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DYNAMICS OF LATTICE STRAIN FIELD NEAR PHASE TRANSITION

Research Project

Project/Area Number 09440133
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTHE UNIVERSITY OF TOKYO

Principal Investigator

KAKURAI Kazuhisa  THE UNIV. OF TOKYO, ISSP, PROF., 物性研究所, 教授 (00204339)

Co-Investigator(Kenkyū-buntansha) NISHI Masakazu  THE UNIV. OF TOKYO, ISSP, RESEARCH ASSOCIATE, 物性研究所, 助手 (90156034)
NAKAJIMA Kenji  THE UNIV. OF TOKYO, ISSP, RESEARCH ASSOCIATE, 物性研究所, 助手 (10272535)
FUJII Yasuhiko  THE UNIV. OF TOKYO, ISSP, PROF., 物性研究所, 教授 (00013524)
ASO Naofumi  THE UNIV. OF TOKYO, ISSP, RESEARCH ASSOCIATE, 物性研究所, 助手 (40313118)
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥10,000,000 (Direct Cost: ¥10,000,000)
Fiscal Year 1999: ¥1,800,000 (Direct Cost: ¥1,800,000)
Fiscal Year 1998: ¥4,100,000 (Direct Cost: ¥4,100,000)
Fiscal Year 1997: ¥4,100,000 (Direct Cost: ¥4,100,000)
KeywordsNEUTRON SCATTERING / SPIN ECHO SPECTROSCOPY / PHASE TRANSITION / 中性子錯乱
Research Abstract

The aim of this project is the development of the thermal neutron spin echo spectroscopy for the detailed study of lattice dynamics near phase transition.
1. For this purpose the newly developed thermal neutron spin echo option on ISSP-PONTA spectrometer has been improved.
(1) Spin echo test experiment using neutron wave length λ=1.609Å has been performed. The use of this wave length pushes the lower limit of the dynamical time range down to 7 picosec, thus covering the dynamical range of 7 to 155 picosec by using both 1.609Å and 2.35Å wave length neutrons.
(2) Spin echo experiment at large Q=2.9ÅィイD1-1ィエD1 has been successfully performed.
(3) Pairs of gradient coils have been designed constructed and tested. These coils create additional neutron spin precession field integral component depending on the neutron flight paths within the divergence of the neutron beam and allow to match the slope of the spin echo line to the slope of the excitation dispersion to be studied (spin echo focussin … More g).
2. Spin echo experiment at finite energy transfer and especially the use of above mentioned gradient coils demand the introduction of spin echo simulation program to plan and analyse the experiments.
(1) Spin echo simulation program has been developed and is being tested.
(2) The phonon line width measurement in SrTiO3 has been analysed using the simulation program.
3. Few quasielastic thermal neutron spin echo experiments have been performed.
(1) Slow spin dynamics in 2-D, triangular lattice system CuFeィイD20.95ィエD2AlィイD20.05ィエD2OィイD22ィエD2 has been studied, showing the static nature of the moment at low T in the time scale of 140 picosec.
(2) Larmor spin precession phase shift near the magnetic satellite peak of Ho in transmission geometry has been observed for the first time.
(3) Slow dynamics in Polybutadiene towards its glass transition at large Q=2.9ÅィイD1-1ィエD1 has been studied for the first time. The T-dependence of the dynamics at this large Q is found to be different than that of small Q sofar studied.
4. Possible candidates to study the lattice distortions near phase transition with spin echo spectroscopy have been studied, especially the spin and lattice dynamics in the spin-Peierls system CuGeOィイD23ィエD2 and the charge ordering system NaVィイD22ィエD2OィイD25ィエD2 have been studied. Less

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (43 results)

All Other

All Publications (43 results)

