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Coexistence of superconductivity and magnetic order in rare-earth compounds.

Research Project

Project/Area Number 10640337
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionNiigata University

Principal Investigator

DONNI Andreas  Niigata University, Faculty of Science, Associate Prof., 理学部, 助教授 (50292199)

Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥2,900,000 (Direct Cost: ¥2,900,000)
Fiscal Year 1999: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1998: ¥2,100,000 (Direct Cost: ¥2,100,000)
Keywordssuperconductivity / magnetic structure / crystal structure / successive magnetic phase transitions / low-temperature neutron scattering / specific heat / 遂次磁気相転移
Research Abstract

Coexistence of superconductivity and magnetic order has been reported for the cubic Heusler alloys ErPdィイD22ィエD2Sn (Tc = 1.17 K, TィイD2NィエD2 = 1.0 K) and YbPdィイD22ィエD2Sn (Tc = 2.3 K, TィイD2NィエD2 = 0.22 K). We have prepared a polycrystalline YbPdィイD22ィエD2Sn sample, investigated the superconducting transition by electrical resistivity, magnetic ac susceptibility and specific heat experiments and performed low temperature neutron diffraction experiments down to 30 mK to determine the kind of magnetic structure that coexists with superconductivity. The results showed that the magnetic structures that coexist with superconductivity are different for ErPdィイD22ィエD2Sn (FCC-type II antiferromagnet, k=[1/2, 1/2, 1/2] with an additional incommensurate component) and for YbPdィイD22ィエD2Sn (FCC type I antiferromagnet, k=[0, 0, 1], with no incommensurate component).
For the high-temperature superconductors RィイD22ィエD2BaィイD24ィエD2CuィイD27ィエD2OィイD215-δィエD2(R=Dy,Er) we have used the sol gel technique to prepar … More e large amounts (over 3 cmィイD13ィエD1) of single phase samples. By systematic measurements of the low temperature specific heat we have studied the long- and short-range magnetic rare-earth interactions which coexist with superconductivity as a function of the rare-earth element (R) and of the oxygen content (δ). According to our specific heat results, changing the oxygen concentration in Er247 samples from a high or a low value to an intermediate value causes a larger in-plane anisotropy and tends to lower dimensionality and correlation range of the magnetic interactions of the ErィイD13+ィエD1 ions. Such an effect is not observed for the Dy247 samples, where the specific heat anomaly at TィイD2NィエD2 = 1.0 K is found to be almost independent of the oxygen concentration except for a small broadening for the sample DyィイD22ィエD2BaィイD24ィエD2CuィイD27ィエD2OィイD214.45ィエD2 with intermediate oxygen content, where electronic disorder in the CuOィイD22ィエD2-planes causes some disorder in the exchange interactions. Less

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (24 results)

All Other

All Publications (24 results)

