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Electron Energy Bands Studied by 2-Dimensional and Polarization Dependent Photoelectron Spectroscopy Using Synchrotron Radiation

Research Project

Project/Area Number 10304024
Research Category

Grant-in-Aid for Scientific Research (A).

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionRitsumeikan University

Principal Investigator

NAMBA Hidetoshi  Ritsumeikan Univ., Fac.Science and Engineering, Professor, 理工学部, 教授 (40118766)

Co-Investigator(Kenkyū-buntansha) HATTORI Ken  Nara Institute of Science and Technology, Graduate School of Materials Science, Department of Materials Science, Assocate Professor, 物質創成科学研究科, 助教授 (00222216)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥37,900,000 (Direct Cost: ¥37,900,000)
Fiscal Year 2000: ¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 1999: ¥5,000,000 (Direct Cost: ¥5,000,000)
Fiscal Year 1998: ¥29,400,000 (Direct Cost: ¥29,400,000)
KeywordsNew Surface Materials / One Dimensional Materials / Two Dimensional Materials / Fermi Surface / Energy Band / Photoelectron Spectroscopy / Synchrotron Radiation
Research Abstract

Electronic states of 2- or 1-dimensional materials on surfaces and high-temperature superconductors can be best studied by 2-dimensional display type ultraviolet photoelectron spectroscopy using synchrotron radaition (SR). We developed a new beamline for this purpose at BL-7 of Ritsumeikan University SR Center. Linearly polarized SR of the photon energy from 30 to 150 eV is available by this beamline. By using a 2-dimensional display type spherical mirror electron energy analyzer for angle-resolved photoelectron spectroscopy, we can measure electronic energy bands of crystalline materials over a very wide range of the Brilluion zone within a very short time of measurements. We can also determine the atomic orbitals of the energy bands by analyzing the polarization dependence of 2-dimensional photoelectron emission patterns. So we constructed a new experimental apparatus for these purposes. The electronic states of single crystalline graphite and of the clean surfaces of Si(100) were st … More udied by this method.
Photoelectron emission patterns of graphite as a function of the binding energy of electrons were recorded and the energy bands over the wide range of the Brilluion zone were determined. The Fermi surface of graphite was determined from the emission pattern displayed at the binding energy of the Fermi level. The specific changes of the photoelectron emission patterns as a function of the photon energy were revealed. The structure factor of photoemission processes was estimated from the results. By analyzing the incident angle dependence of the emission patterns, the characters of the atomic orbitals of the valence bands are determined.
On the clean surfaces of Si(100), the photoelectron emission patterns from the dangling bonds of the surface dimer are found. The bulk electronic states near T-point of the Brilluin zone is also detected.
In conclusion, the experimental system for the exclusive use of 2-dimensional display type photoelectron spectroscopy by using SR was completed. This opens unique studies of low dimensional electron physics of new materials in future. Less

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (29 results)

All Other

All Publications (29 results)

  • [Publications] T.Nishimura,Y.Hoshino,H.Namba and Y.Kido: "Oxidation processes for Si(111)-7x7 surfaces analyzed in situ by synchrotron radiation induced photoemission and medium energy ion scattering"Proceedings of Synchrotron Radiation Instruments 2000. (in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nishimura,Y.Hoshino,H.Namba and Y.Kido: "Initial oxidation of Si(111)-7x7 surfaces studied by photoelectron spectroscopy combined with medium energy ion scattering"Surf.Sci.. 461. 146-154 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Y.Kido,T.Nishimura,Y.Hoshino and H.Namba: "Surface structure of SrTiO3(001)and Ni/SrTiO3(001)studied by mediumenergy ion scattering and SR-photoelectron spectroscopy"Nucl.Instr.and Meth.. B136-138. 371-376 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Hattori,A.Kobayashi,K.Fukumoto,Y.Miyatake and H.Daimon: "Effective magnetic quantum number and effective emitrer-scatterer distance obtained from W 4f photoelectron diffraction induced by circularly polarized light on W(110)"Surf.Sci.. (in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kotsugi,S.Imada,S.Suga,K.Hattori,H.Daimon et al.: "Construction of two-dimensional photoelectron spectroscopy at Spring-8"Proceedings of Synchrotron Radiation Instruments 2000. (in press).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Enomoto,Y.Muyatake,K.Fukumoto,A.Kobayashi,K.Hattori and H.Daimon: "Two-dimensional circularly-polarized-light photoelectron diffraction for the analysis of magnetic and electronic properties on surfaces"Surf.Rev.Lett.. 7. 643-647 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nishimura, Y.Hoshino, H.Namba and Y.Kido: "Oxidation processes for Si (111)-7x7 surfaces analyzed in situ by synchrotron radiation induced photoemission and medium energy ion scattering"Proceedings of Synchrotron Radiation Instruments. (In press.). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nishimura, Y.Hoshino, H.Namba and Y.Kido: "Initial oxidation of Si (111)-7x7 surfaces studied by photoelectron spectroscopy combined with medium energy ion scattering"Surf. Sci. 461. 146-154 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Y.Kido, T.Nishimura, Y.Hoshino and H.Namba: "Surface structure of SrTiO3 (001) and Ni/SrTiO3 (001) studied by medium-energy ion scattering and SR-photoelectron spectroscopy"Nucl. Instr. And Meth. B136. 371-376 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Hattori, A.Kobayashi, K.Fukumoto, Y.Miyatake and H.Daimon: "Effective magnetic quantum number and effective emitter-scatterer distance obtained from W 4f photoelectron diffraction induced by circularly polarized light on W (110)"Surf. Sci.. (In press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kotsugi, S.Imada, S.Suga, K.Hattori, H.Daimon et al.: "Construction of two-dimensional photoelectron spectroscopy at Spring-8"Proceedings of Synchrotron Radiation Instruments. (In press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Enomoto, Y.Miyatake, K.Fukumoto, A.Kobayshi, K.Hattori and H.Daimon: "Two-dimensional circularly-polarized-light photoelectron diffraction for the analysis of magnetic and electronic properties on surfaces"Surf.Rev.Lett. 7. 643-647 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Nishimura,Y.Hoshino,H.Namba and Y.Kido: "Oxidation processes for Si(111)-7x7 surfaces analyzed in situ by synchrotron radiation induced photoemission and medium energy ion scattering"Proceedings of Synchrotron Radiation Instruments 2000. (in press).

