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RESEARCH ON SPIN QUANTUM FLUCTUATION AND ORDERING PROCESS OF ITINERANT HEAVY FERMION

Research Project

Project/Area Number 09440137
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionOsaka University

Principal Investigator

MIYAKO Yoshihito,  Graduate School of Science, Osaka University, Professor, 大学院・理学研究科, 教授 (10000837)

Co-Investigator(Kenkyū-buntansha) TAKEUCHI Tetsuya  Low Temperature Center, Osaka University, Assistant, 低温センター, 助手 (90260629)
TANIGUCHI Toshifumi  Graduate School of Science, Osaka University, Assistant, 大学院・理学研究科, 助手 (80207183)
AKAI Hisazumi  Graduate School of Science, Osaka University, Professor, 大学院・理学研究科, 教授 (70124873)
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥13,100,000 (Direct Cost: ¥13,100,000)
Fiscal Year 1999: ¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 1998: ¥1,900,000 (Direct Cost: ¥1,900,000)
Fiscal Year 1997: ¥9,000,000 (Direct Cost: ¥9,000,000)
KeywordsHeavy Fermion / SDW / Quantum Phase Transition / Spin Quantum Fluctuation / 量子揺らぎ / Ce(Ru_4-_xRh_x)_2Si_2 / UR_<U2>Si_2 / Ce(Ru_<1-X>Rh_X)_2Si_2 / URu_2Si_2 / 非フェルミ液体 / スピン密度波 / Heavy Fermion / SDW / Antiferromagnetism / Quantum Phase Transition / Resistivity / Non-Fermi Liquid / Specific heat / μSR
Research Abstract

In Ce(RuィイD21-xィエD2RhィイD2xィエD2)ィイD22ィエD2SiィイD22ィエD2 compound, x-dependence of the material is investigated in detail. In Ru rich side, the ground state is Fermi liquid for x < 0.03 and an anisotropic spin density wave (SDW) appears in 0.03 < x < 0.4 with maximum TィイD2NィエD2 = 5.5 K at x = 0.15. The nature of the anisotropic SDW is characterized by the anisotropic anomaly in the resistivity below TィイD2NィエD2. The anisotropy of the SDW is discussed from the view point of nesting of the Fermi surfaces of itinerant heavy fermion quasi-particle bands. Another interesting nature is non-Fermi liquid behavior observed for x = 0.4 and 0.5. Appearance of quantum Griffiths's like phase is indicated for x = 0.5 form the measurements of μ SR, ac susceptibility and nonlinear susceptibility. The temperature dependence of the susceptibility and the magnetoresistance with 0.1 T dc field are well explained in terms of the mean field theory based on spin fluctuations. The phase transition of URuィイD22ィエD2 at 17.5K(=TィイD20ィエD2) is considered to be due to quadrupolar ordering from the behaviors of sharp anomaly in nonlinear susceptibility at TィイD20ィエD2 and very large consumption of entropy below TィイD20ィエD2 compared to small staggered ordered moment ,0.02μ(B). We recently found that the phase transition is not due to magnetic origin by the neutron scattering experiment under pressure. The susceptibility and magnetization in dilute alloys of UィイD2XィエD2LAィイD21-XィエD2RuィイD22ィエD2SiィイD22ィエD2 are well explained by assuming non-Kramers doublet ground state of the J = 4 crystalline field level. From these experiments, the phase transition of URuィイD22ィエD2SiィイD22ィエD2 at TィイD20ィエD2 is understood by the model of quadrupolar ordering of non-Kramers doublet which coexists with antiferromagntic short range order.

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (27 results)

All Other

All Publications (27 results)

