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Summary of research on anomalous magnetic properties associated with orbital ordering and fluctuations

Research Project

Project/Area Number 11220201
Research Category

Grant-in-Aid for Scientific Research on Priority Areas (B)

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionUniversity of Tokyo (2000-2002)
Hokkaido University (1999)

Principal Investigator

SAKAKIBARA Toshiro.  Univ. of Tokyo, Inst. For Solid State Physics., Professor, 物性研究所, 教授 (70162287)

Co-Investigator(Kenkyū-buntansha) UEDA Kazuo  Univ. of Tokyo, Inst. For Solid State Physics, Professor, 物性研究所, 教授 (70114395)
OHKAWA Fusayoshi.J  Hokkaido Univ., Dept. of Physics, Professor, 大学院・理学研究科, 教授 (00107442)
AMITSUKA Hiroshi  Hokkaido Univ., Dept. of Physics, Associate Professor, 大学院・理学研究科, 助教授 (40212576)
Project Period (FY) 1999 – 2001
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥47,500,000 (Direct Cost: ¥47,500,000)
Fiscal Year 2001: ¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2000: ¥12,000,000 (Direct Cost: ¥12,000,000)
Fiscal Year 1999: ¥32,100,000 (Direct Cost: ¥32,100,000)
Keywordsmultipole order / neutron scattering / uniaxial pressure / field-induced gap / filled skutterudite / metal-insulator transition / hidden order parameter / orbital degeneracy / I軸応力効果 / ヘリカル構造 / スピン密度波 / f電子化合物 / 四重極転移 / 軸性圧力効果 / 高圧下中性子散乱 / 高圧下NMR / 低温磁化測定 / ミュオン緩和スペクトル / 磁気揺らぎ / 反強四重極転移 / 反強磁性転移 / 圧力効果 / 磁気相図 / 磁気八重極相互作用 / 磁化測定
Research Abstract

In this project, we have investigated various phase transition phenomena and unusual magnetic properties originating from the orbital degrees of freedom in f electron systems, with special interest in the antiferro-quadrupolar (AFQ) transition, hidden order, and metal-insulator transitions.
We established the magnetic phase diagram of the typical AFQ ordering system PrPb3 and found that the transition temperature is enhanced in magnetic field depending on the field orientation. The results are successfully explained by magnetic interactions between field-induced antiferromagnetic moments in the AFQ phase.
In the phase IV of CexLa1-xB6, whose order parameter is still unknown, we performed magnetic measurements under uniaxial pressure and found that a strong magnetic anisotropy is induced by a pressure along the [100] direction. The results indicate that the order parameter in phase IV is intrinsically anisotropic, such as Gamma-5 type octupoles. In URu2Si2, neutron diffraction experiment under high pressure revealed that a non-magnetic order and an antiferromagnetic one coexist in the ordered phase of this system. Although the true order parameter of the non-magnetic phase is still unknown, the present results forces a constraint on the theoretical models of this system.
In the filled skutterudite compound PrRu4P12, the metal-insulator transition has been explained by the lattice distortion mechanism which remove the orbital degeneracy of a Gamma-3 non-Kramers doublet. The field-induced gap observed in Yb4As3 has been explained on the basis of alternating Dzyaloshinsky-Moriya interaction.

Report

(4 results)
  • 2002 Final Research Report Summary
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • Research Products

    (30 results)

All Other

All Publications (30 results)

