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Variations and Cycles of Greenhouse Gases on the Earth's Surface

Research Project

Project/Area Number 10144103
Research Category

Grant-in-Aid for Scientific Research on Priority Areas (A)

Allocation TypeSingle-year Grants
Research InstitutionTohoku University

Principal Investigator

NAKAZAWA Takakiyo  Tohoku Univ., Grad.School. of Sci., Prof., 大学院・理学研究科, 教授 (30108451)

Co-Investigator(Kenkyū-buntansha) NAKAMURA Toshio  Nagoya Univ., Dating Mater.Res.Center, Prof., 年代測定資料研究センター, 教授 (10135387)
YOSHIDA Naohiro  Tokyo Inst.Tech., Dep.Environ.Sci.Tech., Prof., 大学院・総合理工学研究科, 教授 (60174942)
MAKIDE Yoshihiro  Tokyo Univ., Radioisotope Center, Prof., アイソトープ総合センター, 教授 (40011746)
MORIMOTO Shinji  Nat.Inst.Pol.Res., Assist.Prof, 助手 (30270424)
AOKI Shuji  Tohoku Univ., Grad.School of Sci., Asso.Prof., 大学院・理学研究科, 助教授 (00183129)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥126,300,000 (Direct Cost: ¥126,300,000)
Fiscal Year 2000: ¥30,800,000 (Direct Cost: ¥30,800,000)
Fiscal Year 1999: ¥43,800,000 (Direct Cost: ¥43,800,000)
Fiscal Year 1998: ¥51,700,000 (Direct Cost: ¥51,700,000)
Keywordsgreenhouse gas / carbon dioxide / methane / nitrous oxide / halocarbon / isotope / material cycle / global warming / 物質循環 / 一酸化ニ窒素
Research Abstract

In order to elucidate variations and cycles of greenhouse gases on the Earth's surface, extensive studies with systematic measurements and development of numerical models were performed. The results obtained from this study are summarized as follows :
(l) The concentrations and isotopic ratios of various greenhouse gases such as CO_2, CH_4, N_2O, CO, HCFC, HFC, PFC and SF_6 were systematically measured over Japan, the Pacific Ocean, Siberia, Syowa Station and Spitzbergen Islands, and their temporal and spatial variations as well as causes and governing processes were clarified. Measurements of the isotopomers of atmospheric N_2O succeeded for the first time, and quantitative estimation of the N_2O budget was tried on the basis of the measurement results. Double-deconvolution analysis of the CO_2 concentration and its δ^<13>C was also made to elucidate the recent global budget of anthropogenic CO_2. Furthermore, temporal changes in HCFC, HFC and SF_6 emissions were investigated using a n … More orthernsouthern hemispheric two box-model and their measurement results. (2) A three-dimensional atmospheric transport model was developed and then applied to elucidate their global cycles in terms of the concentration and δ^<13>C.A spatially high-resolution ecosystem model was also developed to examine the role of the terrestrial biosphere in the global carbon cycle, and partial pressure differences of CO_2 between the atmosphere and the ocean were calculated and ocean uptake of CO_2 was estimated using a newly developed three-dimensional ocean carnon cycle model. A multi-box model developed in this study succeeded in reconstructing the history of the atmtospheric N_2O concentration over the last 500 years. (3) For a better understanding of the carbon cycle between the atmosphere and the lithosphere, carbon fluxes due to weathering and the release of carbon from the deep underground were quantitatively estimated by their extensive measurements. Systematic measurements were also carried out in several coral reefs in Okinawa, and it was revealed that the role of coral in the ocean carbon cycle was different depending on coral itself. Less

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (39 results)

All Other

All Publications (39 results)

