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Core-level Spectroscopy using Coincidence of Synchrotron Radiation and Laser

Research Project

Project/Area Number 10304025
Research Category

Grant-in-Aid for Scientific Research (A).

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionOkazaki National Institutes

Principal Investigator

KAMADA Masao  Institute for Molecular Science, Okazaki National Institutes Associate Professor, 分子科学研究所, 助教授 (60112538)

Co-Investigator(Kenkyū-buntansha) TAKAHASHI Kazuhiko  Institute for Molecular Science.Research Associate, 分子科学研究所, 助手 (30332183)
TSUJIBAYASHI Toru  Osaka Dental University, Lecturer, 講師 (50214771)
ITOH Minoru  Shinshu University Faculty of Engineering. Professor, 工学部, 教授 (80126664)
ARIMOTO Osamu  Okayama Univ., Faculty of Science, Associate Professor, 理学部, 助教授 (70193092)
ITOH Hiroshi  Kagawa University Faculty of Engineering, Professor, 工学部, 教授 (60112249)
渡辺 雅之  京都大学, 総合人間学部, 助手 (20240525)
田中 慎一郎  岡崎国立共同研究機構, 分子科学研究所, 助手 (00227141)
浅香 修治  岡崎国立共同研究機構, 分子科学研究所, 助手 (00167876)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥34,600,000 (Direct Cost: ¥34,600,000)
Fiscal Year 2000: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 1999: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 1998: ¥31,500,000 (Direct Cost: ¥31,500,000)
KeywordsSynchrotron Radiation / Pulsed Photon / Laser Coincidence / Core-level Spectroscopy / Two-photon Spectroscopy / Core Exeiton / Photo-induced Phenomena / Time-resolved Photoelectron / レーザー / 同期実験 / ポンプ プローブ / BaF2 / CaF2 / GaAs / レーザー同期 / 真空紫外光 / レーザー誘起 / ポンプ-プローブ / BaF_2
Research Abstract

The coincidence of synchrotron radiation and laser is a powerful method to investigate solids and surfaces. There are three types of combinations : two-photon excitation of SR and laser, SR pump and laser probe. and Laser pump and SR probe. In this project. we have developed these three types of combinational uses of SR and laser. For examples. we have observed the luminescence from a wide-band gap material BaF2 excited by two photons (SR and laser), since BaF2 is one of interesting materials showing the Auger-free luminescence.
Besides this, the two-photon reflection technique was also developed and the sharp structures were observd in the spectra of GaAs and ZnSe. A core-level photoelectron spectroscopy was developed to investigate the laser-induced phenomena on semiconductor and metal-organic complexes. The GaAs system showed a surface photovoltage effect and its temporal structure. The spin-cross over complex showed the remarkable change in the photoelectron spectra by laser irradiation.

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (28 results)

All Other

All Publications (28 results)

