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Determination of the energy spectrum of secondary neutron flux for lunar samples and its application for meteoritics

Research Project

Project/Area Number 10640476
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 地球化学
Research InstitutionHiroshima University

Principal Investigator

HIDAKA Hiroshi  Hiroshima University, Faculty of Science, Associate Professor, 理学部, 助教授 (10208770)

Project Period (FY) 1998 – 1999
Project Status Completed (Fiscal Year 1999)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,900,000)
Fiscal Year 1999: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1998: ¥3,100,000 (Direct Cost: ¥3,100,000)
Keywordslunar soil / aubrite / chondrite / cosmic-ray / neutron capture reaction / samarium / gadolinium / isotopic composition / 中性子捕獲 / エネルギー共鳴 / 隕石
Research Abstract

The isotopic compositions of Sm and Gd in seven lunar samples from the Apollo 12 and 15 drill cores were determined to discuss the effects of neutron capture near the lunar surface. Neutron fluence values calculated from the isotopic shifts of A- 12 and A- 15 samples were (1.77 - 2.17) x10ィイD116ィエD1ncmィイD1-2ィエD1 and (3.02 - 4.68)x10ィイD116ィエD1 n cmィイD1-2ィエD1, respectively. Variations of εィイD2SmィエD2/εィイD2GdィエD2 with depth are interpreted as due to variations in the neutron energy spectrum. Our data suggest that the neutron is more thermalized at the lower layers than it is at the upper layers (Hidaka et al., in press).
This approach was applied for meteoritics. Large isotopic deviations of ィイD1149ィエD1Sm-ィイD1150ィエD1Sm and ィイD1157ィエD1Gd-ィイD1158ィエD1Gd derived from neutron capture effects were observed in five enstatite achondrites (aubrites). The isotopic variations of these aubrites correspond to irradiation with neutron fluence of (1.17-3.99)x10ィイD116ィエD1 n cmィイD1-2ィエD1 which is within the … More range of estimated neutron fluence values of some lunar samples. These results indicate that aubrites may have been located near the surface of their parent body for several hundreds of Ma. Furthermore, the neutron energy spectrum obtained from the combination of Sm and Gd isotope systematics (εィイD2SmィエD2/εィイD2GdィエD2) suggests that the energy of thermalized neutrons in five aubrites was in the range from 200 〜 400 K, and was lower than those in A-12 and A-15 lunar samples (Hidaka et al., 1999). Isotopic compositions of Sm and Gd in eight chondrites show an evidence of neutron capture effects in the chondrites, correspond to thermal neutron fluences of (1.03 〜 5.17)x10ィイD115ィエD1 n cmィイD1-2ィエD1. The Sm and Gd isotopic results of four of eight chondrites were compared with information on epi-thermal and fast neutron fluences calculated from literature Ne and Kr isotopic data. Thermal neutron fluence values of them are in agreement with epi-thermal neutron fluences (Hidaka et al., to be submitted). Less

Report

(3 results)
  • 1999 Annual Research Report   Final Research Report Summary
  • 1998 Annual Research Report
  • Research Products

    (32 results)

All Other

All Publications (32 results)

