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Study on dry deposition of sulfur dioxide to the Chinese desert soil and estimation of its dry removal from the atomosphere

Research Project

Project/Area Number 09480114
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionSaitama University

Principal Investigator

SAKAMOTO Kazuhiko  Department of Environmental Science and Human Engineering, Graduate School of Science and Engineering, Saitama University, Professor, 大学院・理工学研究科, 教授 (20111411)

Co-Investigator(Kenkyū-buntansha) ISHIHARA Hidekazu  Department of Applied Chemistry, Faculty of Engineering, Saitama University, Res, 工学部, 助手 (20261878)
Project Period (FY) 1997 – 1998
Project Status Completed (Fiscal Year 1998)
Budget Amount *help
¥7,900,000 (Direct Cost: ¥7,900,000)
Fiscal Year 1998: ¥3,200,000 (Direct Cost: ¥3,200,000)
Fiscal Year 1997: ¥4,700,000 (Direct Cost: ¥4,700,000)
Keywordsdesert soil / Yellow sand particles / sulfur dioxide / dry deposition / deposition velocity / basicity / relative humidity / photoirradiation / 中国砂漠土壌 / ニ酸化硫黄 / 不均一反応 / 光触媒 / 人工肺 / 濃瓊測定法 / 酸性ガス
Research Abstract

In order to obtain the fundamental data to estimate the removal amount of SO_2 from the atmosphere by its dry deposition on the Chinese desert and yellow sand soils, we investigated the exposure of the above soils and several model soils to the experimental gases containing trace level of SO_2, NO_2, or HNO_3. The results obtained by the above exposure experiments etc, were summarized as below.
1) Elemental analyses for desert yellow sand soils in China were achieved. The results indicated the intimate relation of acidity of soil particles with content of Ca. It suggests the relation of soil acidity with the frequency of acid rain appearence.
2) Dry deposition velocity of SO_2 to desert and yellow sand soils in China depended on soil alkalinity and humidity of exposure gas.
3) Dry deposition velocity of HNO_3 to various soils was similar level of that of SO_2. While, that of NO_2 was much lower than that of SO_2.
4) S(VI)/S(IV) deposited on desert, yellow sand, and model soils was increased with increase in the humidity of exposure gas and the irradiation time with a simulated sun-light (black-light).
5) The artificial lung was applied to collection of low concentration SO_2 and gaseous HNO_3.
6) In order to estimate the removal amount of SO_2 from the atmosphere by its dry deposition on the Chinese desert and yellow sand soils, further investigation is needed.

Report

(3 results)
  • 1998 Annual Research Report   Final Research Report Summary
  • 1997 Annual Research Report
  • Research Products

    (30 results)

All Other

All Publications (30 results)

