-Investigator(Kenkyū-buntansha) HORVATH Helmuth  Univ. Vienna, Institute of Experimental Physics, Professor, 実験物理学科, 教授
YAMAMOTO Kohei  Kyoto Univ., Graduate School of Energy Science, Lecturer, エネルギー科学研究科, 助手 (10263154)
TOHNO Susumu  Kyoto Univ., Graduate School of Energy Science, Assoc. Prof., エネルギー科学研究科, 助教授 (80135607)
GANGL Martine s.  Univ. Vienna, Institute of Experimental Physics, Researcher, 実験物理学科, 研究員
KRUISZ Christian  Univ. Vienna, Institute of Experimental Physics, Researcher, 実験物理学科, 研究員
KRUISZ Chris  ウィーン大学, 実験物理学科, 研究員
HELMUTH Horv  ウィーン大学, 実験物理学科, 教授
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 1999: ¥1,300,000 (Direct Cost: ¥1,300,000)
Fiscal Year 1998: ¥1,200,000 (Direct Cost: ¥1,200,000)
Fiscal Year 1997: ¥1,200,000 (Direct Cost: ¥1,200,000)
KeywordsAtmospheric aerosols / Atmospheric environmental effects / Global warming / cooling / Fog and raindrops / Fixation of liquid particles / Elemental analysis / Acid deposition / Long-range transport model / 元素濃度 / PIXE分析 / エアロゾル粒子 / 大気環境 / 元素状炭素 / 有機炭素 / 酸性雨
Research Abstract

Atmospheric aerosols play an important role in environmental problem. To evaluate the effects of aerosol on atmospheric environment, the three works : (1) Physical and chemical characteristics of atmospheric aerosols, (2) Global warming/cooling effects of atmospheric aerosols, (3) Mechanism of acid rain/acid deposition, were carried out during 1997-1999.
1. Characteristics of atmospheric aerosols
Physical and chemical properties were investigated under the various meteorological and environmental conditions. The particle size distribution of mass was expressed always as a bimodal distribution that was divided into fine and coarse fraction at around 1-2μm. The size distribution of each chemical component was classified into three types : single modal distribution within either fine or coarse fraction and the bimodal one as well as total mass. Water solubility of aerosols depended strongly upon their elemental components. Although Fe, Si and Ti showed high insolubility, almost whole of S a … More nd Cl dissolved.
2. Global warming/cooling effects of atmospheric aerosols
The simultaneous measurements of aerosol properties and radiation were performed as the campaign experiments at ground in 1998 and at both ground and aircraft in 2000, as well as the routine measurement. The radiative forcing was calculated from radiation and aerosol data. The average radiative forcing in Kyoto and Nagoya were -1.5 and +3.3W/mィイD12ィエD1, respectively. The difference in their values originates in the difference of chemical composition, i.e. optical property of aerosols.
3. Mechanisms of acid rain/acid deposition
The sampling method and treatment procedures to fix fog-and rain-droplets were investigated and the elemental analysis of the fixed single particle was tried applying PIXE and micro-PIXE analyses. Liquid particles were easily fixed by either exposing to cyanoacrylate vapor or freezing method. The elemental concentrations in single raindrop were obtained as a function of raindrop diameter. The concentrations in raindrop were extremely high at the begging of rain. Less

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (61 results)

All Other

All Publications (61 results)

