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Anomalous spin fluctuations new the Molt transition in manganites

Research Project

Project/Area Number 10640329
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionThe University of Tokyo, Institute for Solid State Physics

Principal Investigator

YOSHIZAWA Hideki  Institute for Solid State Physics, University of Tokyo, Associate Prof., 物性研究所, 助教授 (00174912)

Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 1999: ¥1,400,000 (Direct Cost: ¥1,400,000)
Fiscal Year 1998: ¥1,600,000 (Direct Cost: ¥1,600,000)
KeywordsNeutron diffraction / Colossal magnefoesistance / Charge ordering / 巨大磁気抵抗 / Mn酸化物 / 中性子散乱 / スピンダイナミクス
Research Abstract

The hole concentration dependence of the crystal and magnetic structures of the hole doped manganite systems have been studied systematically with use of neutron diffraction technique, and their phase diagrams have been determined. The studies on the spin dynamics further revealed that the spin fluctuation changes its nature from ferromagnetic correlations to antiferromagnetic correlations at and near the charge ordering transition temperature. We discovered that the spin ordering in the CE-type charge/spin ordered state is not a true long range order. The orbital degree of freedom gives rise to two domains of orbital ordering patterns, and reduces the spin correlation, in the CE-type order.

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (37 results)

All Other

All Publications (37 results)

