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A study on cooperation and competition between the magnetic correlation and transport properties in systems with localized and itinerant electrons

Research Project

Project/Area Number 10304026
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

YAMADA Kazuyoshi  Kyoto University, Professor, 化学研究所, 教授 (70133923)

Co-Investigator(Kenkyū-buntansha) SATO Noriaki  Kyoto University, Assistant Professor, 大学院・理学研究科, 助教授 (30170773)
IKEDA Yasunori  Kyoto University, Instructor, 化学研究所, 助手 (20243090)
FUJITA Masaki  Kyoto University, Instructor, 化学研究所, 助手 (20303894)
Project Period (FY) 1998 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥32,010,000 (Direct Cost: ¥31,200,000、Indirect Cost: ¥810,000)
Fiscal Year 2001: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2000: ¥4,800,000 (Direct Cost: ¥4,800,000)
Fiscal Year 1999: ¥11,000,000 (Direct Cost: ¥11,000,000)
Fiscal Year 1998: ¥12,700,000 (Direct Cost: ¥12,700,000)
Keywordselectron-doped superconductivity / hyigh-Tc superconductivity / neutron scattering / muon spin rotation / 超伝導と磁気秩序の共存 / 単結晶育成
Research Abstract

In this program, we systematically studied cooperation or competition between magnetic order or fluctuation and superconductivity of strongly correlated electron systems such as high temperature superconductors and uranium compounds by using neutron scattering and other microscopic techniques on single crystals with high quality.
The superconductivity in the high temperature cuprates appears by carrier doping into the Mott insulators. In recent years, the self-organization of the doped carriers was found in these cuprates particularly in the 2-1-4 type cuprates. One of the main issues is whether the self-organization commonly occurs in other types of cuprates and induces novel quantum properties such as high temperature superconductivity. Although this issue is still continuing, in this program we could provide several key experimental results for the elucidation of this problem.
In the study on the uranium compounds particularly on UPd_2Al_3 , we completed a model for the paring mechanism, where three 5f-electrons of U play a role differently for the superconductivity in this compound ; one constructs a magnetic framework and the other forms the Cooper paring through the magnetic excitations of the framework. It turns out this model can explain not only the symmetry of the superconductivity also many of the physical properties of this system.
As seen in UPd_2Al_3 the possibility of contribution from different types of electrons for mechanism of the paring force in the high temperature superconductor will be one of the main issues and elucidated if one succeeds in distinguishing the intrinsic electronic inhomogeneity from that caused by the chemical randomness by doping carriers.

Report

(5 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (75 results)

All Other

All Publications (75 results)