  • [Publications] M.Kamada 他: "Combined System of SR and Laser for Solid-State Research"J.Synchrotron Rad.. 5. 1035-1037 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Asaka 他: "Time-Gated Photon Counting Metod for Two-Photon Spectroscopy Using Synchrotron Radiation and Laser"Rev.Sci.Instrum. 69. 1931-1933 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsujibayashi 他: "Resonance enhancement effect on two-photon absorption due to excitons in alkaline-earth fluorides excited with synchrotron radiation and laser light"Phys.Rev.B. 60. 8442-8445 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsujibayashi 他: "Two-photon excitation spectra of exciton luminescence in BaF_2 obtained by using synchrotron radiation and laser"J.Luminescence. 87-89. 254-256 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kamada 他: "Photo-induced change in semiconductor-vacuum interface of p-GaAs (100) studied by photoelectron spectroscopy"Surface Science. 454-456. 525-528 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Asaka 他: "Ultraviolet light amplification within a nanometer-sized layer"Phys.Rev.B. 63. 81104-81107 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] O.Arimoto et al.: "Combination of Synchrotron Radiation and Laser for Two-Photon Spectroscopy of BaF_<>"J.Electron Spectrosc.Relat Phenom. 92. 219-222 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kamada et al.: "Combined System of SR and Laser for Solid-State Research"J.Synchrotron Rad. 5. 1035-1037 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Asaka et al.: "Time-Gated Photon Counting Meted for Two-Photon Spectroscopy Using Synchrotron Radiation and Laser"Rev.Sci.Instrum. 69. 1931-1933 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kamada et al.: "Simultaneous Measurements of Photoelectron and Luminescence of Barium Halides"J.Electron Spectrosc Relat.Phenom.. 88. 297-301 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsujibayashi et al.: "Resonance enhancement effect on two-photon absorption due to excitons in alkaline-earth fluorides excited with synchrotron radiation and laser light"Phys.Rev.B. 60. 8442-8445 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kamada et al.: "Nano-Second Desorption of Alkali Fluorides Excited by Synchrotron Radiation Pulses"J.Electron spectroscopy and Related Phenom.. 101/103. 599-602 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsujibayashi et al.: "Two photon excitation spectra of exciton luminescence in BaF_2 obtained by using synchrotron radiation and laser"J.Luminescence. 87/89. 254-255 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Kamada et al.: "Photo induced change in semiconductor-vacuum interface of p-GaAs (100) studied by photoelectron spectroscopy"Surface Science. 454/456. 525-528 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.More et al.: "Coadsorption of Cs and O on GaAs : Formation of negative electron affinity surfaces at different temperatures"Surface Science. 454/456. 161-165 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Asaka et al.: "Ultraviolet light amplification within a nanometer-sized layer"Phys.Rev.B. 63. 81104-81107 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsujibayashi 他: "Two-photon excitation spectra of exciton luminescence in BaF_2 obtained by using synchrotron radiation and laser"J.Luminescence. 87-89. 254-256 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Kamada 他: "Photo-induced change in semiconductor-vacuum interface of p-GaAs (100) studied by photoelectron spectroscopy"Surface Science. 454-456. 525-528 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.More 他: "Coadsorption of Cs and O on GaAs : Formation of negative electron affinity surfaces at different temperatures"Surface Science. 454-456. 161-165 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Kamada 他: "Beam-line systems for pump-probe photoelectron spectroscopy using SR and laser"Nucl.Instrum.Methods. (印刷中). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Asaka 他: "Optical detection system using time structure of UVSOR for combined laser-SR experiments"Nucl.Instrum.Methods. (印刷中). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Asaka 他: "Ultraviolet light amplification within a nanometer-sized layer"Phys.Rev.B. 63. 81104-81107 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] V.B. Mikahailik et al.: "Amplification of impurity-associated Auger-free Luminescence in mixed rubidium-caesium chloride crystals under core-level excitation with undulator radiation"Optics Commun.. 171. 71-76 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T. Tsujibayashi et al.: "Resonant enhancement effect on two-photon absorption due to excitons in alkaline-earth fluorides excited with synchrotron radiation and laser light"Phys. Rev. B. 60. 8442-8445 (1990)

    • Related Report
      1999 Annual Research Report
  • [Publications] M. Kamada et al.: "Nano-Second Desorption of Alkali Fluorides Excited by Synchrotron Radiation Pulses"J. Electron spectroscopy and Related Phenom.. 101/103. 599-602 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Asaka,et al.: "Time-gated photon counting method for two-photon spectroscopy using synchrotron radiation and laser" Rev.Sci.Instr.69巻5号. 1931-1933 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] O.Arimoto,et al.: "Combinational Use of Synchrotron Radiation and Laser for Two-Photon Spectroscopy of BaF2" J.Electron Spectroscopy and Related Phenomena. 72巻. 219-223 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] M.Kamada,et al.: "Combined systems of SR and Laser for solid-state researches" J.Synchrotron Radiation. 5巻. 1035-1037 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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