  • [Publications] M.Kasahara: "Application of PIXE techanique to studies on atmospheric environment"Proceedings of the 34th seminar on science and technology. 179-186 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S.Tohno: "Numerical simulation of belowcloud scavenging of gascous and particulate matters"J. Aerosol Sci. 28. (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "Comparson of the Light Absorption Coefficient and Carbon measures for Remote Acrosols : an Independent Analysis of Data from the Improve Network I and II"Atmospheric Environment. 31. 2885-2887 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "A Study of the Aerosol of Santiago de Chile III Light Absorption Measurements"Atmospheric Environment. 31. 3737-3744 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "Systematic Deviations of Light Absorption Measurements by Filter Transmission"J. Aerosol Science. 28. (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "Experimental Calibration of Aerosol Light Absorption Measuremetnts Using the Integrating Plate Method- Summary of the Data"J. Aerosol Science. 28. 1149-1161 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 東野達: "エアロゾル計測におけるデータ逆変換"エアゾル研究. 12. 281-287 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 笠原三紀夫: "大気環境研究へのPIXE法の応用"放射線. 23. 87-96 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "Physical and chemical Characteristics of atmospheric aerosols in urban area"Abstracts of 16th Annual AAAR Confernce. 251 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 東野達: "二次元同時蒸着混合薄膜を用いた個別エアロゾル粒子中の硫酸塩および硝酸塩混合状態の同定"エアゾル研究. 13. 230-236 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S.Tohno: "Application of X-ray Absorption Fine Structure(XAFS) Spectrometry to Identify the Chemical States of Atmospheric Aerosols"J. Aerosol Science. 29. (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "Wet Scavenging of Atmospheric Aerosols by Rain Water"Abstracts of 17th Annual AAAR Confernce. 15 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "Physical and chemical characteristics of atmospheric aerosols in Kyoto"J. Aerosol Science. 30. (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 山本浩平: "東アジア地域における人為起源硫黄酸化物排出量地図の作成"大気環境学会誌. 34. 435-444 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "Single particle analysis-Its importance in aerosol research"Abstracts of First Asia Aerosol Cnference. 136-137 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "New Approach for Characterization of Single Liquid Particle"Abstracts of 18thAnnual AAAR Cnference. 156 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S.Tohno: "Chemical Characterzation of Atmospheric Aerosols by PIXE and Other Analytical Technique"Abstracts of 3rd International Symposium on Bio-PIXE. 27 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 山本浩平: "東アジア地域における資源・人為起源硫黄化合物からの沈着量推定-雲内変質過程を考慮した長距離輸送もでる開発と評価-"大気環境学会誌. 25. 21-35 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara: "Characterization of atmospheric aerosols using PIXE, EAS, and IC"Extended Abstracts of PM2000. 1. 36-37 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "Aerosols : An Introduction"J. Environmental Radioactivity. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Horvath: "Optical Characteristics of the Aerosol IN Austria and Spain"J. Aerosol Science. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara(分担): "Aerosols : Generation and Role in Medicine, Industry and Environment"Allied Pub. Lim.. (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara(分担): "Analytical Chemistry of Aerosols"Lewis Publisher. (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara: "Application of PLXE technique to studies on atmospheric environment"Proceedings of the 34th Seminar on Science and Technology.. 179-186 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Tohno, J. Ueda and M. Kasahara: "Numerical simulation of below-cloud scavenging of gaseous and particulate matters"J. Aerosol Science. 28. S455-456 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath: "Comparison of the Light Absorption Coefficient and Carbon measures for Remote Aerosols : an Independent Analysis of Data from the Improve Network I and II : Discussion"Atmospheric Environment. 31. 2885-2887 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath, L. Catalan, A. Trier: "A Study of the Aerosol of Santiago de Chile III Light Absorption Measurements"Atmospheric Environment. 31. 3737-3744 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath: "Systematic Deviations of Light Absorption Measurements by Filter Transmission Methods"J. Aerosol Science. 28. S55-S56 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath: "Experimental Calibration of Aerosol Light Absorption Measurements Using the Integrating Plate Method-Summary of the Data"J. Aerosol Science. 28. 1149-1161 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Tohno: "Data inversion on the measurement of the size distribution of aerosols (in Japanese)"J. Aerosol Research, Japan. 12. 281-287 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara: "Application of PLXE to Atmospheric Environmental Study (in Japanese)"Radiation. 23. 87-96 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, S. Chatani, K. Yamamoto and S. Tohno: "Physical and chemical Characteristics of atmospheric aerosols in urban area"Abstracts of 16th Annual AAAR Conference. 251 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Tohno, S. Chatani and M. Kasahara: "Identification of mixing state of sulfate and nitrate ions in individual aerosol particles using a mixing thin film created by dual simultaneous vacuum deposition (in Japanese)"J. Aerosol Research, Japan. 