  • [Publications] H. Yoshizawa: "Anisotropic spin waves in a metallic antiferromagnet Nd_<0.43>Sr_<0.55>MnO_3"Phys. Rev. B. 58. R571-574 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota: "Impact of La substitution on the magnetic structure of a low-carrier-density Kondo system: Ce_<0.9>La_<0.1>P"Phys. Rev. B. 58. R2929-2932 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] R. Kajimoto: "Anomalous ferromagnetic spin fluctuations in an antiferromagnetic insulator Pr_<1-x>Ca_xMnO_3"Phys. Rev. B. 58. R11837-11840 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Hirota: "Neutron-diffraction studies on the magnetic ordering process in the layer Mn perovskite La_<2-2x>Sr_<1+2x>Mn_2O_7"J. Phys. Soc. Jpn.. 67. 3380-3383 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Itoh: "Spin dynamics in two-dimensional percolating Heisenberg antiferromagnets"J. Phys. Soc. Jpn.. 67. 3610-3616 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota: "Interplay of the CE-type charge ordering and the A-type spin ordering in half-doped bilayer manganite"J. Phys. Soc. Jpn.. 68. 2202 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Katsufuji: "Commensurability effect on the charge ordering of La_<2-x>Sr_xNiO_4"Phys. Rev. B. 60. R5097-5100 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] R. Kajimoto: "Hole concentration induced transformation of the magnetic and orbital structure in Nd_<1-x>Sr_xMnO_3"Phys. Rev. B. 60. 9506-9517 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yoshizawa: "Spin order at low temperatures in La_<2-x>Sr_xNiO_4 with 0.289【less than or equal】 x 【less than or equal】 1/2"Phys. Rev. B. 61. R854-857 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yoshizawa: "Magnetic ordering and spin fluctuations in nearly half-doped manganites"Materials Science & Engineering B. 63. 125-132 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] R. Kajimoto: "Quasi-elastic ferromagnetic excitations in Nd_<1/2>Sr_<1/2>MnO_3"J. Phys. Chem. Solids. 60. 1177-1180 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota: "Neutron scattering studies on magnetic structure of couble-layered manganite La_<2-2x>Sr_<1+2x>Mn_2O_7 (0.30【less than or equal】 x 【less than or equal】 0.50)"J. Phys. Chem. Solids. 60. 1161-1164 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yoshizawa, H. Kawano, J. A. Fernandez-Baca, H. Kuwahara, and Y. Tokura,: "Anisotropic spin waves in metallic antiferromagnet NdィイD20.45ィエD2SrィイD20.55ィエD2MnOィイD23ィエD2"Phys. Rev. B. 58. R571-R574 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota, Y. Oohara, H. Yoshizawa, N. Mori. H. Takahashi, A. Uesawa, and T. Suzuki: "Impact of La substitution on the magnetic structure of a low-carrier-density Kondo system : CeィイD20.9ィエD2LaィイD20.1ィエD2P"Phys. Rev. B. 58. R2929-R2932 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] R. Kajimoto, T. Kakeshita, Y. Oohara, H. Yoshizawa. Y. Tomioka, and Y. Tokura: "Anomalous ferromagnetic spin fluctuations in an antiferromagnetic insulator PrィイD21-xィエD2CaィイD2xィエD2MnOィイD23ィエD2"Phys. Rev. B. 58. R11837-R11840 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Hirota. Y. Moritomo, H. Fujioka, M. Kubota, H. Yoshizawa, and Y. Endoh: "Neutron-diffraction studies on the magnetic ordering process in the layered Mn perovskite LaィイD22-2xィエD2SrィイD21+2xィエD2MnィイD22ィエD2OィイD27ィエD2"J. Phys. Soc. Jpn.. 67. 3380-3383 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] S. Itoh, H. Ikeda, H. Yoshizawa, M. J. Harris, and U. Steigenberger: "Spin dynamics in two-dimensional percolating Heisenberg antiferromagnets"J. Phys. Soc. Jpn. 67. 3610-3616 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota, H. Yoshizawa, Y. Moritomo, H. Fujioka, K. Hirota, and Y. Endoh: "Interplay of the CE-type charge ordering and the A-type spin ordering in half-doped bilayer manganite LaSrィイD22ィエD2MnィイD22ィエD2OィイD27ィエD2"J. Phys. Soc. Jpn.. 68. 2202-2205 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Katsufuji, T. Tanabe, Y. Tokura, T. Kakeshita, R. Kajimoto, and H. Yoshizawa: "Commensurability effect on the charge ordering of LaィイD22-xィエD2SrィイD2xィエD2NiOィイD24ィエD2"Phys. Rev. B. 60. R5097-R5100 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] R. Kajimoto, H. Yoshizawa, H. Kawano, H. Kuwahara, Y. Tokura, K. Ohoyama, and M. Ohashi: "Hole concentration induced transformation of the magnetic and orbital structure in NdィイD21-xィエD2SrィイD2xィエD2MnOィイD23ィエD2"Phys. Rev. B. 60. 9506-9517 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. Yoshizawa, T. Kakeshita, R. Kajimoto, T. Katsufuji, T. Tanabe, and Y. Tokura: "Spin order at low temperatures in LaィイD22-xィエD2SrィイD2xィエD2NiOィイD24ィエD2 with 0.289 < x < 1/2"Phys. Rev. B. 61. R854-R857 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] M. Kubota, H. Fujioka, K. Hirota, K. Ohoyama, Y. Moritomo, H. Yoshizawa, and Y. Endoh: "Relation between the crystal and magnetic structures of the layered manganite LaィイD22-2xィエD2SrィイD21+2xィエD2MnィイD22ィエD2OィイD27ィエD2 (0.30 < x < 0.50)"J. Phys. Soc. Jpn.. (submitted to).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Yoshizawa: "Anisotropic spin waves in a metallic antiferromagnet Nd_<0.45> Sr_<0.55> MnO_3"Phys.Rev.B. 58. R571-574 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kubota: "Impact of La substitution on the magnetic structure of a low-carrier-densitry kondo system: Ce_<ag> La_<ar>P"Phys.Rev.B. 58. R2929-2932 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] R.Kajimoto: "Anomalous ferromagnetic spin fluctuations in an antiferromagnetic insulator Pr_<1-x>C_<ax>MnO_3"Phys.Rev.B. 58. R11837-11840 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Hirota: "Neutron-diffraction studies on the magnetic ordering process in the layest Mn perovskite La_<2-2x> Sr_<1+2x> Mn_2 O_7"J.Phys.Soc.Jpn.. 67. 3380-3383 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Itoh: "Spin dynamics in two-dimonsinal percolating Heisenberg antiferromagnets"J.Phys.Soc.Jpn.. 67. 3610-3616 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kubota: "Interplay of the CE-type charge ordering and the A-type spin ordering in half-doped bilayer manganite"J.Phys.Soc.Jpn.. 68. 2202-2205 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Katsufuji: "Commensurability effect on the charge ordering of La_<2-x>Sr_xNiO_4"Phys.Rev.B. 60. R5097-5100 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] R.Kajimoto: "Hole concentration induced transformation of the magnetic and orbital structure in Nd_<1-x>Sr_xM_nO_3"Phys.Rev.B. 60. 9506-9517 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Yoshizawa: "Spin order at low temperatures in La_<2-x>Sr_xNiO_4 with 0.289【less than or similar】×【less than or similar】(1/2)"Phys.Rev.B. 61. R854-857 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Yoshizawa: "Magnetic ordering and spin fluctuations in nearly half-doped manganites"Materials Science & Engineering B. 63. 125-132 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] R.Kajimoto: "Quasi-elastic ferromagnetic excitations in Ndy_2Sry_2MnO_3"J.Phys.Chem.Solids. 60. 1177-1180 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kubota: "Neutron scattering studies on magnetic structure of double-layered manganiee La_<2-2x>Sr_<1+2x>Mn_2O_7 (0.30【less than or equal】x【less than or equal】0.50)"J.Phys.Chem.Solids. 60. 1161-1164 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Yoshizawa: "Anisotropic spin waves in a metallic ontiferromagnet Nd_<0.45>Sr_<0.55>MnO_3" Phys.Rev.B. 58. R571-574 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] R.Kajimoto: "Anomalous ferromagnetic spin fluctuations in an antiferromagnetic insulator Pr_<1-X>Ca_xMnO_3" Phys.Rev.B. 58. R11837-11840 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] K.Hirota: "Neutron-diffraction studies on the mgnetic ordering process in the layerd Mn perovskit La_<2-2X>Sr_<1+22>Mn_2O_7" J.Phys.Soc.Jpn.67. 3380-3383 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2020-05-15  

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