  • [Publications] K.Kurahashi: "Heat treatment effects on the superconductivity and crystal structure of Nd_<1.85>Ce_<0.15>CuO_4 studied using a single crystal"J. Phys. Soc. Jpn.. 71(印刷中). (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Sato: "Observation of d_<x2-y2>-like Superconducting Gap in an Electron-Doped High-Temperature Superconductor"Science. 291. 1517-1519 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] E.J.Singley: "Electron dynamics in Nd_<1.85>Ce_<0.15>CuO_4 : Similarities to hole doped cuprates"Phys. Rev..B. 64. 2244503 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] I.Watanabe: "μSR study of magnetic properties of Nd_<2-x>Ce_xCuO_4 around a boundary between the magnetically ordered state and superconducting state"Physica C. 357-360. 212-215 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] N.Yamamoto: "Superocnducting Anisotropy in Nd_<1.85>Ce_<0.15>CuO_4 Single crystals"Physica C. 357-360. 298-301 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T.Uefuji: "Coexistence of Antiferromagnetic Ordering and High-Tc Superconductivity in Electron-Doped Superconductor Nd_<2-x>Ce_xCuO_4"Physica C. 357-360. 208-211 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Kurahashi: "Heat treatment effects on the superconductivity and Ctystal structure on ND1.85Ce0.15CuO4 studied using a Single crystal."J. Phys. Soc. Jpn.. (to be published). (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Sato: "Observation of dx2-y2-like superconducting gap in an electron-Doped high-temperature superconductor."Science. 291. 1517-1519 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] E.J. Singly: "Electron dynamics in ND1.85Ce0.15Cu04 : Similatities to hole doped cuprates"Phys. Rev. B. 64. 2244503 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] I. Watanabe: "MSR study of magnetic properties of Nd2-xCexCuO4 around A boundary between the magnetically ordered state and superconducting state."Physica C. 357-360. 212-215 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] N. Yamamoto: "Superconducting anisotropy in ND1.85Ce0.15CuO4 single Crystals."Physica C. 357-360. 298-301 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] T. Uefuji: "Coexistence of Antiferromagnetic ordering and High-Tc Superconductivity in electron-doped superconductor Nd2-xCexCuO4"Physica C. 357-360. 208-211 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Kurahashi: "Heat treatment effects on the superconductivity and crystal structure of Nd_<1.85>Ce_<0.15>CuO_4 studied using a single crystal"J.Phys.Soc.Jpn.. 71(印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sato: "Observation of d_<x2-y2>-like Superconducting Gap in an Electron-Doped High-Temperature Superconductor"Science. 291. 1517-1519 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] E.J.Singley: "Electron dynamics in Nd_<1.85>Ce_<0.15>CuO_4: Similarities to hole doped curates"Phys.Rev.B. 64. 224503 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] I.Watanabe: "μSR study of magnetic properties of Nd_<2-x>Ce_xCuO_4 around a boundary between the magnetically ordered state and superconducting state"Physica C. 357-360. 212-215 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] N.Yamamoto: "Superocnducting Anisotropy in Nd_<1.85>Ce_<0.15>CuO_4 Single crystals"Physica C. 357-360. 298-301 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T Uefuji: "Coexistence of Antiferromagnetic Orderihg and High-Tc Superconductivity in Electron-Doped Superconductor Nd_<2-x>Ce_xCuO_4"Physica C. 357-360. 208-211 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Wakimoto: "Systematic study of short range antiferromagnetic order and the spin-glass state in lightly doped La_<2-x>Sr_xCuO_4"Phys.Rev.B. 62. 3547-3553 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Hamada: "Development of itinerant-electron antiferromagnetism in the approach to metal-insulator transition in metallic NiS_<2-x>Se_x as studied by ^<77>Se NMR"Physica B. 281 & 282. 641-643 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Matsuura: "Magnetic phase diagram and metal-insulator transition of NiS_<2-x>Se_x"J.Phys.Soc.Jpn.. 69. 1503-1508 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Kimura: "Incommensurate geometry of the elastic peaks in supercondcuting La_<1.88>Sr_<0.12>CuO_4"Phys.Rev.B. 61. 14366-14369 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Matsuda: "Static and dynamical spin correlations in the spin-glass phase of slightly doped La_<2-x>Sr_xCuO_4"Phys.Rev.B. 62. 9148-9154 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Katano: "Enhancement of static antiferromanetic correlations by magnetic field in a superconductor La_<2-x>Sr_xCuO_4 with x=0.12"Phys.Rev.B. 62. R14677-R147680 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.