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Time-domain coherent phonon spectroscopy and dynamics of structural change

Research Project

Project/Area Number 09440119
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionOsaka University

Principal Investigator

NAKASHIMA Shin-ichi  Department of Applied Physics, Osaka University, Professor, 大学院・工学研究科, 教授 (20029226)

Co-Investigator(Kenkyū-buntansha) KISODA Kenji  Department of Applied Physics, Osaka University, Research Associate, 大学院・工学研究科, 助手 (90243188)
MIZOGUCHI Kohji  Department of Applied Physics, Osaka University, Research Associate, 大学院・工学研究科, 助手 (10202342)
HARIMA Hiroshi  Department of Applied Physics, Osaka University, Associate Professor, 大学院・工学研究科, 助教授 (00107351)
Project Period (FY) 1997 – 1998
Project Status Completed (Fiscal Year 1998)
Budget Amount *help
¥14,500,000 (Direct Cost: ¥14,500,000)
Fiscal Year 1998: ¥3,800,000 (Direct Cost: ¥3,800,000)
Fiscal Year 1997: ¥10,700,000 (Direct Cost: ¥10,700,000)
Keywordscoherent phonons / femotosecond pulse laser / plasmon LO-phonon coupled mode / ultra fast dynamics / semiconductor / semimatal / semiconductor superlattice / フェムト秒パルスレーザー
Research Abstract

We have constructed a system for measurement of high frequency coherent oscillations of phonons and electrons in solids, using Ti : sapphire pulse lasers with 〜 ten femtosecond duration. The characteristics of the constructed system has been evaluated by measurements of the coherent phonons in various materials and the SHG signals. The pulse duration of 16fs and reflectivity change (ΔR/R) of the order of 10-7 have been obtained. Using this system we were able to measure the coherent phonons in Ge with a good S/N ratio, which was so far difficult to observe them. We have examined coherent phonons in semimetals, superlattices, semiconductors, semiconductor- and semimetal-and materials which undergo phase transition.
The results of our studies are as follows :
(1) We have found from a comparison of the Raman and coherent phonon spectra that the decay of the coherent phonons is mainly governed by the energy relaxation and that the contribution of the pure dephasing is very small in Bi.
(2) Fo … More r Bi/Sb superlattices, we have first observed coherent oscillations of optical modes confined in the constituent layers, Bi-Sb interface modes, folded longitudinal acoustic modes. The deviation of the observed frequency of the coherent folded modes from the calculated ones is attributed to elastic anomaly in very thin Bi layers.
(3) We have produced pulse trains using spatial modulation filters and a grating pair and experimentally proved that the control of the amplitude of the coherent phonons and the selective excitation of specified phonon modes are possible for Bi/Sb mixed crystals.
(4) We have first observed both the upper and lower branches of coherent LO-phonon plasmon coupled modes in GaAs and InP. We also determined carrier density dependence of coupled-mode decays and discussed the dynamics.
(5) The coherent oscillations of folded longitudinal acoustic phonons are observed in GaAs-AlAs superlattices. We have obtained a clue for understanding the generation and detection mechanisms for the coherent phonons.
(6) We have observed coherent phonons in materials which undergo phase transitions in VィイD22ィエD2OィイD23ィエD2, η-MoィイD24ィエD2OィイD211ィエD2 and GeTe and obtained much information on the mechanisms of the generation and relaxation of the coherent phonons. Less

Report

(3 results)
  • 1998 Annual Research Report   Final Research Report Summary
  • 1997 Annual Research Report
  • Research Products

    (43 results)

All Other

All Publications (43 results)