  • [Publications] T. Takeuchi, et al.: "Magnetoelastic Coupling in U_2Rh_3Sl_5 Studied by Thermal Expression and Magnetrostriction"J. Phys. Soc. Joc.. 68. 1086-1089 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Yamamoto, et al.: "Low temperature properties of the heavy-termion Ce(Rul-Rh-x)_2Si_2 at the magnetic nonmagnetic boundaries"Physica B. 259-261. 66-67 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J. Souletie, et al: "Scaling analysis of the susceptibility of Ce(Rul-_xPh_x)2Si2 in the Fermi and non-Fermi liquid ranges"Physica B. 259-261. 372-373 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka, et al: "Effect of Pressure on Tiny Antireromagnetic Moment in the Heavy-Electron Compound Uru2Si2"Phys. Rev. Lett.. 83. 5114-5117 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Takeuchi, et al.: "Low temperature Specific heat of UniSi2"J. Magn. Magn. Matter. 177-181. 55-56 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Takeuchi. et al: "Magnetoelasic Coupling in UィイD22ィエD2RhィイD21ィエD2SiィイD25ィエD2 Studied by Thermal Expension Magnetostriction."J. Phys. Soc. Jpn. No.68. 1086-1089 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Yamamoto. et. al: "Lowtemperature properties of the heavy-termion Ce(RuィイD21ィエD2-RhィイD2xィエD2)ィイD22ィエD2SiィイD22ィエD2 at the magneticnon magnetic boundries."Physica B. No.259-261. 66-67 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J. Souletie. al: "Scaling analysis of the susceptibilty of Ce(RuィイD21ィエD2-xRhィイD22ィエD2)ィイD22ィエD2SiィイD22ィエD2 in the Fermi and non-Fermi liquid ranges."Physica B. No.259-261. 372-373 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka. et. al: "Effect of pressure on Tiny Antirerromagnetic Moment in the Heavy. Effection Compound URuィイD22ィエD2SiィイD22ィエD2"Phys. Rev. Leff. No.83. 5114-5117 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Taniguchi et. al: "Low temperture Specitic heat of UNiSiィイD22ィエD2"J. Magn. Magn. Matter. No.177-181. 55-56 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T.Takeuchi et, al.: "Magnetoelastic Coupling in U2Rh3Si5 Studied by Thermal Expansion and Magnetostriction"J.Phys.Soc.Jpn.. 68. 1086-1039 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Yamamoto et, al.: "Low temperature properties or the heavy-termion Ce(Rul-Rhx)2Si2 at the magneticnonmagnetic boundaries"Physica B. 259-261. 66-67 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] J.Souletie al.: "Scaling analysis of the susceptibility of Ce(Rul-xRhx)2Si2 in the Fermi and non-Fermi liquid ranges"Physica B. 259-261. 372-373 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Amitsuka et, al.: "Effect of Pressure on Tiny Antirerromagnetic Moment in the Heavy-Electron Compound URu2Si2"Phys.Rev.Lett.. 83. 5114-5117 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Taniguchi et al.: "Low temperature specific heat of UNiSi2"J.Magn.Magn.Mater.. 177-181. 55-56 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Taniguchi et al.: "Low temperature specific heat of UNiSi2" J.Magn.Magn.Mater.177-181. 55-56 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Marumoto et al.: "Crystal field splitting of praseodymium in the dilute system(Pr_XLa_<1-X>)Ru_2Si_2," J.Magn.Magn.Mater.177-181. 353-354 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] G.Dumpichet al.: "Resistance and magnetic behavior of Ce_<1-X>Al_X thin films at low temperature" J.Magn.Magn.Mater.177-181. 377-378 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Taniguchi et al.: "Non-Fermi liquid like behavior in Ce(Ru_<1-X>Rh_X)_2Si_2 (0.3<X<0.5)" J.Magn.Magn.Mater.177-181. 419-420 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Takeuchi et al.: "In plane magnetic anisotropy in ErRu_2Si_2" J.Magn.Magn.Mater.177-181. 1081-1082 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Tabata et al.: "Spin Fluctuation and Magnetic Phase Transition in Itinerant Heavy Electron System Ce(Ru_<1-X>Rh_X)_2Si_2 (X=0,0.03,and 0.05)" J.Phys.Soc.Jpn,. 67. 2484-2487 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Miyako, T.Takeuchi, S.Kawarazaki, M.Acet, et.al.: "INVAR like behavior of heavy electrons in Ce (Ru_<0.85>Rh_<0.15>)_2Si_2," Physica B. 230-232. 1014-1016 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Miyako, T.Taniguchi, Y.Tabata, H.Tanabe, et.al.: "Low temperature specific heat of Ce (Ru_<1-x>Ru_X)_2Si_2 and (Ce_<1-X>La_X)Ru_2Si_2," Physica B. 230-232. 123-125 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Miyako, S.Kawasaki, T.Taniguchi, T.Takeuchi, et al.: "Spin density wave and heavy electrons in Ce (Ru_<1-x>Ru_X)_2Si_2 and Ce_<1-X>La_XRu_2Si_2" Physica B. 230-232. 1011-1013 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Miyako, S.Kawarazaki, M.Sato, H.Kadowaki, et.al.: "Long range magnetic order on the Kondo lattice-SDW in Ce (Ru_<1-X>Rh_X)_2Si_2 as satudied by neutron diffraction" J.Phys.Soc.Jpn. (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Miyako, T.Takeuchi, et.al.: "Coupled Spin-Lattice Transition in U2RhSi5 : Thermal Expansion and Magnetization," Phys.Rev.B. (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Miyako, T.Taniguchi, et.al.: "Low temperature specific heat of UNiSi_2" Physica B. 230-232. 123-125 (1997)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2020-05-15  

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