-H.Lee: "Charge and spin order in La_<2-x>Sr_xNiO_4 (x=0.275 and 1/3)"Phys.Rev.B. (to be published). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Takahashi: "Para-ferro magnetic phase transition of CoS_2 studied by high-resolution photoemission spectroscopy"Phys.Rev.B. (to be published). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] A.Schenck: "Study of the positive Muon Knight shift in UNi_2Al_3 : evidence for a tetravalent U^<4+>-state and crystalline electric field (CEF) splitting"Eur.Phys.J.B.. 13. 245 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] N.Kernavanois: "Polarized neutron scattering and X-ray magnetic circular dichroism studies of the heavy-fermion superconductor UNi_2Al_3"J.Phys.: Condens.Matter. 12. 7857-7867 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] N.Aso: "Neutron-scattering study of the magnetic response in the heavy-fermion superconductor UNi_2Al_3"Phys.Rev.B. 61. R11867-R11870 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Nishioka: "High pressure magnetization measurements on URu_2Si_2"J.Phys.Soc.Jpn.. 69. 2415-2418 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Sakon: "Temperature and field dependence of magnetization on UPd_2Al_3"Physica B. 282 & 282. 240-241 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] F.Steglich: "Unconventional normal-state properties and superconductivity in heavy-fermion metals"Physica C. 341-348. 691-694 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Miyake: "Unconventional Cooper pairing in the superconducting state of UPd_2Al_3"Phys.Rev.B (to be published). 63. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] N.K.Satp: "Strong coupling between local moments and superconducting heavy electrons in UPd_2Al_3"Nature (to be published). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.-H.Lee: "Search for Orbital Moments in Underdoped Cuprate Metals"Phys. Rev. B. 60. 10405-10417 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Wakimoto: "New Inommensurate Magnetic Correlations at the Lower Critical Concentration of the Superconductivity, La_<1.95>Sr_<0.05>CuO_4"Phys. Rev. B. 60. R769-R772 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Sato: "Pseudogap of Optimally Doped La_<1.85>Sr_<0.15>CuO_4 Observed by Ultrahigh-Resolution Photoemision Spectroscopy"Phys. Rev. Lett. 83. 2254-2257 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] R.J.Birgeneau: "Instantaneous Spin Correlations in La_2CuO_4"Phys. Rev. B. 59. 13788-13794 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.J.Kim: "Quantum Monte Carlo Study of Weakly Coupled Spin Ladders"Phys. Rev. B. 60. 3294-3304 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Suzuki: "Conventional Superconductor-like Behaviour of Superconducting Transition of La_2CuO_4 around x=0.12 in Magnetic Fields"Phys. Rev. B. 60. 10500-10503 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.S.Lee: "Neutron-scattering Study of Spin-density Wave Order in the Superconducting State of Excess-oxygen-doped La_2CuO_<4+y>"Phys. Rev. B. 60. 3643-3654 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Kimura: "Structural Instability Associated with the Tilting of CuO_6 Octahedron in La_<2-x>Sr_xCuO_4"J. Phys. Soc. Jpn.. (to be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] C.H.Lee: "Energy Spectrum of Spin Fluctuations in the Superconducting La_<2-x>Sr_xCuO_4 (x=0.10. ,0.15, 0.18 and 0.25)"J. Phys. Soc. Jpn.. (to be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Matsuda: "Freezing of Anisotropic Spin Clusters in La_<1.98>Sr_<0.02>CuO_4"Phys. Rev. B. (to be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Sato: "Effect of Quasi Two-dimensional Fermi Surfaces on Electronicproperties in YbSb_2"Phys. Rev. B. 59. 4714-4719 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Takahashi: "Crystallographic Parameters in the Compounds La_<1-x>Ce_xB_6"J. Phys. Soc. Jpn.. 68. 692-693 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Sato: "Possible Negative Mode-mode Coupling in Upd_2Al_3"J. Phys.: Condens. Matter. 11. 3405-3412 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Fujimori: "Absence of U 5f Band States in Resonant Photoemission Spectrum of Upd_2Al_3"Phys. Rev. B. 59. 10469-10472 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Sato: "Correlation between Low-energy Spin Fluctuations and Superconductivity in Upd_2Al_3 and Upt_3"Physica B. 259-261. 634-635 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Bernfoeft: "Magnetic Fluctuations above and below T_c in the Heavy Fermion Superconductor Upd_2Al_3"Physica B. 259-261. 