  • [Publications] H.Hidaka: "Geochemical and neutronic characteristics of the natural fossil fission reactors at Oklo and Bangombe,Gabon"Geochimica et Cosmochimica Acta. 62. 89-108 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka: "Isotopic analyses by using a Sensitive High Resolution Ion Micro-probe(SHRIMP)for natural logue study of Oklo Bangombe naturalfission reactors"Radio Chimica Acta. 82. 327-330 (1998)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka: "Isotopic stydy of natural fission reactors at Oklo and Bangombe,Gabon"Journal of Radio analytical and Nuclear Chemistry. 239. 53-58 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka: "Tc/Ru fractionation in the Oklo and Banombe natural fission reactors,Gabon"Chemistry Geology. 155. 323-333 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka et al.: "High fluences of neutrons determined ftom Sm and Gd lstopic compositions in aubrites"Earth and Planetary Science Letters. 173. 41-51 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] 日高洋: "20億年前の原子炉"電気評論. 84. 18-22 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka et al.: "Neutron capture effects on Sm,Eu and Gd in Apllo15 deep drill core samples"Meteoritics&Planetary Science. (in press). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka et al.: "Redistribution of fissiogenio and non-fissiogenic REE,Th and U in and around natural fission reactors at Oklo and Bangombe,Gabon"Geochimica et Cosmochimca Acta. (in press). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y.Fujii et al.: "The nuclrear interaction at Oklo 2 billion years ago"Nuclear Physics B. (in press). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hidaka: "The Oklo uranium ore as a natural fission rector:Its isotopic characterization by mass spectrometric approaches"Proceedings of 8th ISMAS Symposium on Mass Spectrometry. (in press). (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA and P. Holliger: "Geochemical and neutronic characteristics of the natural fossil fission reactors at Oklo and Bangombe (Gabon)."Geochim. Cosmochim. Acta.. 62. 89-108 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA: "Isotopic analyses by using a Sensitive High Resolution Ion Micro-Probe (SHRIMP) for natural analogue study of Oklo and Bangombe, natural fission reactors."Radiochim. Acta.. 82. 327-330 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA: "Isotopic study of natural fission reactors at Oklo and Bangombe, Gaobn."J. Radioanal, Nucl. Chem., Article. 239. 53-58 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA, P. Holliger and F. Gauthier-Lafaye: "Tc/Ru fractionation in the Oklo and Bangombe natural fission reactors, Gabon."Chem. Geol.. 155. 323-333 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA et al.: "High fluences of neutrons determined from Sm and Gd isotopic compositions in aubrites."Earth Planet Sci. Lett.. 173. 41-51 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA: "2 billion-years-old fission reactors."Denki-Hyoron. 84(9). 18-22 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA et al.: "Neutron capture effects on Sm. Eu and Gd in Apollo 15 deep drill core samples."Meteoritics & Planet. Sci.. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA et al.: "Redistribution of fissiogenic and non-fissiogenic REE. Th and U in and around natural fission reactors at Oklo and Bangombe, Gabon."Geochim. Cosmochim. Acta. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] Y. FUJII: "The nuclear interaction at Oklo 2 billion years ago."Nuclear Phys. B. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H. HIDAKA: "The Oklo uranium ore as a natural fission reactor: Its isotopic characterization by mass spectrometric approaches."Proc. of 8th ISMAS Symposium on Mass Spectrometry. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1999 Final Research Report Summary
  • [Publications] H.Hideka et al.: "High fluences of neutrons determined from Sun and Gd and isotopic compositions in aubrites"Earth and Planetary Science Letters. 173. 41-51 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 日高 洋: "20億年前の原子炉"電気評論. 84・9. 18-22 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Hideka et al.: "Nutron capture effects on Sm,Eu and Gd in Apollo 15 deep drill core samples"Meteoritics & Planetary Science. (in press). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Hideka et al.: "Redistribution of fissiogenic and non-fissiogenic REE, Th and U in around natural fission reactors at Oklo and Bangombe,Gabon"Geochimica et Cosmochimica Acta. (in press). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Fujii et al.: "The nuclear interaction at Oklo 2 billion years ago"Nuclear Physics B. (in press). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Hideka: "The Oklo uranium ore as a natural fission reactor:Its isotopic characterization by mass spectrometric approaches"Proceedings of 8th ISMAS symposium on Mass Spectrometry. (in press). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Hidaka: "The comparison of neutron energy spectrum between aubrites and lunar soils (A-15) obtained from Sm and Gd isotopic compositions" Meteoritics & Planetary Science. 33. A67 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Hidaka: "Geochevrical and neutronic characteristics of the natural fossil fission reactors at Okls and Bangombe, Gabon" Geochimica et Cosmochimica Acta. 62. 89-108 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Hidaka: "Isotopic analyses by using a sensitive High Resolution Ion Micro-Probe (SHRIMP) for natural analoque study of Okls and Bangombe natural fission reactors" Radiochimica Acta. 82. 327-330 (1998)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Hidaka: "Isotopic study of natural fission reactors at Okls and Bangombe, Gabon" Journal of Radioanabalytical and Nuclear Chemistry. 239. 53-58 (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Hidaka: "Tc/Ru fractionation in the Okls and Bangombe natural fission reactors" Chemical Geology. (印刷中). (1999)

    • Related Report
      1998 Annual Research Report
  • [Publications] H.Hidaka: "Samarium and gadolinium isotopic compositions of lunar samples" Lunar and Planetary Science. 30(印刷中). (1999)

    • Related Report
      1998 Annual Research Report

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Published: 1998-04-01   Modified: 2016-04-21  

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