  • [Publications] T.Sakakibara, (8authors): "Multipole Ordering in felectron systems"J. Phys. Chem. Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakakibara, (5authors): "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in CexLal-xB6"J. Phys. Soc. Jpn.. 71(Suppl.). 48-51 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K.Matsuda, (3authors), H.Amitsuka: "Spatially Inhomogeneous Development of Antiferromagnetism in URu_2Si_2 : Evidence from ^<29>SiNMR under Pressure"Phys. Rev. Lett.. 87. 87203-1-87203-4 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Amitsuka, (3authors), T.Sakakibara, (5authors): "Hidden Order and Weak Antiferromagnetism in URu_2Si_2"Physica B. 312-313. 390-396 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.H.Curnoe, K.Ueda, (2authors): "Theory of Metal-Insurator Transition in PrFe_4P_<12> and PrRu_4P_<12>"J. Phys. Chem. Solids. 63. 1207-1210 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H.Satoh, F.J.Ohkawa: "Theory of the metamagnetic crossover in CeRu_2Si_2"Phys. Rev. B. 63. 184401-1-184401-13 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Sakakibara, T. Tayama, K. Tenya, M. Yokoyama, H. Amitsuka, D. Aoki, Y. Onuki, Z. Kletowski and S. Kunii: "Mutipole Orderng in f electron systems"J. Phys. Chem. Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Sakakibara, K. Tenya, M. Yokoyama, H. Amitsuka, and S. Kunii: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in Ce_xLa_<1-x>B_6"J. Phys. Soc. Jpn.. 71, Suppl.. 48-51 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] K. Matsuda, Y. Kohori, T. Kohara, K. Kuwahara, and H. Amitsuka: "Spatially Inhomogeneous Development of Antiferromagnetism in URu_2Si_2 : Evidence from ^<29>SiNMR under Pressure"Phys. Rev. Lett.. 87. 87203-1-4 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H. Amitsuka, M. Yokoyama, S. Miyazaki, K. Tenya, T. Sakakibara, W. Higemoto, K. Nagamine. K. Matsuda, Y. Kohori, and T. Kohara: "Hidden Order and Weak Antiferromagnetism in URu_2Si_2"Physica B. 312-313. 390-396 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] S.H. Cumoe, K. Ueda, H. Harima, and K. Takegahara: "Theory of Metal-Insulator Transition in PtFe_4P_<12> and PrRu_4P_<12>"J. Phys. Chem. Solids. 63. 1207-1210 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] H. Satoh, and F.J. Ohkawa: "Theory of the metamagnetic crossover in CeRu_2Si_2"Phys. Rev. B. 63. 184401-1-13 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakakibara: "Multipole Ordering in f electron systems"J. Phys. Chem. Solids. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Sakakibara: "Anomalous Uniaxial Pressure Effect on the Phase IV Ordering in CexLal-xB6"J. Phys. Soc. Jpn.. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Matsuda: "Spatially Inhomogeneous Development of Antiferromagnetism in URu_2Si_2 : Evidence from ^<29>Si NMR under Pressure"Phys. Rev. Lett.. 87. 87203-1-87203-4 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] H.Amitsuka: "Hidden Order and Weak Antiferromagnetism in URu_2Si_2"Physica B. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.H.Curnoe: "Structural Phase Transition and Anti-Quadrupolar Ordering in PrFe_4P_<12> and PrRu_4P_<12>"Physica B. (印刷中). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] H.Satoh: "Theory of the metamagnetic crossover in CeRu_2Si_2"Phys. Rev. B. 63. 184401-1-184401-1-13 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Tayama: "Antiferro-Quadrupolar Ordering and Multipole Interactions in PrPb_3"J.Phys.Soc.Jpn.. 70. 248-258 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Sakakibara: "Interplay of Orbital and Magnetic Degrees of Freedom in f-Electron Systems : The case of PrPb_3 and TmTe"J.Phys.Soc.Jpn.Suppl.A. 69. 25-32 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Amitsuka: "Pressure-Induced Magnetic Phase Transition of the 5f Electron System URu_2Si_2"J.Phys.Soc.Jpn.Suppl.A. 69. 5-12 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Takikawa: "Magnetic Properties of Ce_<0.75>La_<0.25>B_6 Under Uniaxial Stress"Physica B. 281&282. 561-562 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] E.Miyai: "Curie-Weiss law for almost localizecl itienerant-electron ferromagnets"Phys.Rev.B. 61. 1357-1365 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Y.Yamashita: "Spin Driven Jahn-Teller Distortion in a Pyrochlore system"Phys.Rev.Lett.. 85. 4960-4964 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] F.J.Ohkawa: "Quadrupole and dipole orders in URu2Si2"J. Phys. Condens. Matter. 11. L519-L524 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Amitsuka: "Effect of pressure on the tiny antiferromagnetic moment in the heavy-electron compound URu2Si2"Phys. Rev. Lett.. 83. 5114-5117 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Sakakibara: "Low Temperature Magnetization of Antiferro-Quadrupolar Ordering System TmTe"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Takikawa: "Magnetic Properties of Ce0.75La0.25B6 Under Uniaxial Stress"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Yokoyama: "Unusual Low Temperature Behavior of the Dilute Uranium Alloys La1-xUxRu2Si2(x<0.07)"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] H.Amitsuka: "Non-Fermi Liquid Behavior in R1-xUxRu2Si2(R=Th, Y and La)"Physica B. (印刷中). (2000)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2018-03-28  

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