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Synthesis and Orbital structure of structure- and valence-controlled layered manganites

Research Project

Project/Area Number 10440091
Research Category

Grant-in-Aid for Scientific Research (B).

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionNagoya University

Principal Investigator

NAKAMURA Arao  Nagoya University, Center for Integrated Research of Science and Engineering, Prof., 理工科学総合研究センター, 教授 (50159068)

Co-Investigator(Kenkyū-buntansha) ICHIDA Masao  Nagoya University, Center for Integrated Research of Science and Engineering, Assistant Prof., 理工科学総合研究センター, 助手 (30260590)
MORITOMO Yutaka  Nagoya University, Center for Integrated Research of Science and Engineering, Associated Prof., 理工科学総合研究センター, 助教授 (00283466)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥15,200,000 (Direct Cost: ¥15,200,000)
Fiscal Year 2000: ¥1,600,000 (Direct Cost: ¥1,600,000)
Fiscal Year 1999: ¥5,500,000 (Direct Cost: ¥5,500,000)
Fiscal Year 1998: ¥8,100,000 (Direct Cost: ¥8,100,000)
Keywordsperovskite manganites / photoinduced phase transition / double exchange system / ferromagnetic phase transition / ultrafasst laser spectroscopy / half-metal / 超高速レーザー分光 / ペルプスカイト型酸化物 / 電荷移動遷移 / ヤーンテラーポーラロン / ペルブスカイト型酸化物 / スモールポーラロン
Research Abstract

We have systematically investigated electric, magnetic and optical properties of structure- and valencecontrolled manganites which show photoinduced magnetic transitions. The following is a major result.
1. The temperature variations of the resistivity and specific heat have been measured for prototypical half-metallic ferromagnets R_<0.6>Sr_<0.4>MnO_3 by controlling the one-electron band width. We have observed the T^3 dependence of the resistivity which is interpreted in terms of the anomalous single-magnon scattering process in the half-metallic system.
2. Photoinduced spin disorder and its dynamical behavior have been investigated for La_<0.7>Ca_<0.3>MnO_3. By optical injection of down-spin electrons into the Mn e_g orbital the spin disorder in the ferromagnetic phase is induced. We have found that the recovery time to the spin ordered state is lengthened from 30 ns at 5 K to 30 μs when the temperature approaches to the critical temperature of the phase transition. This result clearly demonstrates the critical slowing down of relaxation time in the phase transition.
3. Photoinduced resistivity change in a La_<0.6>Ca_<0.4>MnO_3 film has been investigated with variation of the excitation photon energy and temperature. The magnitude of the photoinduced resistivity change steeply decreases with increasing temperature above the transition temperature of 315 K.Since the photoinduced signal is enhanced by injection of the down spin carriers, the resistivity change is ascribed to the photoinduced spin disorder in the ferromagnetic metallic state. This result indicates that one can detect photoinduced spin disorder with the resistivity signal.

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (29 results)

All Other

All Publications (29 results)

