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NMR on Spin Dynamics in Spin Ladder & High-T Superconductor

Research Project

Project/Area Number 10044044
Research Category

Grant-in-Aid for international Scientific Research

Allocation TypeSingle-year Grants
SectionJoint Research
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionHOKKAIDO UNIVERSITY

Principal Investigator

KUMAGAI Ken-ichi  Hokkaido University, Graduate School of Science, Professor, 大学院・理学研究科, 教授 (70029560)

Co-Investigator(Kenkyū-buntansha) マリ M  スイス, チューリッヒ大学, 講師
ブリンクマン D  スイス, チューリッヒ大学, 教授
ヤクボフスキー A  ロシア, クルチャトフ研究所, 主任研究員
ボルサ F  米国, アイオワ州立大学, 教授
BRINKMANN Detlef  Zurich University, Department of Physics, Switzerland, Professor
MALI Mija  Zurich University, Department of Physics, Switzerland, Lecturer
BORSA Ferdinando  Iowa State University, USA,Professor
YAKUBOVSKII Andrey  Kurchatov Institute, Russia, Head of Scientist
Project Period (FY) 1998
Project Status Completed (Fiscal Year 1998)
Budget Amount *help
¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 1998: ¥2,200,000 (Direct Cost: ¥2,200,000)
KeywordsNMR / Oxides / High-T.superconductors / Strong correlated electron / Metal-insulator transition / spin ladder compounds / quantum spin systems
Research Abstract

In this project, unusual electronic properties of the strongly correlated systems such as ladder compounds and transition metal oxides have been investigated by NMR/NQR measurements aa well as magnetic susceptibility and heat capacity measurement. These researches were done under the collaboration of Iowa State University, Kurchatov Institute and Zurich University.
Hole-doping effects on the spin gaps for both the chain and the ladder site are investigated by Cu-NMR and NQR for single crystals of Sr_<14-x>A_1Cu_<24>O_<41> (A=Ca and La). We have confirmed longrange antiferromagnetic order of Cu moments of the chain for 3*x*6 of Sr_<14-x>La_xCu_<24>O_<41>. The experimental results indicate that the magnetic order of Cu spins in the chain is ferromagnetic within the chain, and is antiferromagnetic for the inter-chains. The field-induced staggered moments appears far above T_N. The temperature dependence of the induced field obeys the Curie-Weiss like behavior. These results suggest that the staggered field is not related to the ordered Cu chain moments but is attributed to the magnetic nature of the ladder Cu spins. Possible origins of the field-induced staggered moments at the ladder Cu site are discussed. In addition, we have investigated detail nature of the magnetic order which is observed for a highly hole-doped compound of Sr_<2.5>Ca_<11.5>Cu_<24>O_<41>.
We have also studied metal-insulator (MI) transition in some transition metal oxides. Magnetic and local electronic states near the Metal-Insulator transition have been discussed and presented in original papers We have also presented the results at the lnternational Conference on Strongly Correlated Electron Systems in France, Workshop on NMR in Elecronic Conductors, France, and Colloquium on Magnetic Resonance in High-T.Superconductors, Switzerland.

Report

(2 results)
  • 1998 Annual Research Report   Final Research Report Summary
  • Research Products

    (12 results)

All Other

All Publications (12 results)

  • [Publications] 熊谷 健一: "Study of Antiferromagnetic Order in U(Pt_<1-X>Pd_3)_3 by Heat Capacity Measurement" J.Mag, Mag, Materials. 177-181. 461-462 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 熊谷 健一: "^<63>Cu-NMR Study of Infinite-Lager Conpound Sr_<1-X> La_X CuO_2" Physica C. 304. 165-171 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 熊谷 健一: "Microscopically homogeneous magnetic structure of La_<1-x>MnO_3 beyond the nance of 0.<X<0.1 observed by La-NMR" Phys, Rev.B. 59. 97-99 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 熊谷 健一: "NMR Study of Fell Induced Staggered Moments in Single Aystal of Spin Ladder Sr_<1-X>Lax Ar_<24> O41" J. May, Mag, Materials. in press.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kumagai: "Study of Antiferromagnetic Order in U(Pt_<1-x>Pd_x)_3 by Heat Capacity Measurement" J.Mag.Mag.Materials. 177-181. 461-462 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kumagai: "^<63>Cu NMR Study of Infinite-Layer Compound Sr_<1-x>La_xCuO_2" Physica. C304. 165-171 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kumagai: "Microscopically homogeneous magnetic structure of La_<1-x>Sr_xMnO_3 beyond the range of 0<x<0.1 observed by La NMR" Phys.Rev.B59. 97-99 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] K.Kumagai: "NMR Study of Field Induced Staggered Moments in Single Crystal of Spin Ladder Sr_<14-x>La_xCu_<24>O_<41>" J.Mag.Mag.Materials. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1998 Final Research Report Summary
  • [Publications] 熊谷健一: "Study of Antiferromagnetic Order in U(Pt_<1-X>Pd_2)_3 by Heat Capacity Measurement" J.Mag.Mag.Materials. 177-181. 461-462 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 熊谷健一: "^<63>Cu-NMR Study of Infinite-Layer Compound Sir_2 Lax CuO_2" Physica C. 304. 165-171 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 熊谷健一: "Microscopically homogeneous magnetic structure of LarcbrxMnO_3 beyond the range of 0<x<0.1 observed by La-NMR" Phys.Rev.B. 59. 97-99 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] 熊谷 健一: "NMR Study of Field Induced Staggered Moments in Single Crystal of Spectra Ladder Sr_<1-x>La_xAr_<24>O_<41>" J.Mag.Mag.Materials. (発表予定).

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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