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Experimental Study on Nuclear Data Measurements of Actinide Nuclides in the Resonance Neutron Energy Region

Research Project

Project/Area Number 10480119
Research Category

Grant-in-Aid for Scientific Research (B).

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

KOBAYASHI Katsuhei  Kyoto Univ., Res. Reactor Inst., Associate Prof., 原子炉実験所, 助教授 (80027466)

Co-Investigator(Kenkyū-buntansha) MITSUGASHIRA Toshiaki  Tohoku Univ., Inst. for Material Res., Associate Prof., 金属材料研究所, 助教授 (30005938)
HAJIMU Yamana  Kyoto Univ., Res. Reactor Inst., Associate Prof., 原子炉実験所, 助教授 (30283683)
MORIYAMA Hirotake  Kyoto Univ., Res. Reactor Inst., Professor, 原子炉実験所, 教授 (90127150)
木村 逸郎  京都大学, 大学院・工学研究科, 教授 (40027404)
Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥9,000,000 (Direct Cost: ¥9,000,000)
Fiscal Year 2000: ¥2,500,000 (Direct Cost: ¥2,500,000)
Fiscal Year 1999: ¥1,900,000 (Direct Cost: ¥1,900,000)
Fiscal Year 1998: ¥4,600,000 (Direct Cost: ¥4,600,000)
KeywordsLead Slowing-down Spectrometer / Actinide Nuclides / Chemical Purification Samples / ^<243>An (n, f) Reaction Cross Section / ^<231>Pa (n, f) Reaction Cross Section / ^<229>Th (n, f) Reaction Cross Section / ^<230>Th (n, f) Reaction Cross Section / Double Fission Chambers / ^<237>Np (n, γ)Reaction Cross Section / Prompt Capture Gamma Mcasurements / C_6D_6 Liquid Scintillator / Ar-gas Proportional Counter / 共鳴中性子領域 / Th-229核分裂断面積 / Th-230核分裂断面積 / Np-237中性子捕獲断面積 / 飛行時間分析法 / ENDF / B-VI / JENDL-3.2 / アルゴンガス入り比例計数管 / C6D6シンチレータ / 背中合わせ型核分裂電離箱 / Am-243(n,f)反応断面積 / Am-242m(n,f)反応断面積
Research Abstract

The present status of nuclear data for actinide nuclides, Am-243, Pa-231, Th-229, Th-230 and Np-237, has been reviewed. Making use of the Kyoto University Lead slowing-down Spectrometer (KULS) coupled to a 46 MeV electron linear accelerator (linac) of the Kyoto University Research Reactor Institute (KURRI), the fission cross sections of Am-243, Pa-231, Th-229 and Th-230 and the capture cross section of Np-237 have been measured below 10 keV.A back-to-back type double fission chamber has been applied to the fission cross section measurement. An Ar-gas proportional counter for the capture gamma-ray measurement and a BF_3 proportional counter for the neutron flux/spectrum monitor have been used for the Np-237 capture cross section measurement. In this case, after the self-shielding correction in the Np-237 sample has been made, the relative measurement has been normalized to a reference cross section value in the lower energy region. By comparing with each of the results obtained, the existing experimental and evaluated data have been investigated. We could supply new data which had not been measured before in some nuclide/energy region.
The capture cross section of Np-237 has been also measured with a 12 m flight path and the linac time-of-flight (TOF) method below 10 keV relative to the ^<10>B(n, α) reaction using a pair of C_6D_6 liquid scintillation detectors. After the self-shielding correction for the Np-237 sample, the cross section has been normalized at 0.0253 eV to the reference value of 181 b. The previous data have been investigated by comparing with the present measurement. The KULS measurement for the ^<237>Np(n, γ)^<238>Np reaction has been compared with the result obtained by energy-broadening the TOF data. General agreement can be seen between them, although some small discrepancies are observed in the big resonance region.

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (27 results)

All Other

All Publications (27 results)