  • [Publications] A. Donni: "MAGNETIC ORDER AND CRYSTAL-FIELD EXCITATIONS IN Nd_3Pd_<20>Ge_6"J. Phys : Condensed Matter. 10. 7219-7229 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] D. X. Li: "EVIDENCE FOR THE FORMATION OF THE SPIN GLASS STATE IN U_2PdSi_3"Phys. Rev. B. 57. 7434-7437 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "ANTIFERROMAGNETIC ORDERING IN THE CUBIC SUPERCONDUCTOR YbPd_2Sn"Physica B. 259・261. 705-706 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Herrmannsdorfer: "SUCCESSIVE MAGNETIC ORDERING OF THE Tb SUBLATTICES IN Tb_3Pd_<20>Si_6"J. Phys : Condensed Matter. 11. 2929-2936 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "EVIDENCE FOR AN ISOSTRUCTURAL PHASE TRANSITION IN THE METASTABLE HIGH-TEMPERATURE MODIFICATION OF TbPdA1"J. Alloys Compounds. 289. 11-17 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Kramer: "NONCOLLINEAR TWO-AND THREE-DIMENSIONAL MAGNETIC ORDERING IN THE HONEYCOMB LATTICES OF ErX_3(X=Cl, Br, I)"Phys. Rev. B (Rapid Communications). 60. 3724-3727 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "MAGNETIC ORDER AND CRYSTAL-FIELD EXCITATIONS IN NdィイD23ィエD2PdィイD220ィエD2GeィイD26ィエD2"J. Phys : Condensed Matter. 10. 7219-7229 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] D. X. Li: "EVIDENCE FOR THE FORMATION OF THE SPIN GLASS STATE IN UィイD22ィエD2PdSiィイD23ィエD2"Phys. Rev. B. 57. 7434-7437 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "ANTIFERROMAGNETIC ORDERING IN THE CUBIC SUPERCONDUCTOR YbPdィイD22ィエD2Sn"Physica B. 259-261. 705-706 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] T. Herrmannsdorfer: "SUCCESSIVE MAGNETIC ORDERING OF THE Tb SUBLATTICES IN TbィイD23ィエD2PdィイD220ィエD2SiィイD26ィエD2"J. Phys : Condensed Matter. 11. 2929-2936 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "EVIDENCE FOR AN ISOSTRUCTURAL PHASE TRANSITION IN THE METASTABLE HIGH-TEMPERATURE MODIFICATION OF TbPdAl"J. Alloys Compounds. 289. 11-17 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] K. Kramer: "NONCOLLINEAR TWO- AND THREE-DIMENSIONAL MAGNETIC ORDERING IN THE HONEYCOMB LATTICES OF ErXィイD23ィエD2 (X = Cl, B, I)"Phys. Rev. B (Rapid communications). 60. 3724-3727 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] A. Donni: "MAGNETIC ORDER AND CRYSTAL-FIELD EXCITATIONS IN Nd_3Pd_<20>Ge_6"J. Phys: Condensed Matter. 10. 7219-7229 (1998)

    • Related Report
      1999 Annual Research Report
  • [Publications] A. Donni: "ANTIFERROMAGNETIC ORDERING IN THE CUBIC SUPERCONDUCTOR YbPd_2Sn"Physica B. 259-261. 705-706 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] A. Donni: "EVIDENCE FOR AN ISOSTRUCTURAL PHASE TRANSITION IN THE METASTABLE"J. Alloys Compounds. 289. 11-17 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K. W. Kramer: "NONCOLLINEAR TWO- AND THREE-DIMENSIONAL MAGNETIC ORDERING IN THE HONEYCOMB LATTICES OF ErX_3 (X = Cl, Br, I)"Phys. Rev. B (Rapid Commun.). 60. 3724-3727 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] D. X. Li: "SPIN-GLASS BEHAVIOUR WITH EXTENDED SHORT-RANGE FERROMAGNETIC ORDER IN U_3RhSi_3"J. Phys: Condensed Matter. 11. 8263-8274 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T. Herrmannsdorfer: "SUCCESSIVE MAGNETIC ORDERING OF THE Tb SUBLATTICES IN Tb_3Pd_<20>Si_6"J. Phys: Condensed Matter. 11. 2929-2936 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H. Kitazawa: "MAGNETIC STRUCTURES OF THE RARE-EARTH PLATINUM ALUMINIDES RPtAl(R=Ce,Pr,Nd)" J.Solid State Chem. 140. 233-241 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] A.Donni: "MAGNETIC ORDER AND CRYSTAL-FIELD EXCITATIONS IN Nd_3Pd_<20>Ge_6" J.Phys: Condensed Matter. 10. 7219-7229 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] D.X.Li: "EVIDENCE FOR THE fORMATION OF THE SPIN GLASS STATE IN U_2PdSi_3" Phys.Rev.B. 57. 7434-7437 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] A.Donni: "CRYSTALLINE-ELECTRIC FIELD EXCITATIONS OF RPd_2Ga_3(R=Ce,Pr,Nd) STUDIED BY POWDER NEUTRON SCATTERING" Z.Phys.B: Condensed Matte. 10. 403-409 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] G.Bottger: "LOW-TEMPERATURE SPECIFIC HEAT OF Er_2Ba_4Cu_7O_<15-δ>" Z.Phys.B: Condensed Matter. 104. 195-198 (1997)

    • Related Report
      1998 Annual Research Report
  • [Publications] A.Donni: "NEUTRON-CRYSTALLINE ELECTRIC FIELD SPECTROSCOPY OF RPd_2Al_3(R=Ce,Pr,Nd)" J.Phys: Condensed Matter. 9. 5921-5933 (1997)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2021-04-07  

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