  • [Publications] M.Hase: "Dynamics of coherent plasmon-phonon coupled modes in GaAs using ultrashort laser pulses,"Journal of Luminescence,. 76. 68-71 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M.Hase: "Dynamics of coherent phonons in bismuth generated ultrashort laser pulses,"Physical Review B,. 58. 5448-5442 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kisoda: "Coherent phonons from the CDW state in \ ゜Mo_4O_<11>,"Physical Review B,. 58. 7484-7487 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] O.Misochko: "Optical study of the Mott transition in V_2O_3 : Comparison of time and frequency-domain results,"Physical Review B,. 58. 12879-12794 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kisoda: "Pump power dependence of coherent phonons in \Mo_4O_<11>,"Physica B,. 263. 51-53 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Misoguchi: "Study of coherent folded acoustic phonons in semiconductor superlattices by pump-probe techniqve."Physica B,. 263. 48-50 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Mizoguchi: "Resonance E Aect of Coherent Folded Acoustic Phonons Generated by Ultrashort Light Pulses in GaAs/AlAs Superlattices,"Physica B,. 249. 887-890 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M.Hase: "Selective enhancement of coherent optical phonons using THz-rate pulse train,"Japanese Journal of Applied Physics. 37. 281-283 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S.Nakashima: "Coherent Phonon Oscillations in Photo-Excited Semiconductors and Semimetals,"Journal of Luminescence,. 76. 6-14 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S.Nakashima: "Coherent phonons in mixed semimetals and semimetal superlatioes,"Physica B,. 263. 67-69

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Mizoguchi: "Study of coherent folded acoustic phonons by pump-probe technique,"International Workshop on Current Topics of Laser Technology. 39 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M.Hase: "Generation of coherent THz phonons in Bi-Sb mixed crystals,"International Workshop on Current Topics of Laser Technology. 37 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kisoda: "Coherent phonons from quasi-two-dimensional conductor \-Mo_4O_<11>,"in International Workshop on Current Topics of Laser Technology Kobe. 76 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] O.V.Misochko: "Coherent phonons in V_2O_3 above and below the Mott transition"in International Workshop on Current Topics of Laser Technology Kobe. 78 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 中島信一: "固体におけるコヒーレントフォノン,"表面科学. 19-2. 2-9 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 中島信一: "フェムト秒領域のコヒーレントフォノンの振舞"日本物理学会誌. 53-8. 607-611 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M. Hase, K. Mizoguchi, H. Harima, F. Miyamaru, S. Nakashima, R. Fukasawa, M. Tani and K. Sakai: "Dynamics of coherent plasmon-phonon coupled modes in GaAs using ultrashort laser pulses"Journal of Luminescence. Volume 76 & 77. 68-71 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M. Hase, K. Mizoguchi, H. Harima, S. Nakashima, and K. Sakai: "Dynamics of coherent phonons in bismuth generated by ultrashort laser pulses"Physical Review B. Volume 58. 5448-5442 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K. Kiasoda, M. Hase, H. Harima, S. Nakashima, M. Tani, K. Sakai, H. Negishi and M. Inoue: "Coherent phonons from the CDW state in \° MoィイD24ィエD2OィイD211ィエD2"Physical Review B. Volume 58. R7484-R7487 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] O. Misochko, M. Tani, K. Sakai, K. Kisoda, S. Nakashima, V. N. Andreev, and F. A. Chudnovskiy: "Optical study of the Mott transition in VィイD22ィエD2OィイD23ィエD2 Comparison of time- and frequency-domain results"Physical Review B. Volume 58. 12879-12794 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K. Kisoda, M. Hase, H. Harima, S.Nakashima, K. Sakai, M. Tani, H. Negishi, and M. Inoue: "Pump power dependence of coherent phonons in \-MoィイD24ィエD2OィイD211ィエD2"Physica B. vol. 263-264. 51-53 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K. Mizoguchi, M. Hase, S. Nakashima, and M. Nakayama: "Study of coherent folded acoustic phonons in semiconductor superlattices by pump-probe technique"Physica B. vol. 263-264. 48-50 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K. Mizoguchi, K. Matsutani, M. Hase, S. Nakashima, and M. Nakayama: "Resonance E Aect of Coherent Folded Acoustic Phonons Generated by Ultrashort Light Pulses in GaAs/AlAs Superlattices"Physica B. vol. 249-251. 887-890 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M. Hase, K. Mizoguchi, H. Harima, S. Nakashima, and K. Sakai: "Selective enhancement of coherent optical phonons using THz-rate pulse train"Japanese Jpurnal of Applied Physics. Volume 37. L281-L283 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S. Nakashima, K. Mizoguchi, H. Harima, and K. Sakai: "Coherent Phonon Oscillations in Photo-Excited Semiconductors and Semimetals"Journal of Luminescence. vol. 76/77. 6-14 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S. Nakashima, M. Hase, K. Mizoguchi, H. Harima, K. Sakai, S. Cho, A. DiVenere, and J. B. Ketterson: "Coherent phonons in mixed semimetalls and semimetal superlatioes"Physica B. 263 & 264. 67-69