  • [Publications] K.Kobayashi et al.,: "Measurements of Neutron-induced Fission Cross Section of Am-243 from Thermal Neutron Energy to 15 keV Using Lead Slowing-down Spectrometer and Thermal Neutron Facility"J.Nucl.Sci.Technol.. 36. 20-28 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.,: "Measurements of Neutron-induced Fission Cross Section of Pa-231 from 0.1 eV to 10 keV with Lead Slowing-down Spectrometer and at 0.0253 eV with Thermal Neutron Facility"J.Nucl.Sci.Technol.. 36. 549-551 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi: "MA Nuclear Data Measurements with Lead Slowing-down Spectrometer"Proc.of the 1999 Symp.on Nucl.Data,JAERI-Conf 2000-005. 26-31 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Fission Cross Section Measurements of Th-229 and Pa-231 Using Linac-driven Lead Slowing-down Spectrometer"Procof the Tenth Int'l Symp.on Reactor Dosimetry,ASTM STP-1398. 439-446 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Y.Lee,K.Kobayashi et al.: "Neutron Capture Cross Section Measurement of Np-237 below 10 keV by Linac Time-of-Flight Method"Proc.of the 2000 Symp.on Nucl.Data,JAERI-Conf. (印刷中). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Measurement of Neutron-induced Fission Cross Sections of ^<221>Th and ^<231>Pa Using Linac-driven Lead Slowing-down Spectrometer"Nucl.Sci.Eng.. (印刷中). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Measurements of Neutron-induced Fission Cross Section of Am-243 from Thermal Neutron Energy to 15 keV Using Lead Slowing-down Spectrometer and Thermal Neutron Facility"J.Nucl. Sci. Technol.. 36(1). 20-28 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Measurements of Neutron-induced Fission Cross Section of Pa-231 from 0.1 eV to 10 keV with Lead Slowing-down Spectrometer and at 0.0253 eV with Thermal Neutron Facility"J.Nucl. Sci. Technol.. 36(6). 549-551 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "MA Nuclear Data Measurements with Lead Slowing-down Spectrometer"Proc. of the 1999 Symp. on Nucl. Data, JAERI-Conf. 2000-005. 26-31 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Fission Cross Section Measurements of Th-229 and Pa-231 Using Linac-driven Lead Slowing-down Spectrometer"Proc of the Tenth Int'1 Symp. on Reactor Dosimetry, Osaka. ASTM STP-1398. 439-446 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Lee, K.Kobayashi et al.: "Neutron Capture Cross SectionMeasurement of Np-237 below 10 keV by Linac Time-of-Flight Method"Proc. of the 2000 Symp. on Nucl. Data, JAERI-Conf. (in print.).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Kobayashi et al.: "Measurement of Neutron-induced Fission Cross Sections of 229Th and 231Pa Using Linac-driven Lead Slowing-down Spectrometer"Nucl. Sci. Eng.. (in print.).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 小林捷平,山名元: "Measurements of Neutron-induced Fission Cross Section of Americium-243 from Thermal Neutron Energy to 15 keV Using Lead Slowing-down Spectrometer and Thermal Neutron Facility"J.Nucl.Sci.Technol.. 36・1. 20-28 (1999)

    • Related Report
      2000 Annual Research Report
  • [Publications] 小林捷平,山名元,三頭聡明: "Fission Cross Section Measurements of Th-229 and Pa-231 Using Linac-Driven Lead Slowing-Down Spectrometer"Proc.of the Tenth Int'l Symp.on Reactor Dosimetry, Held at Osaka, Sept.12-Sept.17,1999,Edited by J.G.Williams,D.W.Vehar,F.H.Ruddy and D.M.Gilliams, ASTM STP 1398,in print.. (印刷中). (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] 森山裕丈,山名元: "Analysis of Mononuclear Hydrolysis Constants of Actinide Ions by Hard Sphere Model"Radiochimica Acta. 87. 97-104 (1999)

    • Related Report
      2000 Annual Research Report
  • [Publications] 森山裕丈,山名元: "An Application of Actinide Elements for a Redox Flow Battery"J.Nucl.Sci.Tehenol.. 37. 253-256 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] 山名元,森山裕丈: "Distribution Equibrium of Lanthanides in the Liquid-Liquid extraction System of TBP and Molten Ca(NO_3)_2・4H_2O"Radiochimica Acta. 84. 191-200 (1999)

    • Related Report
      2000 Annual Research Report
  • [Publications] 山名元,森山裕丈: "Simultaneous Measurement of Prompt Neutrons and Fission Fragments for ^<239>Pu(n_<th>,f)"J.Nucl.Sci.Technol.. 37・11. 941-948 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Kobayashi 他: "Measurements of Neutron-induced Fission Cross Section of Americium-243 from Thermal Neutron Energy to 15 keV Using Lead Slowing-down Spectrometer and Thermal Neutron Facility"J. Nucl. Sci. Technol.. 36・1. 20-28 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kobayashi 他: "Measurements of Neutron-induced Fission Cross Section of Protactiniumu-231 from 0.1eV to 10keV with Lead Slowing-down Spectrometer and at 0.0253 eV with Thermal Neutron Facility"J. Nucl. Sci. Technol.. 36・6. 549-551 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Kai,K.Kobayashi 他: "Fission Cross Section Measurement for Am-242m with TOF Methods in Low Energy Region"Proc. Of the 1998 Symp. On Nucl. Data, JAERI-Conf 99-002. 240-245 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kobayashi 他: "Fission Cross Section Measurements of Th-229 and Pa-231 Using LINAC-Driven Lead Slowing-down Spectrometer"Proc.Of the 10 th Int'l Symp. On Reactor Dosimetry, STP-1398, ASTM. (To be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kobayashi 他: "Capture Cross Section Measurement of Np-237 below 1 keV with Lead Slowing-down Spectrometer"Proc. Of the 1999 Symp. On Nucl. Data, JAERI-Conf.. (To be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kobayashi: "MA Nuclear Data Measurement with Lead Slowing-down Spectrometers"Proc. Of the 1999 Symp. On Nucl. Data, JAERI-Conf.. (To be published). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Kobayashi他: "Measurements of Neutron-induced Fission Cross Section of Am-243 from Thermal Neutron Energy to 15 Key Using Lead Slowing-down Spectrometer and Thermal Neutron Facility" J.Necl.Sci,Technol.36・1. 20-28 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Kai,K.Kobayashi他: "Fission Cross Section Measurement for Am-242m with TOF Methods in Low Energy Region" Proc.of the 1998 Symp.on Nucl.Data,JAERI-Conf. (To be published). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Kobayashi他: "Measurement of Fission Cross Section of Pa-231 using Lead Slowing-down Spectrometer" Proc.of the 1998 Symp.on Nucl.Data,JAERI-Conf. (To be published). (1999)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2016-04-21  

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