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Local Non-Fermi-Liquid Anomaly and Inter-Site Effects of 5f Electron Systems

Research Project

Project/Area Number 10440096
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionHOKKAIDO UNIVERSITY

Principal Investigator

AMITSUKA Hiroshi  Hokkaido University, Graduate School of Science, Lecturer, 大学院・理学研究科, 講師 (40212576)

Co-Investigator(Kenkyū-buntansha) TENYA Kenichi  Hokkaido University, Graduate School of Science, Instructor, 大学院・理学研究科, 助手 (70261279)
Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥5,500,000 (Direct Cost: ¥5,500,000)
Fiscal Year 1999: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1998: ¥5,000,000 (Direct Cost: ¥5,000,000)
KeywordsNon Fermi Liquid / Kondo Effects / Multi-Channel Kondo Effects / Non-Kramers Configuration / Heavy Fermion / Weak Antiferromagnetism / Pressure Effects / Neutron Scattering / ウラン希薄合金 / 非クラマース電子系 / 比熱 / 電気抵抗
Research Abstract

Single-U-ion properties of heavy-electron compound URuィイD22ィエD2SiィイD22ィエD2 have been investigated by a series of diluting experiments on RィイD21-xィエD2UィイD2xィエD2RuィイD22ィエD2SiィイD22ィエD2(R=Y, Th; x 【less than or equal】0.07). A strong uniaxial magnetic anisotropy of local 5f moments is commonly observed throughout the dilutions. From a large enhancement of Χ and C/T at T → 0, we suggest a non-Kramers, magnetic doublet ΓィイD25ィエD2 (fィイD12ィエD1) to be eminently suitable for the crystal-field lowest level, contrary to general views of low-lying singlets for the periodic system. We have further confirmed absence of the conventional Kondo effect in all these dilutions. A strong suppression of 5f moments at low temperatures accompanies a non-trivial lnT decrease in ρ and a small change in the magnetic entropy. Specific-heat measurements in magnetic fields up to 12 T have revealed no sign of the residual entropy, eliminating the simple application of the two-channel Kondo theory to the present alloys. We have also found through neutron-scattering experiments that the periodic system URuィイD22ィエD2SiィイD22ィエD2 undergoes a new phase transition under high pressure.

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (42 results)

All Other

All Publications (42 results)

