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Study on Isotope Enrichment of Nitrogen-15 with Cascading Assembly of Thermal Diffusion Columns

Research Project

Project/Area Number 09480098
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field エネルギー学一般・原子力学
Research InstitutionNagoya University

Principal Investigator

YAMAMOTO Ichiro  Nagoya University, School of Engineering, Professor, 工学研究科, 教授 (50023320)

Co-Investigator(Kenkyū-buntansha) KOBAYASHI Noboru  Nagoya University, School of Engineering, Research Associate, 工学研究科, 助手 (70293652)
ENOKIDA Youichi  Nagoya University, School of Engineering, Associate Professor, 工学研究科, 助教授 (40168795)
Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥11,900,000 (Direct Cost: ¥11,900,000)
Fiscal Year 1999: ¥2,100,000 (Direct Cost: ¥2,100,000)
Fiscal Year 1998: ¥3,600,000 (Direct Cost: ¥3,600,000)
Fiscal Year 1997: ¥6,200,000 (Direct Cost: ¥6,200,000)
KeywordsIsotope Separation / Thermal Diffusion / Thermal Diffusion Column / Cryogenic / Nitrogen Isotopes / Nitrogen-15 / Computer Simulation / Numerical Analysis
Research Abstract

A numerical simulation system was developed to analyze isotope separation performance in the thermal diffusion column for nitrogen isotope separation. Hydrodynamic flow in the thermal diffusion column was numerically simulated and mole fractions of nitrogen molecules of mass numbers, 28, 29 and 30 were computed as function of vertical and radical positions by solving a convective diffusion equation. The thermal diffusion factor, which is most important value in the analysis, was expressed in a practical form, still keeping consistent relationship with generalized Stefan-Maxwell equation, applicable to multi-component mixture of nitrogen isotopes. In our study, the effect of inelastic collision of nitrogen molecules was considered to the thermal diffusion factor. The effect of cold wall temperature on separation performance for ィイD114ィエD1N-ィイD115ィエD1N and ィイD114ィエD1NィイD22ィエD2 separation was evaluated with the numerical simulation system and compared with experimental results with the thermal diffusion column of an effective height of 950mm, a hot wire of 0.15mm in radius and a cold wall of 5.0mm in radius. The solutions numerical analyses gave good reproduction of dependence of separation factors on cut and cold wall temperature.
Studied as a design example was cascade composed with an assembly of thermal diffusion columns of an effective height of 10m. The number required for a series of stages of the thermal diffusion column was 5 so as to achieve the final enrichment of 99.9% of ィイD115ィエD1N. The total number of the thermal diffusion columns was evaluated 89,600 in a plant which produces ィイD115ィエD1N to meet the demand for UN fuel of one fast breeder reactor of 1 GW electric power in a year.

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (14 results)

All Other

All Publications (14 results)

  • [Publications] N. Kobayashi: "Isotopic Approximation to Thermal Diffusion Coefficient in Multi-domponent Mixture"Journal of Nuclear Science and Technology. 34. 394-397 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamakawa: "Inverse Power Series Fittings of Temperature Dependence of Thermal Diffusion Factors between Two Components of Hydrogen Isotope Molecules"Journal of Nuclear Science and Technology. 35. 234-239 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamakawa: "Effect of Gravity and Inter-molecular Performances of "Cryogenic-wall" Thermal Diffusion Column"Fusion Engineering and Design. 39/40. 1015-1020 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamakawa: "Thermal Diffusion Factor for Diatomic Gas Mixture in Multicomponent System"Journal of Nuclear Science and Technology. 37(印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] N. Kobayashi et al.: "Isotopic Approximation to Thermal Diffusion Coefficient in Multi-component Mixture"Journal of Nuclear Science and Technology. 34. 394-397 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamanaka et al.: "Inverse Power Series Fittings of Temperature Dependence of Thermal Diffusion Factors between Two Components of Hydrogen Isotope Molecules"Journal of Nuclear Science and Technology. 35. 234-239 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamanaka et al.: "Effect of Gravity and Inter-molecular Forces on Separation Performances of "Cryogenic-wall" Thermal Diffusion Column"Fusion Engineering and Design. 39/40. 1015-1020 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yamanaka et al.: "Thermal Diffusion Factor for Diatomic Gas Mixture in Multicomponent System"Journal of Nuclear Science and Technology. 2000 (in press). (37)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Yamakawa: "Thermal Diffusion Factor for Diatomic Gas Mixture in Multicomponent System"Journal of Nuclear Science and Technology. 37(印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Yamakawa: "Inverse Power Series Fittings of Temperature Dependence of Thermal Diffusion Fac-tors between Two Components of Hydrogen Isotope Molecules" Journal of Nuclear Science and Technology. 35. 234-239 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Yamakawa: "Effect of Gravity and Inter-molecular Performances of “Cryogenic-wall" Thermal Dif-fusion Column" Fusion Engineering and Design. 39/40. 1015-1020 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] N. Kobayashi: "Isotopic Approximation to Thermal Diff usion Coefficient in Multi-component Mixture" Journal of Nuclear Science and Technology. 34. 394-397 (1997)

    • Related Report
      1997 Annual Research Report
  • [Publications] H. Yamakawa: "Inverse Power Series Fittings of Temperature Dependence of Thermal Diff usion Factors between Two Components of Hydrogen Isotope Molecules" Journal of Nuclear Science and Technology. 35(in press). (1998)

    • Related Report
      1997 Annual Research Report
  • [Publications] H. Yamakawa: "Effect of Gravity and Inter-molecular Performances of "Cryogenic-wall"Thermal Diffusion Column" Fusion Engineering and Design. (in press). (1998)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2016-04-21  

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