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Development of Neutron Dosimetry Technique Based on Resonant Laser Ablation with Tunable Diode Laser

Research Project

Project/Area Number 09308014
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field エネルギー学一般・原子力学
Research InstitutionNagoya University

Principal Investigator

IGUCHI Tetsuo  Nagoya University, Graduate School of Engineering, Professor, 工学研究科, 教授 (60134483)

Co-Investigator(Kenkyū-buntansha) TAKAHASHI Hiroyuki  The University of Tokyo, Graduate School of Engineering, Associate Professor, 工学系研究科, 助教授 (70216753)
URITANI Akira  Nagoya University, Graduate School of Engineering, Associate Professor, 工学研究科, 助教授 (10213521)
ENOKIDA Yoh-ichi  Nagoya University, Graduate School of Engineering, Associate Professor, 工学研究科, 助教授 (40168795)
KAWARABAYASHI Jyun  Nagoya University, Graduate School of Engineering, Research Assistant, 工学研究科, 助手 (80283414)
HASEGAWA Syu-ichi  The University of Tokyo, Graduate School of Engineering, Lecturer, 工学系研究科, 講師 (90262047)
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥23,600,000 (Direct Cost: ¥23,600,000)
Fiscal Year 1999: ¥2,500,000 (Direct Cost: ¥2,500,000)
Fiscal Year 1998: ¥9,200,000 (Direct Cost: ¥9,200,000)
Fiscal Year 1997: ¥11,900,000 (Direct Cost: ¥11,900,000)
KeywordsResonance Ionization / Laser Ablation / Isotope Analysis / Tunable Diode Laser / Nuclear Reaction Product / Neutron Dosimetry
Research Abstract

The present study is aiming at the development of innovative technique to measure the concentration and/or isotopic ratio of trace elements produced by nuclear reactions with neutrons and new application to nuclear engineering by using Resonant Ionization Spectroscopy (RIS), which has fundamental features of ultra high sensitivity and good elemental selectivity. In particular, we propose to make good use of 'Resonant Laser Abration (RLA)', which combines laser ablation and RIS simultaneously with a single laser. For this purpose, our research subjects are roughly classified into two categories ; one is to understand the basic process of RLA phenomena experimentally and to establish a theoretical model for RLA, and the other is to develop an RLA analytical system with a tunable diode laser, which would be suitable for engineering application, in particular for neutron dosimetry.
The main results are summarized as follows ;
(1) The basic experimental data base has been systematically obtained for RLA phenomena on several elements of nuclear nuaterials.
(2) The theoretical model for RLA has been successfully developed to reproduce the experimental resuls quantitatively. Based on this theoretical calculation, the methodology was established to search an optimal condition on laser power for detection of an element of interest.
(3) Through basic experiments to detect ^<27>Al (n, 2n) ^<26>Al reaction in an Al sample which was heavily irradiated by 14MeV neutrons, the applicability of RLA has been demonstrated as new neutron dosimetry technique.
(4) Some useful findings have been obtained to make basic design of an RLA analytical system with a tunable diode laser and a quadrupole mass spectrometer suitable for engineering application, and athe technical problems to be solved have been also made clear.

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (12 results)

All Other

All Publications (12 results)

  • [Publications] K.Watanabe: "Development of Resonant Laser Ablation Technique for Detection of Trace Elements Produced by Nuclear Reactions"Proc. 11th W.S on Radiation Detectors and Their Uses, KEK Proc.. 97-8. 128-134 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Nakazawa: "Standard neutron fields and researches on advanced nuclear measurement technique"Progress in Nuclear Energy. 32・1/2. 25-41 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe: "Modeling of Vaporization Processes of Resonant Laser Ablation"Applied Physics A. 69[Suppl.]. S845-S848 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe: "Development of Failed Fuel Detection and Location Technique Using RIMS : Improvement of the Detection Limit with Pulsed Supersonic Valve"Proc. 14^<th> WS on Radiation Detectors and Their Uses, KEK Proc.. 2000-14. 183-190 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe: "Optimization of Trace Element Analysis Using Resonant Laser Ablation"Proc. 10^<th> Int. Symp. on RIS and Its Applications, Oct. 8-12, 2000, Knoxville, USA (To be published in AIP Conf. Proc.). 43 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe, T.Iguchi, Y.Yamane, J.Kawarabayashi and Y.Sato: "Development of Resonant Laser Ablation Technique for Detection of Trace Elements Produced by Nuclear Reactions"Proc.11th W.S on Radiation Detectors and Their Uses, KEK Proc.. 97-8. 128-134 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Nakazawa, T.Iguchi, H.Takahashi and E.Takada: "Standard Neutron Fields and Researches on Advanced Nuclear Measurement Technique"Progress in Nuclear Energy. Vol.32, No.1/2. 25-41 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe and T.Iguchi: "Modeling of Vaporization Processes of Resonant Laser Ablation"Applied Physics. A69 [Suppl.]. S845-S848 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe, T.Iguchi, T.Ogita, T.Watanabe, A.uritani, J.Kawarabayashi, H.Harano and S.Nose: "Development of Failed Fuel Detection and Location Technique Using Resonance Ionization Mass Spectrometry : Improvement of the Detection Limit with Pulsed Supersonic Valve"Proc.14^<th> WS on Radiation Detectors and Their Uses, KEK Proc.. 2000-14. 183-190 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe and T.Iguchi: "Optimization of Trace Element Analysis Using Resonant Laser Ablation"Proc.10^<th> Int. Symp. on RIS and Its Applications, Oct. 8-12, 2000, Knoxville, USA. (To be published in AIP Conf.Proc.). 43 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Watanabe: "Modeling of Vaporization Processes of Resonant Laser Ablation"Proc. 5th Int. Conf. on Laser Ablation (COLA99), July 19-23, 1999, Goettingen, Germany (to be Published in Appl. Phys.A). (発行予定). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] 荻田利幸: "共鳴イオン化質量分析法を用いた破損燃料検出システムの開発"放射線. 25・2. 89-93 (1999)

    • Related Report
      1999 Annual Research Report

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Published: 1997-04-01   Modified: 2016-04-21  

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