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Summary of research on orbital orders and fluctuations

Research Project

Project/Area Number 11220202
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionTohoku University

Principal Investigator

KURAMOTO Yoshio  TOHOKU UNIV., DPT. PHYSICS, PROFESSOR, 大学院・理学研究科, 教授 (70111250)

Co-Investigator(Kenkyū-buntansha) GOTO Terutaka  NIIGATA UNIV., FAC. NAT. SCI., PROFESSOR, 大学院・自然科学研究科, 教授 (60134053)
SAKAKIBARA Toshiro  UNIV. TOKYO ISSP, PROFESSOR, 物性研究所, 教授 (70162287)
AOKI Haruyoshi  TOHOKU UNIV., DPT. PHYSICS, PROFESSOR, 超低温科学センター, 教授 (60302246)
AKIMITSU Jun  AOYAMAG.UNIV., DPT. PHYSICS, PROFESSOR, 理工学部, 教授 (80013522)
SERA Masafumi  HIROSHIMA UNIV., ADV. MAT. SCI., PROFESSOR, 大学院・先端物質科学研究科, 教授 (40196978)
Project Period (FY) 1999 – 2002
Project Status Completed (Fiscal Year 2002)
Budget Amount *help
¥23,800,000 (Direct Cost: ¥23,800,000)
Fiscal Year 2002: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2001: ¥10,900,000 (Direct Cost: ¥10,900,000)
Fiscal Year 2000: ¥7,300,000 (Direct Cost: ¥7,300,000)
Fiscal Year 1999: ¥4,100,000 (Direct Cost: ¥4,100,000)
KeywordsORBITAL DEGENERACY / f ELECTRONS / d ELECTRONS / SUPERCONDUCTIVITY / FERROMAGNETISM / ORBITAL ORDER / QUADRUPOLE MOMENT / OCTUPOLE MOMENT / 反強磁 / 反強磁性 / 軌道縮体
Research Abstract

This project has revealed new properties of matter due to orbital degrees of freedom by performing comprehensive study of systems ranging from 2p, 3d, to 4f and 5f electrons with "orbital order" and "orbital fluctuation" taken as key words. Furthermore, we have found new functionary materials by controlling the orbital degrees of freedom. In particular we mention the discovery of high-temperature superconductivity MgB2 and elucidation of its fundamental properties. The material has both sigma and pi orbitals which have very different properties. The coexistence influences essentially the physical property of MgB2. It has not been possible to grow large single crystals during the period of the project, but the project has paved the way for future development. On the other hand, we have reported a new high-temperature ferromagnet CaB2C2, and checked in detail the property of CaB6 and related materials. However, we have not yet excluded the possibility that Fe impurities may play an important role in realizing the ferromagnetism. For f electron systems, we have revealed characteristics of the orbital ordering in CeB6 and related materials, hidden order in URSu2Si2, and one-dimensional magnetism in Yb4As3, among other things.
We organized every year domestic meetings open to general audience and a special meeting after the discovery of MgB2. In 2002 we organized an international conference in Sendai having about 150 participants and active discussions with high quality. The proceedings were published as supplement of the Physical Society of Japan.

Report

(5 results)
  • 2002 Annual Research Report   Final Research Report Summary
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • Research Products

    (39 results)

All Other

All Publications (39 results)

