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Coulomb explosion of molecules in slow collisions of highly charge ions

Research Project

Project/Area Number 10640387
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 物理学一般
Research InstitutionTokyo Metropolitan University

Principal Investigator

OKUNO Kazuhiko  Tokyo Metropolitan University, Dept. of Physics, Professor, 理学研究科, 教授 (70087005)

Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 1999: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1998: ¥2,600,000 (Direct Cost: ¥2,600,000)
Keywordsmultiply charged ion / electron capture process / cross section / Coulomb explosion / fragmentation / three-particle coincedent detection / post collision effect / 多価イオン衝突 / 電子捕獲過程 / 反応分岐比 / フラグメント / 同時計測
Research Abstract

In collisions of highly charged ions with atom and molecules the most dominant processes are charge transfer processes in which highly charged ions capture an electron or many electrons into their excited state levels from targets. Many investigators have studied on electron capture processes of highly charge ions in collisions with atomic targets, however, details of the capture processes for molecular targets have been little investigated till now, because molecular explosion processes are too complicate.
In this project, we have developed a new double-coincidence time-of-flight (TOF) instrument for three particle coincident detection. The experimental technique is very powerful to resolve complex reaction mechanisms in collisions of multiply charged ions with molecules. Especially for diatomic molecules, all reaction processes can be resolved by this technique. Then, for collision systems of HeィイD12ィエD1+ and KrィイD18ィエD1+ with NィイD22ィエD2, OィイD22ィエD2, and CO targets, we have measured fragmentation of N2, C2 and CO in each electron capture processes and branching ratios for each reaction channel and kinetic energy release distribution for each fragmentation have been determined at some energies below 1keV/amu. Also, in the measurements of their collision energy dependence, we have found some new phenomena due to the post collision between projectile ions and target ions after collisions, where coincident ion pair peaks are splitting into two peaks and molecular ion peaks are shifting by getting momentum with decreasing of the collision energy. The observation of the post co9llision effects gives us important information to understand the collision dynamics.

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] Kazuhiko Okuno: "Double Electron Capture Processes in Collisions of He^<2+> with N_2,O_2, and CO at I KeV/amu"Physica Saripta. T80B. 173-175 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kunikazu Ishii: "Single-and Multiple-Charge Changing Cross Sect : ons in Slou Cdlisions of K,^<q+>(q=7-9) with Ne, N_2, O_2. and CO"Physica Seripta. T80B. 176-178 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] tatsuo Kaneyasu: "Fragnentation of CO in Electron Capture Collisions of He^<2+> at energios Kelou 1 KeV/dmu"Atom. Col. Res, in Jpn. 25. 52-53 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kunikazu Ishii: "Charge Changing Cross Sections Measuronents in Slou collisions of Kr^<q+> (q=3-9) with CO"Atom. Col. Res. in Jpn. 25. 50-51 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kouichi Saejima: "Linear cwd Circulon Dichroism in the Double Photoionization of He"Phys. Res. Let.. 83. 1546-1549 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Anatoli Kheifets: "Experimental and theovetical Study of Linearana Cevcular dichrosisin in Helium doubule photoionization"J. Phys. B : At. Md. Opt. Phys.. 32. L501-L509 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kunikazu Ishii: "Charge Changing Cross Section Measurements in Slow Collisions of KrィイD1q+ィエD1 (q=7-9) with Ne, NィイD22ィエD2, OィイD22ィエD2 and CO"Atom. Col. Res.. 24 (in Jpn). 75-76 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Tatsuo Kanayasu: "Double Electron Capture Processes in Collisions of HeィイD12+ィエD1 with HィイD22ィエD2, NィイD22ィエD2, OィイD22ィエD2 and CO at 1 keV/amu"Atom. Col. Res.. 24 (in Jpn). 77-78 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kouichi Soejima: "First Observation of Circular Dichroism in Angular Correlation Patterns for Two-Step Double and Direct Double Photoionization of Xenon"J. Korean Phys. Soc.. 32. 368-372 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kazuhiko Okuno: "Double Electron Capture Processes in Collisions of HeィイD12+ィエD1 with NィイD22ィエD2, OィイD22ィエD2 and CO at 1 keV/amu"Physica Scripta. T80B. 173-175 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kunikazu Ishii: "Single- and Multiple Charge Changing Cross Sections in Slow Collisions of KrィイD1q+ィエD1 (q=7-9) with Ne, NィイD22ィエD2, OィイD22ィエD2 and CO"Physica Scripta. T80B. 176-178 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Tatsuo Kanayasu: "Fragmentation of CO in Electron Capture Collisions of HeィイD12+ィエD1 at Energies below 1 keV/amu"Atom. Col. Res.. 25 (in Jpn). 752-753 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kunikazu Ishii: "Charge Changing Cross Section Measurements in Slow Collisions of KrィイD1q+ィエD1 (q=3-9) with CO"Atom. Col. Res.. 25 (in Jpn). 50-51 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kouichi Soejima: "Linear and Circular Dichroism in the Double Photoionization of Helium"Phys. Rev. Let.. 83. 1546-1549 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Anatoli Kheifets: "Experimental and Theoretical Study of Linear and Circular Dichroism in Helium Double Photoionization"J. Phys. B: At. Mol. Opt. Phys.. 32. K501-L509 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Kazuhiko Okuno: "Double electron capture processes in Collisions of He^<2+> with N_2,O_2 and CO at l KeV/auw"Physica Scripta. T80B. 173-175 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Kunikazu Ishii: "Single-and multiple-charge changing cross sections in slon collisions of Kr^<8+> (q=7-9)with Ne,N_2,O_2and CO"Physica Scripta. T80B. 176-178 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Tasuo Kaneyasu: "Fragmentation of CO in electron capture collisions of He^<2+> at evergies below l Kev/arru"Atom. Col. Res. in Jpn.. 25. 52-53 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Kunikazu Ishii: "Charge changing cross section measurevents in slow collisions of Kr^<8+>(q=3-9) with CO"Atom. Col. Res. in Jpn. 25. 50-51 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Kouichi Soejima: "Lirear and circular dichroism in the double photoinization of He"Phys. Rew. Let.. 83. 1546-1549 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Anatoli Kheifets: "Experimental and theoretical study of linear and circular dichroism in Helium double photoisnization"J. Phys. B. AT. Mol. Opt. Phys.. 32. L501-L509 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] K.Ishii: "Charge changing cross section measurments in slow collisions of Kr^<q+>(q=7-9) with Ne,N_2,O_2 and CO" Atomic Collision Research in Japan. 24. 75-76 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] T.Kaneyasu: "Double electron capture processes of He^<21> with H_2,N_2,O_2 and CO" Atomic Collision Research in Japan. 24. 77-78 (1998)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2016-04-21  

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