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Application of ultrafast optical technique to the time-domain X-ray spectroscopy using short-pulse characteristics of laser and synchrotron radiation

Research Project

Project/Area Number 10554032
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section展開研究
Research Field Physical chemistry
Research InstitutionHimeji Institute of Technology

Principal Investigator

TAKAGI Yoshihiro  Himeji Institute of Technology, Department of Material Science, Professor, 理学部・物質化学科, 教授 (80106161)

Co-Investigator(Kenkyū-buntansha) ADACHI Satoru  Himeji Institute of Technology, Department of Material Science, Research Associate, 理学部・物質化学科, 助手 (10221722)
Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥10,900,000 (Direct Cost: ¥10,900,000)
Fiscal Year 1999: ¥2,400,000 (Direct Cost: ¥2,400,000)
Fiscal Year 1998: ¥8,500,000 (Direct Cost: ¥8,500,000)
Keywordsultrashort pulsed laser / sampling / pump-probe / synchrotron radiation / フェムト秒レーザー / ポンプ・プローブ分光 / 時間分解分光法
Research Abstract

We have developed a subpicosecond non-degenerate pump-probe spectrometer based on the optical sampling technique using a combination of asynchronous tunable femtosecond lasers. Owing to its simple instrumentation time evolution of subpicosecond to nanosecond excited molecular processes in solution and of exciton relaxation processes in semiconductor multiple quantum wells has been detected on an oscilloscope by an effective time base magnification of 760,000 times. Fast acquisition of the temporal profiles and ease of wavelength scanning allowed compilation of time-resolved absorption and excitation spectra. A possible extention of the spectrometer with one of the light sources being a synchrotron radiation instead of the femtosecond laser is discussed.

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (14 results)

All Other

All Publications (14 results)

  • [Publications] S. Adachi and Y. Takagi: "Exciton spin concept or separate-particle spin concept in spin relaxation process of excitons?"Phys. of Low-Dim. Struct.. 1/2. 133-142 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Takeyama, Y. Takagi, T. Karasawa, V. F. Aguekian: "Exciton magnetic polaron localization dynamics in bulk Cd1-xMnxTe"J. of Crys. Growth. 184-185. 917-920 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Takeyama, S. Adachi, Y. Takagi, G. Karczewski, T. Wojtowicz, J. Kossut, T. Karasawa: "Phot-induced magnetic polarons in low-dimensional dilute magnetic semi-conductors"Materials Science and Engineering. B63. 111-118 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. Takagi, S. Adachi: "Subpicosecond optica sampling spectrometer using asynchronous tunable mode-locked laser"Rev. Sci. Instrum.. 70. 2218-2224 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Acachi, Y. Takagi, J. Takeda, K. A. Nelson: "Optical sampling four-wave mixing experiment for exciton relaxation processes"Opt. Commun.. 174. 291-298 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] V. Kubecek, H. Jelinkova, T. Takagi, A. Agnesi, and M. R. Kokta: "Continuously pumped Cr : YAG laser"Proc. of SPIE. 4016. 354-359 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 高木芳弘: "計算機分光学の原点"時潮社. 16 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 高木芳弘: "非線形分光 「光と化学の事典」"丸善 (出版予定). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y.Takagi,and S.Adachi: "Subpicosecond optical sampling spectrometer using asynchronous tunable mode-locked lasers"Rev.Sci.Instrum.. vol.70-5. 2218-2224 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Adachi,Y.Takagi,J.Takeda,K.A.Nelson: "Optical sampling four-wave-mixing experiment for ex citon relaxation"Opt.Commun.. Vol.174. 291-298 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Takeyama,S.Adachi,Y.Takagi,G.Karczewski: "Photo-induced magnetic polarons in low-dimensional dilute magnetic semiconductors"Materials Science and Engineering. Vol.B63. 111-118 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Takagi,and S.Adachi: "Subpicosecond optical sampling spectrometer using asynchronous tunable mode-locked lasers" Rev.Sci.Instrum.70-5(in print). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] S.Adachi and Y.Takagi: "Exciton spin concept or separate-particle spin concept in spin dynamical processes of excitons?" Phys.Low-Dim.Struct.1/2. 133-142 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] 高木芳弘: "計算機分光学の原点" 時潮社, 189 (1999)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2016-04-21  

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