  • [Publications] Y.Kuramoto, K.Kubo: "Interpocket polarization model for magnetic structures in rare-earth hexaborides"J. Phys. Soc. Jpn. 71. 2633-2666 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Koike, (9 authors), H.Aoki: "Magnetic Structure, Phase diagram, and a New Type of Spin Flop Transition Dominated by Many-Body Exchange Interaction in a Localized 4f System U3Pd2OSi6"Phys. Rev. Lett.. 89. 772021-772024 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Sakakibara, (9 authors): "Multipole ordering in felectron systems"J. Phys. Chem. Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T.Goto, B.Luethi: "Charge ordering, charge fluctuation and lattice effects in strongly correlated electron systems"Advances in Physics. 52. 67-118 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] M.Sera, (6 authors): "Anomalous Temperature Dependence of Magnetic Field Induced Autoferromagnetic Moment in the Antiferroquadrupolar Ordered State of CeB6"Phys. Rev. Lett.. 86. 1578-1581 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] J.Nagamatsu, (3authors), J.Akimitsu: "Superconductivity at 39K in magnesium diboride"Nature. 410. 63-64 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Kuramoto, Y.Kitaoka: "Dynamics of heavy electrons"Oxford University Press. 239 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y. Kuramoto, and K. Kubo: "Interpocket polarization model for magnetic structures in rare-earth hexaborides"J. Phys. Soc. Jpn.. 71. 2633-2666 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Koike, N. Metoki, Y.Haga, K.A.McEwen, M.Kohgi, R.Yamamoto, N.Aso, N.Tateiwa, T.Komatsubara, N.Kimura, H.Aoki: "Magnetic Structure, Phase diagram, and a New Type of Spin Flop Transition Dominated by Many-BodyExchange Interaction in a Localized 4f System U3Pd20Si6"Phys. Rev. Lett.. 89. 772021-772024 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Sakakibara, T. Tayama, K. Tenya, M. Yokoyama, H. Amitsuka, D. Aoki, Y. Onuki, Z. Kletowski, and S. Kunii: "Multipole ordeing in f electron systems"J. Phys. Chem. Solids. 63. 1147-1153 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] T. Goto, and B. Luethi: "Charge ordering, charge fluctuation and lattice effects in strongly correlated electron systems"Advances in Physics. Vol.52 No.2. 67-118 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] M. Sera, H. Ichikawa, T. Yokoo, J. Akimitsu, M. Nishi, K. Kakurai, and S. Kunii: "Anomalous Temperature Dependence of Magnetic Field Induced Antoferromagnetic Moment in the Antiferroquadrupolar Ordered State of CeB6"Phys. Rev. Lett.. 86. 1578-1581 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] J. Nagamatsu, N. Nakagawa, T. Muranaka, Y. Zenitani, and J.Akimitsu: "Superconductivity at 39K in magnesium diboride"Nature. 410. 63-64 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2002 Final Research Report Summary
  • [Publications] Y.Kuramoto, K.Kubo: "Interpocket polarization model for magnetic structures in rare-earth hexaborides"J.Phys.Soc.Jpn.. 71. 2633-2666 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] Y.Koike,....(9 authors), H.Aoki: "Magnetic Structure, Phase diagram, and a New Type of Spin Flop Transition Dominated by Many-BodyExchange Interaction in a Localized 4f System U_3Pd_<20>Si_6"Phys.Rev.Lett.. 89. 772021-772024 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Sakakibara,....(8 authors): "Multipole ordering in f electron systems"J.Phys.Chem. Solids. 63. 1147-1153 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Goto,....(6 authors): "Ferroquadrupole ordering of the ternary intermetallic compound Ce_3Pd_<20>Ge_6"Physica B. 312-313. 492-494 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Takigawa, K.Ohishi, J.Akimitsu,....(2 authors), M.Sera, S.Kunii: "Magnetic Properties in Phase IV of Ce_<0.7>La_<0.3>B_6 Studied by Muon Spin Relaxation"J.Phys.Soc.Jpn.. 71. 31-34 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Shiba, K.Ueda, O.Sakai, S.-J.Qin: "Theory of Field-Induced Gap Formation in Charge-Ordered Yb_4As_3"Physica B. 312-313. 309-314 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] J.Nagamatsu, ...