614-620 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Aso: "Single Crystal Growth and Physical Properties in Upd_2(Al_<(1-x)>Ga_x)_3"Physica B. 259-261. 636-637 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] A.V.Kolomiets: "Magnetism and Transport in Uga_2 Single Crystal"Physica B. 259-261. 238-239 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Sato: "Static and Dynamical Properties in the Heavy Fermion Superconductors Upd_2Al_3 and Uni_2Al_3"J .J. A. P. Series. 11. 56-58 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Fujimori: "Photoemission and Inverse-photoemission Study of Heavy-fermion Uranium Compounds"J. J. A. P. Series. 11. 215-217 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Sugiyama: "Metamagnetic Transition of Heavy Fermion Uranium Compounds: Upd_2Al_3, Uru_2Si_2 and Upt_3"J.J.A.P.Series. 11. 18-20 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] N.Mori: "Anomalous Transport Phenomena in SmS ans TmSe with Pressure-induced Valence Transitions"J. J. A. P. Series. 11. 129-131 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] A.Schenck: "Study of the Positive Muon Knight Shift in Uni_2Al_3: Evidence for a Tetravalent U^<4+> -state and Crystalline Electric Field (CEF) Splitting"Eur. Phys. J. B.. 13. 245 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] C.H.Lee: "Growth of Large Single Crystals Using the Improved Lamp-image Floating-zone Furmace: Application to La_<2-x>Sr_xCuO_4" Supercond.Sci.Technol.11. 891-897 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Yamada: "Doping Dependence of Spatially Modulated Dynamical Spin Correlations and Superconducting Transition Temperature in La_<2-x>Sr_xCuO_4" Phys.Rev.B. 57. 6165-6172 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Isawa: "Thermoelectric Power of Delafossite-derived Compounds,RCuO_<2+δ>(R=Y,La,Pr,Nd,Sm,and Eu)" Phys.Rev.B. 57. 7950-7954 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Suzuki: "Observation of Modulated-magnetic Long-range Order in La_<1.88>Sr_<0.12>CuO_4" Phys.Rev.B. 57. R3229-R3232 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Kimura: "Neutron Scattering Study of Static Antiferromagnetic Correlations in La_<2-x>Sr_xCu_<1-y>Zn_yO_4" Phys.Rev.B. 59. in print (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] F.Hayashi: "Anisotropy of the Superconducting Order Parameter of Nd_<2-x>Ce_xCuO_4 Studied by STM/STS" J.Phys.Soc.Jpn.67. 3234-3239 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Sugai: "Separation of Spin and Charge Densities in La_2NiO_<4+δ>" J.Phys.Soc.Jpn.67. 2992-2995 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] N.Kaneko: "Optimum Crucible Material for Growth of Pr_<2-x>Ce_xCuO_4 Crystal" J.Cryst.Growth. 197. 818-824 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Isawa: "Crystal Structure Refinement of the Oxygen-rich RCuO_<2+δ>(R=Y and La) Delafossite by Neutron Diffraction" Advances in Superconductivity X. 395-398 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Yamada: "How Does the High-T_c Superconductivity Disappear by Overdoping? -A Scenario from a Neutron Scattering Study on La_<2-x>Sr_xCuO_4-" Advances in Superconductivity X. 37-42 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] A.Ishiguro: "De Haas-van Alphen Effect in CoS_2" J.Mag.Mag.Mater.177-181. 1355-1356 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Wakimoto: "Magnetism of Lightly Oxygenated La_<2-x>Bi_xCuO_<4+δ>" Physica B. 241-243. 634-636 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Hirota: "Quasi-elastic Incommensurate Peaks in La_<2-X>Sr_XCu_<1-y>O_<4-δ>" Physica B. 241-243. 817-819 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Yamada: "Static and Dynamical Incommensurate Spin Correlations in High-T_c Cuprates of La_<2-x>Sr_xCuO_<4+y>" Proc.Taniguchi Symposium. (in print). (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Wakimoto: "Neutron Scattering Study of Elastic Magnetic Signals in Superconducting La_<1.94>Sr_<0.06>CuO_4" J.Phys.Chem.Solids. (in print). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Kimura: "Neutron Scattering Study of Incommensurate Elastic Magnetic Peaks in La_<1.88>Sr_<0.12>CuO_4" J.Phys.Chem.Solids. (in print). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Yamada: "Neutron Scattering Study on Electron-hole Doping Symmetry of High-T_c Superconductivity" J.Phys.Chem.Solids. (in print). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Ohta: "High Field AFMR Measurement of Bi_2CuO_4" Physica B. 246-247. 557-560 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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