  • [Publications] K.Ishijima: "Concentration variations of troposheric nitrous oxide over Japan"Geophys.Rev.Lett.. 28. 171-174 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Morimoto: "Latitudinal distribution of atmospheric CO_2 sources and sinks inferred by δ^<13>C measurements from 1985 to 1991"J.Geophys.Res.. 10. 24315-24326 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] N.Yoshida: "Constraining the atmospheric N_2O budjet from inframolecular site preference in N_2O isotopemers"Nature. 405. 330-334 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Watai: "Latitudinal distribution of CO_2 fugacity in the North Pacific along 175°E in 1992-1996"J.Oceanography. 55. 655-665 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Shirai: "Rapidly increasing concentrations of CFC alternatives in the atmosphere as observed in Hokkorids and Antarctica"Chem.Lett.. 357-358 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nakamura: "Isotopic analysis and cycling of dissolved in organic carbur at Lake Biwa, Central Japan"Radiocarbon. 40. 933-944 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 中澤高清: "大気の化学と地球環境"学会出版センター(印刷中). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nakazawa: "Encyclopedia "John Wiley and sons(印刷中). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ishijima et al.: "Concentration variations of tropospheric nitrous oxide over Japan."Geophys.Res.Lett.. 28. 171-174 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Yoshimura wt al.: "Geochemical and stable isotope studies on matural water in the Taroko Gorge karst area, Taiwan : Chemical weathering of carbonate rocks by deep source CO_2 and sulfuric acid."Chem.Geol.. (in press). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Morimoto et al.: "Latitudinal distribution of atmospheric CO_2 sources and sinks inferred by δ^<13>C measurements from 1985 to 1991."J.Geophys.Res.. 105. 24315-24326 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] A.Itoh and T.Oikawa: "A model analysis of the relationship between climate perturbations and carbon budget anomalies in global terrestrial ecosystem ; 1970-1997"Clim.Res.. 15. 161-183 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] N.Yoshida et al.: "Constraining the atmospheric N_2O budget from intramolecular site preference in N_2O isotopomers."Nature.. 405. 330-334 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Mabuchi et al.: "Numerical study of the relation between climate and the carbon dioxide cycle on a regional scale."J.Meteorol.Soc.Japan. 78. 25-46 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Watai et al.: "Latitudinal distribution of CO_2 fugacity in the North Pacific along 175E in 1992-1996."J.Oceanography. 55. 655-665 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nakazawa: "Variations of carbon dioxide and methane in the atmosphere and their global cycles."Global Environment. 2. 5-14 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Shirai et al.: "Rapidly increasing concentrations of CFC alyernatives in the atmosphere as observed in Hokkaido and Antarctica."Chem.Lett.. 357-358 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Saeki et al.: "Methane emissions deduced from a two-dimensional atmospheric transport model and surface concentration data."J.Meteorol.Soc.Japan. 76. 307-324 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nakamura et al.: "Isotopic analysis and cycling of dissolved inorganic carbon at Lake Biwa, central Japan."Radiocarbon. 40. 933-944 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Toyoda: "Fractionation of N_2O isotopomers in the stratosphere"J.Geophys.Res.. (in press). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Ishijima: "Concentration variations of troposheric nitrous oxide over Japan"Geophys.Res.Let.. 28. 171-174 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Morimoto: "Latitudinal distribution of atmospheric CO_2 sources and sinks inferred by δ^<13>C measurements"J.Geophys.Res.. 105. 24315-24326 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] C.Y.Shao: "Equilibrium and Rlnetic studies on the complexation of boric acid with chromotropic acid"J.Chem.Soc.Dalton Trans. 18. 3136-3142 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Tohjima: "Variations in atmospheric nitrous, oxide observed at Hateruma munitoring station"Chemosphere for Global Chance Science. 2. 435-443 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Tennichi: "Simultaneous determination of trace, metals by solid phase absorptiometry"Fresenius'J.Aal.Chem. 368. 443-448 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] 中澤高清: "大気の化学と地球環境"学会出版センター(印刷中). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] 吉村和久: "地下水水質の基礎"理工図書. 189 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T. Watai: "Latitudinal distribution of CO_2 fugacity in the North Pacific along 175°E 1992-1996"J. Oceanography. 55. 655-665 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y. Kondo: "NO_y-N_2O correlation observed inside the Arctic Vortex in February 1997 : dynamical and chemical effect"J. Geophys, Res.. 104. 8215-8224 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y. Yokouchi: "Astrong source methyl chloride to the atomosphere from tropicel coastal land"Nature. 403. 295-298 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] U. Tsunogai: "Carbon isotopic compositions of C_2-C_5 hydrocarbons and methyl chloride in urban, coastal and maritime atmosphere rer the Westen North Pacific"J. Geophys. Res.. 104. 16033-16039 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M. Shiobara: "An overview and preliminary results from the Arctic airbone measurment program 1998 Campaian"Polar Meteorol. Glacio.. 13. 99-110 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 井口 敬雄: "3次元輸送モデルを用いた大気中のCO_2収支の研究"京都大学防災研究所年報. 42B1. 385-395 (1991)

    • Related Report
      1999 Annual Research Report
  • [Publications] 中澤 高清: "地球環境学「大気環境の変化」"岩波書店. 326 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Nakazawa: "Variations of carbon dioxide and methane in the atmosphere and their global carbon cydes" Global Environment. 5-14 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Watai: "Tenporal variations of surface oceanic and atmospheric CO_2 fugacity and total dissolved in organic carbon in the northwestern north Pacific" J.Oceanography. 54. 323-336 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Murayama: "Interpretation of high concentration of O_3 observed in the upper troposphere over Syowa Station,Antarctica" Geophys.Res.Lett. 25. 1177-1180 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Saeki: "Methane emissions deduced from a two-dimonsional atmospheric transport model and surface concentration data" J.Meteorol.Soc.Japan. 76. 307-324 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Wessel: "Tropospheric ozone depletion in polar regions.A comparison of observation in the Arctic and Awtaxctic." Tellus. 50B. 34-50 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2016-04-21  

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