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K. Mizoguchi, M. Hase, S. Nakashima and M. Nakayama: "Study of coherent folded acoustic phonons by pump-probe technique"International Workshop on Current Topics of Laser Technology. 39 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] M. Hase, K. Mizoguchi, S. Nakashima and K. Sakai: "Generation of coherent THz phononsin Bi-Sbmixed crystals"International Workshop on Current Topics of Laser Technology. 37 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K Kisoda, M. Hase, H. Harima, S. Nakashima, K. Sakai, M. Tani, H. Negishi, and M. Inoue: "Coherent phonons from quasi-two-dimensional conductor \-MoィイD24ィエD2OィイD211ィエD2"in International Workshop on Current Topics of Laser Technology Kobe. 76 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] O. V. Misochko, M. Tani, K. Sakai, K. Kisoda, and S. Nakashima: "Coherent phonons in VィイD22ィエD2OィイD23ィエD2 and below the Mott transition"in International Workshop on Current Topics of Laser Technology Kobe. 78 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] "Coherent Phonons in Condensed Matter": "Sin-ichi Nakashima, Muneaki Hase, Kohji Mizoguchi and Hiroshi Harima"Surface Science. Vol. 19, No. 2. 2-9 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] "Behavior of Coherent Phonons in Femtosecond Region": "Sin-ichi Nakashima, Muneaki Hase, and Kohji Mizoguchi"Butsuri. Vol. 53, No. 8. 607-611 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 中島信一: "Coherent phonon oscillations in photo-excited semiconductors and semimetals" J.Luminescence. 76/77. 6-14 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 中島信一: "固体におけるコヒーレントフォノン" 表面科学. 19・2. 64-71 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 中島信一: "フェムト秒領域のコヒーレントフォノンの振る舞い" 日本物理学会誌. 53・8. 607-611 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 溝口幸司: "Resonance effect of coherent folded acoustic phonons generated by ultrashort light pulses in GaAs/AlAs superlattices" Physica B. 249-251. 887-890 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 中島信一: "Selective enhancement of coherent optical phonons using THz-rate pulse train" Jpn.J.Appl.Phys.37. L281-L283 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 溝口幸司: "Dynamics of coherent phonons in bismuth generated by ultrashort laser pulses" Phys.Rev.B. 58・9. 5448-5452 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 木曽田賢治: "Optical study of the Mott transition in V203:comparison of time-and frequency-domain results" Phys.Rev.B. 58・19. 12789-12794 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 中島信一: "Dynamics of coherent plasmon-phonon coupled modes in GaAs using ultrashort laser pulses" J.Luminescence. 76/77. 68-71 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 木曽田賢治: "Coherent phonons from the CDW state in η-Mo4O11" Phys.Rev.B. 58・12. R7484-R7487 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 中島信一: "固体におけるコヒーレントフォノン" 表面科学. 19・2. 64-71 (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] 溝口幸司: "Observation of coherent acoustic phonons in Fibonacchi superlattice" Physical Review B. 55・15. 9336-9339 (1997)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2020-05-15  

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