  • [Publications] 王偉,: "中国福建省南部における大気エアロゾルの汚染特徴および酸性雨への寄与," 大気環境学会誌. 32. 204-215 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 王偉,: "中国における大気エアロゾル酸性度と酸性化に関する緩衝能力" エアロゾル研究. 12. 92-102 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 坂本和彦: "DNA中和器内でのSO_2粒子化に与えるO_3の影響" エアロゾル研究. 12. 130-134 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 高世東: "中国重慶市における大気硫黄化合物の乾性沈着について" エアロゾル研究. 13. 44-50 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 高世東: "中国重慶市における森林の林内雨に対する酸性沈着の影響" 大気環境学会誌. 34. 53-64 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 薫旭輝: "中国土壌中のCa, Mgの分布特徴およびその大気中酸性物質との関係" エアロゾル研究. 14(印刷中). (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] Kazuhiko Sakamoto: "Study on dry deposition of SO_2 to Chinese desert soils" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. 印刷中. (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] Hidekazu Ishihara: "Laboratory study on deposition and oxidation to sulfate of SO_2 by use of model soil, CaCO_3" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. 印刷中. (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] W.Wang, K.Sakamoto, W.Wang, D.Tang, J.Du, and J.Gao: "Pollution charateristics of atmospheric aerosol and its relations to acid rain at the southern area of Fujian province in china(in Japanese)" J.Jpn.Soc.Atmos.Environ.32. 2094-215 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] W.Wang, K.Sakamoto, W.Wang, D.Tang, and J.Du: "Acidity and buffering ability to precipitation acidification of atmospheric aerosols collected in China(in Japanese)" J.Aerosol Research Jpn.12. 92-102 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Sakamoto and T.Arai: "Effect of O_3 on particle formation from SO_2 in DMA's neutalizer(in Japanese)" J.Aerosol Research Jpn.12. 130-134 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S.Gao, K.Sakamoto, D.Zhao, and D.Zhang: "An estimate of dry deposition for atmospheric sulfur over Chongqing in China(in Japanese)" J.Aerosol Research Jpn.13. 44-50 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] S.Gao, K.Sakamoto, Y.Xu, D.Zhao, and D.Zhang, and X.Zhou: "The effect of acid precipitation on the throughfall of the forest canopies in Chongqing, China(in Japanese)" J.Jpn.Soc.Atmos.Environ.34. 53-64 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] X.Dong, K.Sakamoto, C.Zheng, H.Quan, Y.Cheng, and W.Wang: "Characteristics of Ca, Mg distribution in soil of China and their relationship to acidic pollutants in the atmosphere(in Japanese)" J.Aerosol Research Jpn.(in contribution).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Sakamoto, K.Mogi, and O.Ishitani: "Study on dry deposition of SO_2 to Chinese desert soils" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. (in press). (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] H.Ishihara, H.Nakano, T.Kambayashi, M.Ohi, I.Iwamoto, and K.Sakamoto: "Laboratory study on deposition and oxidation to sulfate of SO_3 by use of model soil, CaCO_3" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. (in press). (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] X.Dong, K.Sakamoto, H.Quan, and C.Zheng: "Study on pH of soils and its distribution in China(in Japanese)" Environ.Sci.(in contribution).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] X.Dong, K.Sakamoto, W.Wang, H.Liu, C.Zheng, S.Niu and Y.Cheng: "Chemical Composition and acidic buffering ability for size-segregated atmospheric aerosol in the desert area of China(in Japanese)" J.Aerosol Research Jpn.(in contribution).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 王偉,: "中国福建省南部における大気エアロゾルの汚染特徴および酸性雨への寄与," 大気環境学会誌. 32. 204-215 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 王偉: "中国における大気エアロゾル酸性度と酸性化に関する緩衝能力" エアロゾル研究. 12. 92-102 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 坂本和彦: "DMA中和器内でのSO_2粒子化に与えるO_3の影響" エアロゾル研究. 12. 130-134 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 高世東: "中国重慶市における大気硫黄化合物の乾性沈着について" エアロゾル研究. 13. 44-50 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 高世東: "中国重慶における森林の林内雨に対する酸性沈着の影響" 大気環境学会誌. 34. 53-64 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] 薫旭輝: "中国土壌中のCa,Mgの分布特徴およびその大気中酸性物質との関係" エアロゾル研究. 14(印刷中). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] Kazuhiko Sakamoto: "Study on dry deposition of SO_2 to Chinese desert soils" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. (印刷中). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] Hidekazu Ishihara: "Laboratory study on deposition and oxidation to sulfate of SO_2 by use of model soil,CaCO_3" Proceedings of 6th International Conference on Atmospheric Sciences and Applications to Air Quality. (印刷中). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] 坂本和彦(分担執筆): "身近な地球環境問題-酸性雨を考える-(東アジア地域における酸性雨の現状)" コロナ社 (社)日本化学会・酸性雨問題研究会編, 220(143-158) (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 王偉ら(分担執筆): "中国環境ハンドブック(第2節大気汚染1,煤塵汚染(粉塵とSO_2)ほか)" (株)サイエンスフォーラム 定方正毅ら編, 392(68-81) (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 全浩ら(分担執筆): "中国環境ハンドブック(黄砂の発塵と長距離輸送)" (株)サイエンスフォーラム (定方正毅ら編), 392(94-102) (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] 高世東, 坂本和彦, 他2名: "中国重慶における大気硫黄化合物の乾性沈着について" エアロゾル研究. 13巻1号(印刷中). (1998)

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2016-04-21  

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