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Emission Mossbauer Spectroscopy of ^<237>Np Probe in Uranium Compounds.

Research Project

Project/Area Number 09650060
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied physics, general
Research InstitutionTohoku University

Principal Investigator

ONODERA Hideya  Tohoku Univ., Institute of Materials Research Research Associate, 金属材料研究所, 助手 (50005972)

Co-Investigator(Kenkyū-buntansha) KAMIMURA Takashi  Tohoku Univ., Graduate School of Science Professor, 理学部, 教授 (30005813)
KOBAYASHI Hisao  Tohoku Univ., Graduate School of Science Research Associate, 理学部, 助手 (40250675)
YAMAGUCHI Yasuo  Tohoku Univ., Institute of Materials Research Professor, 金属材料研究所, 教授 (80005917)
Project Period (FY) 1997 – 1998
Project Status Completed (Fiscal Year 1998)
Budget Amount *help
¥3,300,000 (Direct Cost: ¥3,300,000)
Fiscal Year 1998: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 1997: ¥2,400,000 (Direct Cost: ¥2,400,000)
KeywordsMossbauer spectroscopy / Neptunium / Uranium compounds / Strong-correlation system / 強相関電子系物質
Research Abstract

This research project was started in order to investigate the physical properties of uranium compounds with strong-correlated electrons by emission ^<237>Np Mossbauer spectroscopy on the basis of new idea that parent ^<237>U nuclei as probes are introduced in U compounds through ^<238>U(gamma, n) reaction. It is also a purpose to establish the emission ^<237>Np Mossbauer spectroscopy to be general and powerful tool for material researches of actinide compounds and alloys. Therefore, the more specific purpose of this work is to develop and construct a spectrometer with sufficient ability for the emission ^<237>Np Mossbauer spectroscopy. The results are summarized as follows.
1. A liquid-helium cryostat for the emission ^<237>Np Mossbauer spectroscopy was constructed. In the cryostat, a standard ^<237>NpO_2 absorber is maintained at a constant temperature of 78 K.A sample Mossbauer source put on a long stem whose temperature is controlled between 1.5 K and room temperature can be driven by a precise velocity wave form of *100 mm/sec.
2. In the geometry mentioned above, the condition for precise drive of source is surveyed using a absolute velocity calibrator using a laser interferometer which is put in the system in order to observe regularly the precise velocity.
3. From the view point of precise drive and velocity calibration, it was confirmed repeatedly that the whole system satisfies the ability demanded for the emission ^<237>Np Mossbauer spectroscopy through measurements of the popular ^<57>Fe Mossbauer effects and the time spectra of interference fringes. Consequently, the whole spectrometer system with sufficient ability for the emission ^<237>Np Mossbauer spectroscopy was completed by the present research project.

Report

(3 results)
  • 1998 Annual Research Report   Final Research Report Summary
  • 1997 Annual Research Report
  • Research Products

    (4 results)

All Other

All Publications (4 results)

  • [Publications] 小野寺秀也: "Magnetic properties of the single cnptalline Dy_3Ni studied by magnetization measurement and ^<161>Dy Mossbauer specttoscopy." J.Magnetism and Magnetic materials. 170. 201-210 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 小野寺秀也: "^<161>Dy and ^<155>Gd Mossbauer spectroscopy of the RTC_2 internetallics (R=Dy, Gd ; T=Ni, Co)" Sci.Rep.RITU A. 45. 1-10 (1997)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] H.Onodera et al: "Magnetic Properties of the Single Crystalline Dy_3Ni Studied by Magnetization Measurement and ^<161>Dy Mossbauer Spectroscopy." J.Magn.Magn.Mater.170. 201-210 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] H.Onodera et al: "^<161>Dy and ^<155>Gd Mossbauer Spectroscopy of the RTC_2 Intermetallics (R=Dy, Gd ; T=Ni, Co)" Sci.Rep RITU. A45. 1-10 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary

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Published: 1997-04-01   Modified: 2016-04-21  

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