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Quantum Monte Carlo Study on Excitonic Complexes in Quantum Structures

Research Project

Project/Area Number 10640303
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionJapan Advanced Institute of Science and Technology

Principal Investigator

TSUCHIYA Takuma  School of Materials Science, Japan Advanced Institute of Science Research Associate, 材料科学研究科, 助手 (40262597)

Project Period (FY) 1998 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2000: ¥500,000 (Direct Cost: ¥500,000)
Fiscal Year 1999: ¥1,100,000 (Direct Cost: ¥1,100,000)
Fiscal Year 1998: ¥1,800,000 (Direct Cost: ¥1,800,000)
Keywordsexcitonic molecules / charged excitons / binding energy / quantum structure / diffusion Monte Carlo / GaAs / CdTe / excitons / 量子細線 / タイプII超格子 / 励起子高分子 / 量子モンテカルロ法 / 量子ドット / 荷量励起子 / CuCl / 量子井戸 / 半導体超格子
Research Abstract

In this research project, we have successfully investigated properties of excitonic complexes or excitons, excitonic molecules, and charged excitons in various quantum structures, using the diffusion Monte Carlo method. This method gives us exact binding energies within a small statistical error under the effective mass approximation and is applicable to any complicated confinement potentials. We have obtained the following results :
1. GaAs/AlGaAs type-I quantum wells
We have found that the biexcitonic binding energies are almost twice of those by variational method. The binding energies for positively charged excitons are smaller than those of biexcitons, and those of negatively charged excitons are smaller than negatively charged ones. For quantum wells narrower than 100 A, the roughness of the heterointerfaces causes lateral confinement of excitonic complexes and resulting strong enhancement of binding energies. This enhancement is observed in recent experiments, and our theoretical … More results reproduce the experimental ones quite well.
2. Quantum dots
It has been found that the binding energies can be negative or can increase strongly for relatively small dots. This comes from the electrostatic potential in a quantum dot resulting from the difference of confinement between an electron and a hole of an exciton in the dot.
3. GaAs/AlAs type-II superlattices
Because of the spatial separation between electron and holes, an exciton in type-II superlattices has dipole moment. Because of the dipole-dipole interaction between these excitons they can bind successively along the growth direction and form an excitonic polymer. The binding energy per excitons of 3 meV is expected.
4. Quantum wires
The properties of excitonie complexes in quantum wires are between those in quantum wells and quantum dots. As in quantum dots, the binding energies can be strongly enhanced, but they cannot be negative. This is because the distance between particles with a repulsive Coulomb interaction between them can be infinity. This means that we can prevent a formation of some kind of excitonic complexes by controlling confinement potentials. Less

Report

(4 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • 1998 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] T.Tsuchiya: "Binding Energies of Biexcitons and Charged Excitons in Quantum Wells : A Diffusion Monte Carlo Study"Proceedings of the 24th International Conference of Physics of Semiconductors. (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsuchiya: "Biexcitons and Charged Excitons in Quantum.Dots"Physica E. 7. 470-474 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsuchiya: "Biexcitons and Charged Excitons in GaAs/AlAs Type-II Super lattices"J.Lumin.. 87-89. 509-511 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsuchiya: "Diffusion Monte Carlo Study on Biexcitons and Charged Excitons in Semiconductor Quantum Structures"Prog.Theor.Phys.Suppl.. 138. 128-129 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsuchiya: "A Quantum Monte Carlo Study on Excitonic Conplexes in GaAs/AlGaAs Quantum Wires"J.Lumin.. (in press). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tsuchiya: "Possibility of Excitonic Polymers in Type-II Super lattices"Proceedings of the 25th International Conference of Physics of Semicanductors . (in press). (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya and S.Katayama: "A Quantum Monte Carlo Study on Excitonic Molecules in Quantum Wells"Solid State Electronics. 42. 1523-1526 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya and S.Katayama: "A Quantum Monte Carlo Study on Excitonic Molecules in Type-II Superlattices"Physica B. 249-251. 612-616 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "A Quantum Monte Carlo Study of Biexcitons and Charged Excitons in Quantum Wells"Extended Abstract of the 17th Electronic Materials Symposium. 171-172 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya and S.Katayama: "Binding Energy of Biexcitons and Charged Excitons in Quantum Wells : A Diffusion Monte Carlo Study"in Proceedings of the 24th International Conference on the Physics of Semiconductors. (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "Biexcitons and Charged Excitons in Quantum Dots : A Quantum Monte Carlo Study"Physica E. 1. 470-474 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "Biexcitons and Charged Excitons in GaAs/AlAs Type-II Superlattices : A Quantum Monte Carlo Study"Journal of Luminescence. 87-89. 509-511 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "Diffusion Monte Carlo Study on Biexcitons and Charged Excitons in Semiconductor Quantum Structures"Progress of Theoretical Physics Supplement. 138. 128-129 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "A Quantum Monte Carlo Study on Excitonic Complexes In GaAs/AlGaAs Quantum Wires"J.Lumin.. (in press). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Takuma Tsuchiya: "Possibility of Excitonic Polymers in Type-II Superlattices"in Proceedinos of the 25th International Conference on the Physics of Semiconductors. (in press). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 土家琢磨: "半導体量子構造における励起子複合体の量子モンテカルロ計算"固体物理. 35・1. 41-49 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Tsuchiya: "A quantum Monte Carlo study on excitonic complexes in GaAs/AlGaAs quantum wires"J Lumin. (印刷中).

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Tsuchiya: "Excitonic polymers in type-II superlattices"Proceedings of The 25th International Conference on the physics of semiconductors. (印刷中).

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Tsuchiya: "Biexcitons and Charged Excitons in Quantum Dots"Physica E. (印刷中).

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Tsuchiya: "Biexcitons and Charged Excitons in GaAs/AlAs type-II Superlattices"Journal of Luminescence. (印刷中).

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Tsuchiya: "Diffusion Monte Carlo Study on Biexcitons and Charged Excitons"Progress of Theoretical Physics,Supplement. (印刷中).

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Tsuchiya: "A quantum Monte Carlo stady on excitonic molecules in quantum wells" Solid-State Electronics. 42,7-8. 1523-1526 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Tsuchiya: "A quantum Monte Carlo stady on excitonic molecules in type-II superlattices" Physica B. 249-251. 612-616 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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