  • [Publications] T.Honma: "Incommensurate-Commensurate Magnetic Phase Transitions of the Ising-5f System UPd_2Si_2 : the H-T Phase Diagram and Mean-Field Analysis"J.Phys.Soc.Jpn.. 67. 1017-1028 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J.-G.Park: "Thermal Hysteresis in Magnetization of Single-Crystal URu_2Si_2"J.Magn.& Magn.Mater.. 177-181. 455-456 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Amitsuka: "Magnetic Properties of Dilute Uranium Alloys Y_<1-X> UxRu_2Si_2 (X【less than or equal】0.07)"JJAP Series. 11. 145-147 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Sato: "Hall Effect and Thermoelectric Power in the Systems Exhibiting the Non-Fermi Liquid Behaviors"Physica B. 259-261. 390-391 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Amitsuka: "Anomalous Transport Properties of Dilute Uranium Alloys R_<1-X>UxRu_2Si_2 (R=Th, YiX【less than or equal】0.07)"Physica B. 259-261. 412-414 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Tenya: "Magnetization Study of Superconductivity in Upt_3 and CeRu_2"JJAP Series. 11. 53-55 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Amitsuka: "Effect of Pressure on Ting Antiferromagnetic Moment in the Heavy-Electron Compound URu_2Si_2"Phys.Rev.Lett.. 83. 5114-5117 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M.Yokoyama: "Unusual Low Temperature Behavior of the Dilute Uranium Alloys La_<1-X>UxRu_2Si_2 (X【less than or equal】0.07)"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Amitsuka: "Non-Fermi-Liquid Behavior in R_<1-X>UxRu_2Si_2 (R=Th, Y.and La ; X【less than or equal】0.07)"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] N.Metoki: "Neutron-Scattering Studies on Heavy-Fermion Superconductors"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T.Honma: "Magnetic, Elastic, Transport and Fermi Surface Properties of a Ferromagnetic Compound UGa_2"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Kuwahara: "Elastic Constants of URu_2Si_2 in Magnetic Fields"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K.Tenya: "Magnetization Study in the Superconducting Mixed State of URu_2Si_2"Physica B. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Amitsuka: "Pressure-Inoluced Magnetic Phase Transition of the 5f Electronic System URu_2Si_2"J.Phys.Soc.Jpn.. (印刷中). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Honma: "Incommensurate-Commensurate Magnetic Phase Transitions of the Ising-5f System UpdィイD22ィエD2SiィイD22ィエD2 : the H-T Phase Diagram and Mean-Field Analysis"J. Phys. Soc. Jpn.. 67. 1017-1028 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] J.-G. Park: "Thermal Hysteresis in Magnetization of Single-Crystal UruィイD22ィエD2SiィイD22ィエD2"J. Magn. & Magn. Mater.. 177-181. 455-456 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Magnetic Properties of Dilute Uranium Alloys YィイD21-xィエD2UィイD2xィエD2RuィイD22ィエD2SiィイD22ィエD2 (x【less than or equal】0.07)"JJAP Series. 11. 145-147 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Sato: "Hall Effect and Thermoelectric Power in the Systems Exhibiting the Non-Fermi Liquid Behaviors"Physica. 259-261. 390-391 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Anomalous Transport Properties of Dilute Uranium RィイD21-xィエD2UィイD2xィエD2RuィイD22ィエD2SiィイD22ィエD2 (R = Th, Y ; x【less than or equal】0.07)"Physica. 259-261. 412-414 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Tenya: "Magnetization Study of Superconductivity in UptィイD23ィエD2 and CeRuィイD22ィエD2"JJAP Series. 11. 53-55 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound UruィイD22ィエD2SiィイD22ィエD2"Phys. Rev. Lett.. 83. 5114-5117 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Non-Fermi-Liquid Behavior in RィイD21-xィエD2UィイD2xィエD2RuィイD22ィエD2SiィイD22ィエD2 (R = Th, Y ; x【less than or equal】0.07)"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Yokoyama: "Unusual Low Temperature Behavior of the Dilute Uranium Alloys LaィイD21-xィエD2UィイD2xィエD2RuィイD22ィエD2SiィイD22ィエD2 (x【less than or equal】0.07)"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] N. Metoki: "Neutron-Scattering Studies on Heavy-Fermion Superconductors"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Honma: "Magnetic, Elastic, Transport and Fermi Surface Properties of a Ferromagnetic Compound UgaィイD22ィエD2"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Kuwahara: "Elastic Constants of URu2Si2 in Magnetic Fields"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Tenya: "Magnetization Study in the Superconducting Mixed State of UruィイD22ィエD2SiィイD22ィエD2"Physica B. (in press). (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Pressure-Induced Magnetic Phase Transition of the 5f Electron System UruィイD22ィエD2SiィイD22ィエD2"to be published in J. Phys. Soc. Jpn.. (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Amitsuka: "Magnetic Properties of Dilute Uranium Alloys Y_<1-x>Li_xRu_2Si_2(x【less than or equal】0.07)"JJAP Series. 11. 145-147 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Sato: "Hall Effect and Thermoelectric Power in the Systems Exhibiting the Non-Fermi Liquid Behaviors"Physica B. 259-261. 390-391 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Amitsuka: "Anomalous Transport Properties of Dilute Uranium Alloys R_<1-x>U_xRu_2Si _2 (R=Th, Y ; x【less than or equal】0.07)"Physica B. 259-261. 412-414 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K. Tenya: "Magnetization Study of Superconductivity in Upt_3 and CeRu_2"JJAP Series. 11. 53-55 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Amitsuka: "Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu_2Si_2"Phys .Rev. Lett.. 83. 5114-5117 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M. Yokoyama: "Unusual Low Temperature Behavior of the Dilute Uranium Alloys La_<1-x>U_xRu_2Si_2(x【less than or equal】0.07)"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Amitsuka: "Non-Fermi-Liquid Behavior in R_<1-x>U_xRu_2Si_2 (R=Th, Y and La ; x【less than or equal】0.07)"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] N. Metoki: "Neutron-Scattering Studies on Heavy-Fermion Superconductors"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] T. Honma: "Magnetic, Elastic, Transport and Fermi Surface Properties of a Ferromagnetic compound UGa_2"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] K. Kuwahara: "Elastic Constants of URu_2Si _2 in Magnetic Fields"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] K. Tenya: "Magnetization Study in the Superconducting Mixed State of URu_2Si_2"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Amitsuka: "Pressure-Induced Magnetic Phase Transition of the 5f Electron System URu_2Si_2"J.Phys.Soc.Jpn.. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Amitsuka: "Magnetic Properties of Dilute Uranium Alloys Y_<1-x>U_xRu_2Si_2(x【less than or equal】0.07)" JJAP Series. 11. 145-147 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Amitsuka: "Anomalous Transport Properties of Dilute Uranium Alloys R_<1-x>U_xRu_2Si_2(R=Th,Y;x【less than or equal】0.07)" Physica B. (出版予定).

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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