| Project/Area Number |
09440149
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| Research Category |
Grant-in-Aid for Scientific Research (B)
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| Allocation Type | Single-year Grants |
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| Section | 一般 |
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| Research Field |
物理学一般
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| Research Institution | University of Tsukuba |
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Principal Investigator |
NAKATSUKA Hiroki University of Tsukuba, Institute of Applied Physics, Professor, 物理工学系, 教授 (10111915)
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| Co-Investigator(Kenkyū-buntansha) |
KONDO Kiminori University of Tsukuba, TARA Center, Lecturer, TARAセンター, 講師 (80225614)
HATTORI Toshiaki University of Tsukuba, Institute of Applied Physics, Lecturer, 物理工学系, 講師 (60202256)
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| Project Period (FY) |
1997 – 1998
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| Project Status |
Completed (Fiscal Year 1998)
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| Budget Amount *help |
¥2,500,000 (Direct Cost: ¥2,500,000)
Fiscal Year 1998: ¥2,500,000 (Direct Cost: ¥2,500,000)
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| Keywords | femtosecond pulse / ultrfast optical nonlinear phenomenon / Mychelson inteferometer / pump-probe spectroscopy / photon echo / nonlinear propagation of light / dve solution / accumulated photon echo / 非線形光パルス伝搬 / 非線形光学 / 自己相関関数 / 相互相関関数 / フーリエ分光 / 自由誘導減衰 |
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| Research Abstract |
At first linear propagation of light was investigated with a white-light Michelson interferometer. This method gives the full information on the deformation of ultra-short fight pulses by the passage through samples in the linear regime. We observed the delay of pulse propagation for cobalt chloride in pyridine, free-induction decay signal for oxazine-1 in methanol, and the increase of peak velocity for nigrosine in water. By Fourier analysis of the interferograms, complex optical constants of the samples were also obtained.
Next the excitation light source was changed from incoherent white light to a coherent ultra-short mode-locked laser. Then the interferometric method by using a Michelson type interferometer was applied to observe the waveform of the accumulared photon echoes in a dye-doped polymer film. By the Fourier analysis of the measured interferograms we obtained detailed shapes of the burned population grating and phase grating in the sample. From the frequency distribution of the dye molecules which are efficient for persistent spectral hole burning, we obtained the inhomogeneous frequency distribution of 0-0 transition from S_0 to S_1 levels of the dye molecules in the polymer film.
Finally we applied the interferometric method to pump-probe spectroscopy. Here the waveform of the probe pulse was measured including the information of the phase of light. The sample was a dye jet. We observed a large peak shift and a phase shift induced by the pump pulse. The deformation of the probe pulse was precisely reproduced by a calculation which combines Bloch equation for dye molecules and Maxwell equation for light wave.
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