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Dynamics of low dimensional quantum spin systems and effects of carrier doping.

Research Project

Project/Area Number 10304027
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionThe University of Tokyo

Principal Investigator

TAKIGAWA Masashi  University of Tokyo, The Institute for Solid State Physics, Professor, 物性研究所, 教授 (10179575)

Co-Investigator(Kenkyū-buntansha) UEDA Yutaka  University of Tokyo, The Institute for Solid State Physics, Professor, 物性研究所, 教授 (20127054)
FUJIWARA Naoki  University of Tokyo, The Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (60272530)
KODAMA Katsuaki  University of Tokyo, The Institute for Solid State Physics, Research Associate, 物性研究所, 助手 (10313115)
TAKAGI Hidenori  University of Tokyo, Graduate School of Frontier Sciences, Professor, 新領域創成科学研究科, 教授 (40187935)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥36,800,000 (Direct Cost: ¥36,800,000)
Fiscal Year 2000: ¥5,100,000 (Direct Cost: ¥5,100,000)
Fiscal Year 1999: ¥16,000,000 (Direct Cost: ¥16,000,000)
Fiscal Year 1998: ¥15,700,000 (Direct Cost: ¥15,700,000)
KeywordsQuantum Spin System / Nuclear Magnetic Resonance / Carrier Doping / Spin Gap / Low Dimensionality / 梯子格子 / 近藤絶縁体 / ホールドープ / 電荷ゆらぎ / 電荷凍結 / 近藤半導体 / スピン拡散 / 高温超伝導
Research Abstract

Since the high temperature superconductivity was discovered in 1986, various attempts were made to dope carriers into low dimensional quantum spin systems, which are the Mott-insulators and to find superconductivity. In such a trend of research, the first objectives of this project was set to clarify the dynamics of the low dimensional quantum spin systems from a microscopic point of view using nuclear magnetic resonance as the principal tool. Second objective was to understand the change in magnetic dynamics upon elemental substitution or doping carriers or impurities. The former was achieved by the experiments on the hole-doped spin-ladder materials and the two-dimensional orthogonal dimer spin systems, which yielded variety of different behavior of spin excitations for the singket ground state. Concerning the latter, experiments on hole-doped ladder materials have shown that interaction between carriers and the magnetic excitations induces paring of holes. The thermally depaired carriers are shown to cause significant damping of magnetic excitations. Furthermore, extremely slow charge fluctuations associated with partial charge ordering were observed in a few quasi-one-dimensional conducting systems. On the other hand, in Kondo insulators, which is another example of spin gap material, we found that local moments are induced near impurities similar to the case of quantum spin systems.

Report

(4 results)
  • 2001 Final Research Report Summary
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (52 results)

All Other

All Publications (52 results)