(3 authors), J.Akimitsu: "Superconductivity at 39K in magnesium diboride"Nature. 410. 63-64 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] J.Akimitsu, ...(2 authors) H.Harima, Y.Kuramoto: "High-Temperature Ferromagnetism in CaB_2C_2"Science. 293. 1125-1127 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] H.Kusunose, Y.Kuramoto: "Non-Collinear Magnetism due to Orbital Degeneracy and Multipolar Interactions"J. Phys. Soc. Jpn.. 70(6). 1751-1761 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Terashima, ...(6 authors), H.Aoki: "Evolution of quasiparticle properties in UGe_2 with hydrostatic pressure studied via the de Haas-van Alphen Effect"Phys. Rev. Lett.. 87. 166401-166404 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Sera, ...(6 authors): "Anomalous Temperature Dependence of Magnetic Field Induced Antiferromagnetic Moment..."Phys. Rev. Lett.. 86. 1578-1581 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Tayama, T.Sakakibara...(7 authors): "Antiferro-quadrupolar ordering and multipole interactions in PrPb_3"J. Phys. Soc. Jpn.. 70. 248-258 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] 斯波 弘行: "電子相関の物理"岩波書店. 198 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Tayama,T.Sakakibara,K.Kitami,M,Yokoyama,K.Tenya,H.Amitsuka,D.Aoki,Y.Onuki and Z.Kletowski: "Antiferro-Ouadruplar Ordering and Multipole Interactions in PrPb_3"J.Phys.Soc.Jpn.. 70. 248-258 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Nakamura,T.Goto,O.Suzuki,S.Kunii and S.Sakatsume: "Screening effect on the multipole moments in the Kondo system Ce_xLa_<1-x>B_6"Phys.Rev.B. 61. 15203-15212 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Hazama,T.Goto,Y.Nemoto,Y.Tomioka,A.Asamitsu and Y.Tokura: "Quadrupolar effect in the perovskite manganite La_<1-x>Sr_xMnO_3"Phys.Rev.B. 62. 15012-15020 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Sera,H.Ichilkawa,T.Yokoo,J.Akimitsu,N.Nishi,K.Kakurai and S.Kunii: "Anomalous Temperature Dependence of the Magnetic Field Induced Antiferromagnetic Moment in the Antiferroquadrupolar Ordered State of CaB_6"Phys.Rev.Lett.. 86. 1578-1581 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Terashima,C.Terakura,Y.Umeda,N.Kimura,H.Aoki,and S.Kunii: "Ferromagnetism vs.Paramagnetism and False Quantum Oscillations in Lanthanum-Doped CaB_6"J.Phys.Soc.Jpn.. 69. 2423-2426 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Kusunose and Y.Kuramoto: "Multipolar Kondo effect in orbitally degenerate f-electron systems"Physica B : Condensed Matter. 281-282. 544-545 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Shiba,O.Sakai and R.Shiina: "Nature of Ce-Ce interaction in CeB_6 and its consequences"J.Phys.Soc.Jpn.. 68. 1988-1993 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Kohgi,K.Iwasa,J.-M.Mignot,N.Pyka,A.Ochiai,H.Aoki and T.Suzuki: "Magnetic excitations in the charge ordered state of Yb_4As_3 and Yb_4(As_<0.6>P_<0.4>)_3"Physica B. 259-261. 269-270 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Nagata,H.Fujino,J.Akimitsu,and others: "Antiferromagnetic ordering in the spin singler state of the ladder/chain material : Sr_<2.5>Ca_<11.5>Cu_<24>O_<11>"J.Phys.Soc.Jpn.. 68. 2206-2209 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] T.Sakakibara,T.Tayama,K.Tenya,H.Amitsuka,D.Aoki,Y.Onuki,and Z.Kletowski: "Magnetization study on the antiferro-quadrupolar ordering in PrPb_3"Physica B. 259-261. 340-342 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Nakamura,S.Sakatsume,O.Suzuki,T.Goto,Y.Nomoto,T.Horino,T.Matsumura,and S.Kunii: "Magnetic phase diagram and low-temperature properties of Ce_<0.5>La_<0.5>B_<0.6>"Physica B. 259-261. 36-37 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] M.Sera and S.Kobayashi: "Magnetic properties of the 4 sublattice model for the AF quadrupolar order"J.Phys.Soc.Jpn.. 68. 1664-1678 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] Y.Kuramoto and Y.Kitaoka: "Dynamics of heavy electrons"Oxford University Press,(Oxford,UK,2000). 239 (2000)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2018-03-28  

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