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Studies on plutonium in terrigenous air-dust

Research Project

Project/Area Number 09640581
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 地球化学
Research InstitutionKanazawa University

Principal Investigator

NAKANISHI Takashi  Faculty of Science, Kanazawa University Professor, 理学部, 教授 (00019499)

Project Period (FY) 1997 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 1999: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1998: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1997: ¥2,400,000 (Direct Cost: ¥2,400,000)
Keywordsair-dust / terrigenous air-dust / Pu-239, 240 / Fe / Po-210 / Pb-210 / ocean flux / 土壌粒子塵 / Am-241 / Pb-210放射能比 / Pu-239
Research Abstract

For a study to estimate terrigenous air-dust fluxes to oceanic region by using environmental plutonium as a tracer, Pu-239, 240 and Fe were determined in air-dust samples collected in Kanazawa, Japan through the years from 1993 to 1998. The air-dust samples were collected using a five-stages (particle size : <1.1 μm, 1.1〜2.0 μm, 2.0〜3.3 μm, 3.3〜7.0 μm, 7.0 μm<) Andersen-type high-volume air sampler, and catcher plates and backup filter were replaced monthly ; air-dust collected every 1-8 months was analyzed as one batch.
Throughout the above mentioned sampling years and particle sizes, the concentrations of Pu-239, 240 and Fe I n the air-dust samples were in a range from 0.1 to 10 μBq-Pu/mg-dust and from 2 to 30 μg-Fe/mg-dust. The Pu/Fe concentration ratios tend to be high in finer air-dust, suggesting that Pu is adsorbed on the surface of terrigenous air-dust. Through the analyses of Po-210/Pb-210 activity ratios in air-dust samples collected occasionally for a few days using Andersen-type low-volume air sampler, from 9 to 140 days were estimated as the apparent floating time of air-dust (particle size : O.06〜0.13 μm, O.13〜0.22 μm, O.22〜0.33 μm, 0.33〜0.52 μm, 0.52〜0.76 μm, 0.76〜1.3 μm, 1.3〜2.5 μm, 2.5〜3.9 μm, 3.9〜5.7 μm, 5.7〜8.5 μm, 8.5〜12.1 μm).

Report

(4 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • 1997 Annual Research Report
  • Research Products

    (16 results)

All Other

All Publications (16 results)

  • [Publications] Y. Miyamoto: "Interferences in neutron and photon activation analysis"J. Radioanal. Nucl. Chem.. 239(1). 165-175 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. A. Haque: "Host phase of ^<239,240>Pu and ^<241>Am in deep-sea sediment"J. Radioanal. Nucl. Chem.. 239(3). 565-569 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. A. Haque: "Chemical dissolution of total content of fallout plutonium in deep-sea sediment"J. Radioanal. Nucl. Chem.. 241(3). 575-579 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Miyamoto, H. Haba, A. Kajikawa, K. Masumoto, T. Nakanishi, K. Sakamoto: "Interferences in neutron and photon activation analysis"J. Radioanal. Nucl. Chem.. 239(1). 165-175 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. A. Haque, T. Nakanishi: "Host phase of ィイD1239,240ィエD1Pu and ィイD1241ィエD1Am in deep-sea sediment"J. Radioanal. Nucl. Chem.. 239(3). 565-569 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. A. Haque, T. Nakanishi: "Chemical dissolution of total content of fallout plutonium in deep-sea sediment"J. Radioanal. Nucl. Chem.. 241(3). 575-579 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y.Miyamoto, H.Haba, A.Kajikawa K.Masumoto, T.Nakanishi, K.Sakamoto: "Interferences in neutron and photon activation analysis"J.Radioanal.Nucl.Chem.. 239(1). 165-175 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.A.Haque,T.Nakanishi: "Host phase of ^<239,240> Pu and ^<241> Am in deep-sea sediment"J.Radioanal.Nucl.Chem.. 239(3). 565-569 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Nakanishi,H.Fukuda,M.Hirose: "Determination of polonium-210 in phosphoric acid"J.Radioanal.Nucl.Chem.. 240(3). 887-891 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.A.Haque,T.Nakanishi: "Chemical dissolution of total content of fallout plutonium in deep-sea sediment"J.Radional.Nucl.Chem.. 241(3). 575-579 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Miyamoto,A.Kajikawa,J.H.Zaidi,T.Nakanishi,K.Sakamoto: "Minor and trace element determination of food spices and pulses of different origins by NAA and PAA"J.Radioanal.Nucl.Chem.. 243(3). 747-765 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.A.Haque,T.Nakanishi: "Host phase of ^<239,240>Pu and ^<241>Am in deep-sea sediment" J.Radioanal.Nucl.Chem.239(3). 565-569 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Nozaki,M.Yamada,T.Nakanishi,Y.Nagaya,K.Nakamura,K.Shitashima,H.Tsubota: "The distribution of radionuclides and some trace metals in the water columns of the Japan and Bonin trenches" Occanologica Acta. 印刷中.

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Nakanishi,K.Miwa,R.Ohki: "Specific radioactivity of Eu-152 in roof tiles exposed to atomic bomb radiation in Nagasaki" J.Radiat.Res.39. 243-250 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] M.A.Haque, T.Nakanishi: "Host phase of plutonium-239,240 and americium-241 in deep-sea sediment" J.Radioanal.Nucl.Chem.(accepted).

    • Related Report
      1997 Annual Research Report
  • [Publications] Y.Nozaki, M.Yamada, T.Nakanishi, Y.Nagaya, K.Nakamura, K.Shitashima, H.Tsubota: "The distribution of radionuclides and some trace metals in the water columns of the Japan and Bonin trenches" Oceanologica Acta. (accepted).

    • Related Report
      1997 Annual Research Report

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Published: 1997-04-01   Modified: 2016-04-21  

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