  • [Publications] T.Akimoto, et al.: "Orbital stability in the spin-ordered phase of bilayer manganites as nvestigated by neutron-diffraction measurements"Phys.Rev.B. 61. 11270-11273 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] X.J.Liu, et al.: "Room-temperature photoswitching in La_<0.6>Sr_<0.4>MnO_3 film"Jpn.J.Appl.Phys.. 39. 670-672 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] A.Machida, et al.: "Reconsideration of the lattice effect on the charge-ordering transition of doped manganites"Phys.Rev.B. 62. 80-83 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] A.Machida, et al.: "Phase separationand insulator-metal behavior of doped manganites"Phys.Rev.B. 62. 3883-3887 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] X.J.Liu, et al.: "Photoinduced resistivity change due to spin-disorder in a manganite film"Jpn.J.Appl.Phys.. 39. L1233-L1235 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Akimoto, et al.: "Observation of anomalous single magnon scattering in half-metallic ferromagnets by chemical pressure control"Phsy.Rev.Lett.. 85. 3914-3917 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Akimoto, et al.: "Orbital stability in the spin-ordered phase of bilayer manganites as investigated by neutron-diffraction measurements"Phys.Rev.B. 61. 11270-11273 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] X.Liu, et al.: "Room-temperature photoswitching in La_<0.6>Sr_<0.4>MnO_3 film"Jpn.J.Appl.Phys.. 39. 670-672 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] A.Machida, et al.: "Reconsideration of the lattice effect on the charge-ordering transition of doped manganites"Phys.Rev.B. 62. 80-83 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] A.Machida, et al.: "Phase separation and insulator-metal behavior of doped manganites"Phys.Rev.B. 62. 3883-3887 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] X.Liu, et al.: "Photoinduced resistivity change due to spin-disorder in a manganite film"Jpn.J.Appl.Phys.. 39. L1233-L1235 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Akimoto, et al.: "Observation of anomalous single magnon scattering in half-metallic ferromagnets by chemical pressure control"Phys.Rev.Lett.. 85. 3914-3917 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Akimoto, et al.: "Orbital stability in the spin-ordered phase of bilayer manganites as investigated by neutron-diffraction measurements"Phys.Rev.B. 61. 11270-11273 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] X.J.Liu, et al.: "Room-temperature photo-switching in La_<0.6>Sr_<0.4>MnO_3 film"Jpn.J.Appl.Phys.. 39. 670-672 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] A.Machida, et al.: "Reconsideration of the lattice effect on the charge-ordering transition of doped manganites"Phys.Rev.B. 62. 80-83 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] A.Machida, et al.: "Phase separation and insulator-metal behavior of doped manganites"Phys.Rev.B. 62. 3883-3887 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] X.J.Liu, et al.: "Photoinduced resistivity change due to spin-disorder in a manganite film"Jpn.J.Appl.Phys.. 39. L1233-L1235 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Akimoto, et al.: "Observation of anomalous single magnon scattering in half-metallic ferromagnets by chemical pressure control"Phys.Rev.Lett.. 85. 3914-3917 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Moritomo 他: "Layered antiferromagnetic state in (Nd_<1-z>La_z)Sr_2Mn_3O_7"Journal of the Physical Society of Japan. 68(2). 631-636 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Akimoto 他: "Interrelation between orbital polarization and magnetic structure in bilayer manganites"Physical Review B. 59(22). R14153-R14156 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Takenaka 他: "Optical reflectivity spectra measured on cleaved surfaces of La_<1-x>Sr_xMnO_3: Evidence against extremely small Drude weight"Journal of the Physical Society of Japan. 68(6). 1828-1831 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Takenaka 他: "Optical spectra measured on cleaved surfaces of double-exchange ferromagnetic La_<1-x>Sr_xMnO_3"Physica Status Solidi(b). 215. 637-641 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Moritomo 他: "Electronic phase diagram and phase separation in Cr-doped manganites"Physical Review B. 60(13). 9223 (9220)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Moritomo 他: "Layered-Type Antiferromagnetic State in Double-Layered Manganities:(Lal-zNdz)2-2xSr1+2xMn207" Jounal of the Physical Society of Japan. 67. 405-408 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Akimoto 他: "Antiferromagnetic metallic state in doped manganites" Phys.Rev.B. 57. R5594-5597 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] Y.Moritomo 他: "Antiferromagnetic metallic state in the heavily doped region of perovskite magnites" Phys.Rev.B. 58. 5544-5549 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Matsuba: "Photoinduced demagnetization and its dynamical behavior in a (Nd_<0.5>Sm_<0.5>)_<0.4>Sr_<0.4>MnO_3 thin film" Phys.Rev.B. 58. R4203-4206 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] M.Ichida: "Femtosecond response of optical constants due to charge-transfer excitations in Nd_3CuO_4" Solid States Communications. 108. 145-149 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] A.Machida 他: "Temperatue evolution of the 1.5-eV absorption band in doped manganites: Formation of John-Teller clusters" Phys.Rev.B. 58. 12540-12542 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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