  • [Publications] Y.Ueda: "Vanadium Family as Spin-Gap Systems"Chem. Mater.. 10. 2653-2664 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Fujiyama: "Nuclear spin-spin coupling in La_<2-x>Sr_xCuO_4 studied by stimulated echo decay"Phys. Rev. B. 60. 9801-9809 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Ikushima: "^<171>Yb NMR in the Kondo semiconductor YbB_<12>"Physica B. 281&282. 274-275 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Fujiyama: "Low energy spin excitations in Sr_<14-x>Ca_xCu_<24>O_<41>"Physica C. 341-348. 461-462 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Fujiyama: "Spin Correlations in Hole-Doped Ladder Cuprates"J. Phys. Soc. Jpn.. 69Suppl.B. 46-53 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Ueda: "Low-Dimensional Vanadlium Oxides"J. Phys. Soc. Jpn.. 69Suppl.B. 149-154 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Fujiyama: "Nuclear Spin Relaxation in Hole-Doped Two-Leg Ladders"J. Phys. Soc. Jpn. 69. 69. 1610-1613 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] J.P.Boucher: "Possible localized modes in the uniform quantum Heisenberg chains of Sr_2CuO_3"Phys. Rev. B. 62. 367-371 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z.Hiroi: "Spin-1/2 Kagome-Like Lattice in Volborthite Cu_3V_2O_7(OH)_22H_2O"J. Phys. Soc. Jpn.. 70. 3377-3384 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] D.Akahoshi: "Oxygen Nonstoichiometry, Structures, and Physical Properties of YbaCo_2O_<5+x>(0.00 x 0.52)"J. Solid State Chem.. 156. 355-363 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Ohwada: ""Devil's Staicase"-Type Phase Transition in NaV_2O_5 under High Pressure"Phys. Rev. Lett.. 87. 086402-1-086402-4 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 瀧川 仁: "モット転移と磁気相関"日本物理学会誌. 54. 90-97 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 藤山 茂樹: "Sr_<14-x>Ca_xCu_<24>O_<41>におけるCuおよびO核NMR"物性研究. 72. 466-469 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 樹神 克明: "2次元スピンギャップ系SrCu_2(BO_3)_2のNMR"物性研究. 76. 516-525 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 廣井善二: "パイロクロア酸化物超伝導体Cd_2Re_2O_7"固体物理. 37. 253-264 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] O.Vyaselev: "Lattice Distortion and First Order Transition in TlCuCl_3"Proceedings of Japanese-French Seminar. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Kodama: "Cu NMR Observation of the Dimer Singlet State in the Quasi-Two-Dimensional Spin System SrCu_2(BO_3)_2"Proceedings of Japanese -French Seminar. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 0.Vyaselev: "Cd and Re NMR/NQR in Pyrochlore Compound Cd_2Re_2O_7"J. Phys. Chem. Solids. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S.Fujiyama: "NMR observation of charge fluctuations in quasi-one-dimesional cuprates"J. Phys. Chem. Solids. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] N.Shishiuchi: "Defect-induced magnetic fluctuations in YbB_<12>"J. Phys. Chem. Solids. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K.Kodama: "Cu nuclear spin-spin coupling in the dimmer singlet state in SrCu_2(BO_3)_2"J. Phys. : Condens. Matter. (印刷中).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Ueda: "Vanadium Family as Spin-Gap Systems"Chem. Mater.. 10. 2653-2664 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Fujiyama: "Nuclear spin-spin coupling in La_<2-x>Sr_xCuO_4, studied by stimulated echo decay"Phys. Rev.. B60. 9801-9809 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Ikushima: "^<171>Yb NMR in the Kondo semiconductor YbB_<12>"Physica. B281&282. 274-275 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Fujiyama: "Low energy spin excitations in Sr_<14-x>Ca_xCu_<24>O_<41>"Physica. C341-348. 461-462 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Fujiyama: "Spin Correlations in Hole-Doped Ladder Cuprates"J. Phys. Soc. Jpn.. 69 (Suppl. B). 46-53 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Ueda: "Low-Dimensional Vanadium Okides"J. Phys. Soc. Jpn.. 69 (Suppl. B). 146-154 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Fujiyama: "Nuclear Spin Relaxation in Hole-Doped Two-Leg Ladders"J. Phys. Soc. Jpn.. 69. 1610-1613 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] J. P. Boucher: "Possible localized modes in the uniform quantum Heisenberg chains of Sr_2CuO_3"Phys. Rev.. B62. 367-371 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Z. Hiroi: "Spin-1/2 Kagome-Like Lattice in Volborthite Cu_3V_20_7(OH)_2 2H_20"J. Phys. Soc. Jpn.. 710. 3377-3384 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] D. Akahoshi: "Oxygen Nonstoichiometry, Structures, and Physical Properties of Yb_aC_2aC_<5+x>(0.00【less than or equal】λ【less than or equal】0.52)"J. Solid State Chem.. 156. 355-363 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Ohwada: "Devil's Staicase-Type Phase Transition in NaV_20_5 under High Pressure"Phys. Rev. Lett.. 87. 086402-1-4 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Masashi Takigawa: "The Mott transition and magnetic correlations"Butsuri. 54 (in Japanese). 90-97 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Shigeki Fujiyama: "Cu and O NMR in Sr_<14-x>Ca_xCu_<24>O_<41>"Bussei-kenkyu. 72 (in Japanese). 466-469 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Katsuaki Kodama: "NMR in the two-dimensional spin-gap material SrCu_2(BO_3)_2"Bussei-kenkyu. 76 (in Japansese). 516-525 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Zenji Hiroi: "The pyrochlore superconductor Cd_2Re_2O_7"Kotaibutsuri. 37 (in Japanese). 253-264 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] O. Vyaselev: "Lattice Distortion and First Order Transition in TlCuCl_3"Proceedings of Japanese-French Seminar. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] K. Kodama: "Cu NMR Observation of the Dimer Singlet State in the Quasi-Twi-Dimensional Spin System SrCu_2(BO_3)_2"Proceedings of Japanese-French Seminar. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] 0. Vyaselev: "Cd and Re NMR/NQR in Pyrochlore Compound Cd_2Re_2O_7"J. Phys. Chem. Solids. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] S. Fujiyama: "NMR observation of charge fluctuations in quasi-one-dimesional cuprates"J. Phys. Chem. Solids. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Shigeki FUJIYAMA: "Nuclear Spin Relaxation in Hole-Doped Two-Leg Ladders"J.Phys.Soc.Japan. 69.No 6. 1610-1613 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Shigeki FUJIYAMA: "Spin Correlations in Hole-Doped Ladder Cuprates"J.Phys.Soc.Japan. 69.Suppl.B. 46-53 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] 藤山 茂樹: "Nuclear spin-spin coupling in La_2-xSrxCuO_4 studies by stimulated echo decay"The Physical Review B. 60・13. 9801-9809 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 藤山 茂樹: "Spin Correlations in Hole-Doped Ladder Compounds"Journal of the Physical of Japan Supplement B. (予定). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] 陰山 洋: "Exact Dimen Ground State and Quantized Magnelization Plateaus in the Two-Dimensional Spin System SrCn_2(Bo_3)_2"The Physical Review Letters. 82・15. 3168-3171 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 藤原 直樹: "Spin Fluctuation neaby Magnetically Unstable Li_<1-X>Zn_XV_2O_4"The Physical Review B. 59. 6294-6300 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 瀧川仁: "モット転移と磁気相関" 日本物理学会誌. 54・2. 90-98 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] 藤原直樹: "Evidence of finite-size effect in an S=1/2 linear chain LiV_2O_5 studied by s'V NMR" The Physical Review B. 58・17. 11134-11137 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 〓山洋: "Spin-Singlet Ground State and Quantized Magnetization Plateaus in the Two Dimensional Spin System SrCu_2(BO_3)_2" The Physical Review Letters. 発表予定. ((1999))

    • Related Report
      1998 Annual Research Report
  • [Publications] 〓山洋: "Magnetic Anisotropy of SrCu_2(BO_3)_2 with a Two-Dimensional Orthogonal Dimer Lattice" Journal of the Physical Society of Japan. 67・12. 4304-4305 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 上田〓: "Magnetic Properties of AV_2O_5 (A=Li, Na, Cs, Ca and Mg)" Journal of Magnetism and Magnetic Materials. 177-181. 741-742 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] N.E.Hussey: "Magnetic field induced dimensional crossover in the normal state of YBa_2Cu_4O_8" The Physical Review Letters. 80・13. 2909-2912 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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