  • [Publications] Zeyen, C.M.E. et al.: "Thermal neutron spin echo three-axis spectrometer with μeV resolution"Neutron News. 8. 7-10 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Fujii Y. et al.: "New Inorganic Spin-Peierls Compound NaV_2O_5 Evidenced by X-ray and Neutron Scattering"J. Phys. Soc. Japan. 66. 326-329 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kakurai K.: "Thermal Neutron Spin Echo Option on PONTA"Neutron Network News. 7-3. 23-28 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nishi M. et al.: "Magnetic Excitations of GuGeO_3 under Applied Pressure"Physica B. 241-243. 537-539 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yoshihama T. et al.: "Magnetic Excitations in Spin-Peierls Compound NaV_2O_5"Physica B. 241-243. 543-545 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. kakurai and Y. Morii: "Neutron Scattering Activities at JRR-3M"Neutron News. 9. 15-22 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Achiwa N. et al.: "Larmor precession of neutron spin through helical magnetic crystal of holmium"Physica B. 241-243. 1204-1206 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yoshihama T. et al.: "Spin Dynamics in NaV_2O_5 - Inelastic Neutron scattering -"J. Phys. Soc. Jpn.. 67. 744-747 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nishi M. et al.: "New aspects of the b^*-LA phonon of CuGeO_3"J. Phys. Chem. Solods. 60. 1109-1112 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Zeyen C.M.E.: "Spin echo three-axis spectrometers for improved energy and momentum resolution"Phys. Chem. Solids. 60. 1573-1578 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nakao H. et al.: "Critical behaviour of crystal lattice of NaV_2O_5"J. Phys. Chem. Solids. 60. 1101-1104 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yosihama T. et al.: "Magnetic inelastic neutron scattering study of NaV_2O_5"J. Phys. Chem. Solids. 60. 1099-1100 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Achiwa N. et al.: "Observation of dynamical diffraction phase due to neutron spin precession through a ferromagnetic crystal of permalloy"J. Phys. Chem. Solids. 60. 1611-1614 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Oohara Y. et al.: "Neutron diffraction study of magnetic ordering in CuFe_<0.95>Al_<0.05>O_2"J. Phys. Soc. Japan. (in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Zeyen, C.M.E. et al.: "Thermal neutron spin echo three-axis spectrometer with μeV resolution"Neutron News. 8. 7-10 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Fujii, Y. et al.: "New Inorganic Spin-Peierls Compound NaVィイD22ィエD2OィイD25ィエD2 Evidenced by X-ray and Neutron Scattering"J. Phys. Soc. Japan. 66. 326-329 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kakurai, K.: "Thermal Neutron Spin Echo Option on PONTA"Neutron Network News. Vol.7, No.3(in Japanese). 23-28 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nishi M. et al.: "Magnetic Excitations of CuGeOィイD23ィエD2 under Applied Pressure"Physica B. 241-243. 537-539 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yosihama, T. et al.: "Magnetic Excitations in Spin-Peierls Compound NaVィイD22ィエD2OィイD25ィエD2"Physica B. 241-243. 543-545 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Kakurai and Y. Morii: "Neutron Scattering Activities at JPR-3M"Neutron News. 9. 15-22 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Achiwa, N. et al.: "Larmor precession of neutron spin through helical magnetic crystal of holmium"Physica B. 241-243. 1204-1206 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yosihama, T. et al.: "Spin Dynamics in NaVィイD22ィエD2OィイD25ィエD2 - Inelastic Neutron Scattering -"J. Phys. Soc. Jpn.. 67. 744-747 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nishi, M. et al.: "New aspects of the bィイD1*ィエD1-LA phonon of CuGeOィイD23ィエD2"J. Phys. Chem. Solids. 60. 1109-1112 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Zeyen, C.M.E.: "Spin echo three-axis spectrometers for improved energy and momentum resolution"J. Phys. Chem. Solids. 60. 1573-1578 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nakao, H. et al.: "Critical behaviour of crystal lattice of NaVィイD22ィエD2OィイD25ィエD2"J. Phys. Chem. Solids. 60. 1101-1104 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Yosihama, T. et al.: "Magnetic inelastic neutron scattering study of NaVィイD22ィエD2OィイD25ィエD2"J. Phys. Chem. Solids. 60. 1099-1100 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Achiwa, N. et al.: "Observation of dynamical diffraction phase due to neutron spin precession through a ferromagnetic crystal of permalloy"J. Phys. Chem. Solids. 60. 1611-1614 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Oohara, Y. et al.: "Neutron diffraction study of magnetic ordering in CuFeィイD20.95ィエD2AlィイD20.05ィエD2OィイD22ィエD2"J. Phys. Soc. Japan. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Nishi, M. et al.: "New aspects of the b^*-LA phonon of Cube O_3"J. Phys. Chem. Solids. 60. 1109-1112 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Zeyen, C. M. E.: "Spin echo three-axis spectrometers for improved energy and momentum resolution"J. Phys. Chem. Solids. 60. 1573-1578 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Nakao, H. et al.: "Critical behavior of crystal lattice of NaV_2O_5"J. Phys. Chem. Solids. 60. 1101-1104 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Yoshihama, T. et al.: "Magnetic inelastic neutron scattering study of NaV_2O_5"J. Phys. Chem. Solids. 60. 1099-1100 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Achiwa, N. et al.: "Observation of dynamical diffraction on phase due to neuron precession through a ferromagnetic crystal of pormalloy"J. Phys. Chem. Solids. 60. 1611-1614 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Oohara, Y. et al.: "Neutron diffraction study of magntic ordering in CuFe_<0.95>Al_<0.05>O_2"J. Phys. Chem. Japan. (発表予定).

    • Related Report
      1999 Annual Research Report
  • [Publications] Kakurai,K.: "Thermal Nentron Spin Echo Option on PONTA" Neutron Network News. 7・3. 23-28 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] Nishi,M.et al.: "Magnetic Excitations of GuGeO_3 under Applied Pressure" Physica B. 241-243. 537-539 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Yosihama,T.et al.: "Magnetic Excitations in Sgin-Peierls Compound NaV_2O_5" Physica B. 241-243. 543-545 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Kakurai,K.& Morii,Y.: "Neutron Scattering Activities at JRR-3M" Neutron News. 9. 15-22 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Achiwa,N.et al.: "Larmor precession of neutron spin through helical magnetic cryoralof nolnium" Physica B. 241-243. 1204-1206 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Yosihama,T.et al.: "Spin Dynamics in NaV_2O_5-Inclastic Neutron Scattering" J.Phys.Soc.Japan. 67・3. 744-747 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Zeyen PHE et al.: "Thermal neutron spin echo 3-axis spectrometon with MeV resolution" Neutron News. 8. 7-10 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Fujii,Y.et al.: "New Inorganic Spin-Beierls Compound NaV_2O_5 Evidenced by X-ray and Neutron Scattering" J-Phys.Soc.Japan. 66. 326-329 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Nishi M.et al.: "Magnetic Excitation of Cube O_3 under Applied Pressure" Physica B. (発表予定).

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2020-05-15  

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