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Nishimura,Y.Hoshino,H.Namba and Y.Kido: "Initial oxidation of Si(111)-7x7 surfaces studied by photoelectron spectroscopy combined with medium energy ion scattering"Surf.Sci.. 461. 146-154 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Kido,T.Nishimura,Y.Hoshino and H.Namba: "Surface structure of SrTiO3(001)and Ni/SrTiO3(001)studied by medium-energy ion scattering and SR-photoelectron spectroscopy"Nucl.Instr.and Meth.. B136-138. 371-376 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Hattori,A.Kobayashi,K.Fukumoto,Y.Miyatake and H.Daimon: "Effective magnetic quantum number and effective emitter-scatterer distance obtained from W 4f photoelectron diffraction induced by circularly polarized light on W(110)"Surf.Sci.. (in press).

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Kotsugi,S.Imada,S.Suga,K.Hattori,H.Daimon et al.: "Construction of two-dimensional photoelectron spectroscopy at Spring-8"Proceedings of Synchrotron Radiation Instruments 2000. (in press).

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Enomoto,Y.Muyatake,K.Fukumoto,A.Kobayashi,K.Hattori and H.Daimon: "Two-dimensional circularly-polarized-light photoelectron diffraction for the analysis of magnetic and electronic properties on surfaces"Surf.Rev.Lett.. 7. 643-647 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Kido,T.Nishimura,Y.Hoshino and H.Namba: "Surface structure of SrTiO3(001) and Ni/SrTiO3(001) studied by MEIS and SR-PES"Nucl.Instrum.Methods B. in press.

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Nishimura,A.Ikeda,H.Namba,T.Morishita and Y.Kido: "Structure Change of TiO2-terminated SrTiO3(001) surfaces by annealed in O2 atomosphere and ultrahigh vacuum"Surf.Sci.. 421. 273-278 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Daimon,M.Kotsugi,T.Okuda and K.Hattori: "Characterization of electronic states using a polarized light and a display analyzer"Jpn.J.Appl.Phys.. 38. 630-633 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kushida,K.Hattori,S.Arai,T.Iimori and F.Komori: "Initial stage of Ag growth on Ge(001) surfaces at room temperature"Surf.Sci.. 442. 300-306 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Daimon,M.Kotsugi,K.Nakatsuji,T.Okuda and K.Hattori: "Deduction of atomic orbitals in a valence band by two-dimensional angular distribution of photoelectrons"Surf.Sci.. 438. 214-222 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Namba, K.Yamamoto, T.Ohta & H.Kuroda: "One-dimensional band-like electronic states on Ni(755) surfaces studied by angle-resolved photoelectron spectroscopy using synchrotron radiation" J. Electron Spectroscopy Releted Phenom.88-89. 707-710 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Nishimura, A.Ikeda, H.Namba & Y.Kido: "Surface relaxation and rumpling of RbI(001) determined by medium energy ion scattering" Surf.Sci.Lett.411. L834-L838 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Namba, M.Obara, D.Kawakami, T.Nishimura, Y.Yan, A.Tagishita & Y.Kido: "A compact vacuum-ultraviolet beamline for synchrotron radiation photoelectron spectroscopy combined with an ion scattering spectrometer, SORIS" J.Synchrotron Rad.5. 557-558 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Iwai, H.Namba, Y.Kido, M.Taguchi & R.Oiwa: "Improvement of spectrometer energy resolution for high-resolution photoelectron spectroscopy" J.Synchrotron Rad.5. 1020-1022 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Hattori, K.Shudo, M.Ueta, T.Iimoro & F.Komori: "Hydrogen-chlorine exchange reactions on Si(111)-7x7 studied with STM" Surf.Sci.402/404. 170-173 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] F.Komori, T.Iwaki, K.Hattori, O.Shinjo & T.Hasegawa: "Tunneling spectroscopy around the boundary of a small impurity phase on the surface of 2H-NbSe2" Appl.Phys.A66. S135-138 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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