13. 230-236 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Tohno, J. Kawai, S. Chatani, M. Ohta, Y. Kitajima, K. Yamamoto, Y. Kitamura and M. Kasahara: "Application of X-ray absorption fine structure (XAFS) spectro-metry to identify the chemical states of atmospheric aerosols"J. Aerosol Science. 29. S235-S236 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, J. -H. Park, K. Yamamoto, S. Tohno: "Wet Scavenging of Atmospheric Aerosols by Rain Water"Abstracts of 17th Annual AAAR Conference. 15 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, T. Chatani, S. Tohno and R. Holler: "Physical and chemical characteristics of atmospheric aerosols in Kyoto"J. Aerosol Science. 30. S257-S258 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Yamamoto, J. Hoshino, T. Yoshida, M. Kasahara: "Estimate of Anthropogenic sulfur dioxide emission in East Asia (in Japanese)"J.Japan Society of Atmospheric Environment. 34. 435-444 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, S. Tohno, S. Akashi and C. J. Ma: "Single particle analysis-Its importance in aerosol research"Abstracts of First Asia Aerosol Conference. 136-137 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, S. Akashi, S. Tohno: "New Approach for Characterization of Single Liquid Particle"Abstracts of 18th Annual AAAR Conference. 156 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Tohno: "Chemical Characterization of Atmospheric Aerosols by PLXE and Other Analytical Technique"Abstracts of 3rd International Symposium on Bio-PLXE. 27 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Yamamoto, T. Yoshida, M. Araki, J. Hoshino, M. Kasahara: "Estimate of sulfur deposition from natural and anthropogenic sources in East Asia-Development of long-range transport model with rainout and washout processes"J. Japan Society of Atmospheric Environment. 35. 21-35 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara, C. J. Ma and S. Tohno: "Characterization of atmospheric aerosols using PLXE, EAS, and IC"Extended Abstracts of PM2000. 1. 36-37 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath: "Aerosols : An Introduction"J. Environmental Radioactivity. in printing.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Horvath, L. Alados, F. Olmo, O. Jovanovic, M. Gangl, W. Kaller and C. Sanchez: "Optical Characteristics of the Aerosol in Austria and Spain"J. Aerosol Science. in printing.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara: "Physical and chemical characteristics of atmospheric aerosols and their effects on the global environment, in Aerosols : Generation and Role in Medicine, Industry and Environment"Allied Pub. Lim.. 315. 207-223 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kasahara: "Characterization of atmospheric aerosols and aerosol studies applying PIXE analysis, in analytical chemistry of aerosols"Lewis Publisher. 486. 145-171 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Kasahara,T.Chatani,S.Tohno,R.Holler: "Physical and chemical characteristics of atmospheric aerosols in Kyoto"J. Aerosol Science. 30,S1. S257-S258 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kasahara,S.Tohno,S.Afashi,C.J.Ma: "Single particle analysis-Its importance in aerosol research ?"Abstracts of First Asia Aerosol Conference. 136-137 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] R.Holler,M.Kasahara,K.Gotoh,Y.Iwasaka: "A study on the relationship of potical and chemical aerosol properties at Nagoya"Abstracts of First Asia Aerosol Conference. 241-242 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kasahara,C.J.Ma,S.Tohno: "Characterization of atmospheric aerosols using PIXE, EAS and IC"Extended Abstracts of PM2000: Particulate Matter and Health. 36-37 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] 山本浩平,吉田知央,荒木真,星野順至,笠原三紀夫: "東アジア地域における資源・人為起源硫黄化合物からの沈着量推定-雲内変質過程を考慮した長距離輸送モデルの開発と評価-"大気環境学会誌. 35,1. 21-35 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] 安座間信暁,南齋規介,東野達,笠原三紀夫: "粒子状大気汚染物質の起源別排出量の推定と解析"第16回エネルギーシステム・経済・環境コンファレンス講演論文集. 129-134 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] Mikio Kasahara: "Analytical Chemistry of Aerosols (分担執筆)"Lewis Pubisher. 486(145-171) (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 東野 達: "二元同時蒸着混合薄膜を用いた個別エアロゾル粒子中の硫酸塩および硝酸塩混合状態の同定" エアロゾル研究. 13・3. 230-236 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Susumu Tohno: "Application of X-ray Absorption Fine Structure(XAFS)Spectrometry to Identify the Chemical States of Atmospheric Aerosols" Journal of Aerosol Science. 29・S1. S235-S236 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 笠原三紀夫(共著): "明日のエネルギーと環境" 日本工業新聞社, 249 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] M.Kasahara(共著): "Aerosols:Generation and Role in Medicine,Industry and Environment" Allied Publishers Lt., 315 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 笠原 三紀夫: "大気環境研究へのPIXE法の応用" 放射線. 23・4. 87-96 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] 東野 達: "エアロゾル計測におけるデータ逆変換" エアロゾル研究. 12・4. 281-287 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Li and M.Kasahara: "Analysis of acid rain 1991〜1995 and regional climate in south China" J.Japan Society of Atmospheric Environment. 33・1. 50-59 (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] S.Tohno, J.Ueda and M.Kasahara: "Numerical simulation of below-cloud scavenging of gaseous and particulate matters" Journal of Aerosol Science. 28・S. S455-S456 (1997)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2016-04-21  

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