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Real-time observation and control of the high-harmonics generation and coulomb explosion of metal clusters in intense laser fields

Research Project

Project/Area Number 11640383
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 物理学一般
Research InstitutionTohoku Univesity

Principal Investigator

OHMORI Kenji  Tohoku University, Research Institute for Scientific Measurements, Research Associate, 科学計測研究所, 助手 (10241580)

Project Period (FY) 1999 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥3,500,000 (Direct Cost: ¥3,500,000)
Fiscal Year 2000: ¥1,300,000 (Direct Cost: ¥1,300,000)
Fiscal Year 1999: ¥2,200,000 (Direct Cost: ¥2,200,000)
Keywordsintense laser field / attosecond / high harmonics generation / interference / femtosecond / wave packet / coherent control / petawatt / クラスター / クーロン爆発 / 実時間観測 / 量子制御 / フェムト秒レーザー
Research Abstract

This research has been carried out in order to reveal the wave-packet dynamics associated with the multiple ionization and high harmonics generation of clusters in intense laser fields and to control those processes based on the quantum optical philosophy. First we succeeded in observing the wave-packet motion on the excited-state surface of the metal-rare gas or the metal-diatomic molecule clusters. The observed wave-packet motion has given the shape of the excited-state surface. We have examined the possibility of controlling the relevant wave-packet motion and found that a phase-locked optical-pulse pair is effective for that purpose. We have successfully carried out this scenario by controlling the interference of two nuclear wave packets generated in a single cluster with an accuracy of attoseconds. Next we constructed the electron time of flight detector (e-TOF) aiming at observing the electrons and ions that are ejected when the relevant wave packet is exposed to petawatt laser fields. We have measured the photoelectron spectra of atoms and molecules put in the petawatt laser fields using that e-TOF and found for the first time a high-energy component around 200 eV in addition to the low-energy valence component below 50 eV observed by many groups so far. This high-energy electron ejection is expected to be a counterpart of the high-harmonics generation in the soft X-ray region. At the moment we are trying to control this high-energy electron ejection through the phase modulation of the petawatt laser pulse. This technique is expected to realize the attosecond soft X-ray pulse source in the near future.

Report

(3 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • Research Products

    (12 results)

All Other

All Publications (12 results)

  • [Publications] K.Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. Vol.11. 284-286 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Kenji Ohmori: "Using optical collision to control the transition-region dynamics"Multiphoton Processes and Spectroscopy. Vol.14. 80-96 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "Femtosecond real-time probing of the ultrafast energy dissipation in the Hg(6^3P_1)-CO van der Waals interaction"J.Chem.Phys.. 113. 461-464 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "A high-resolution angle-resolved electron spectroscopy study of the 5dnp Rydberg series in Ba"J.Phys.B:At.Mol.Opt.Phys.. 32. 5223-5235 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. Vol.11. 284-286 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] Kenji Ohmori: "Using optical collision to control the transition-region dynamics"Multiphoton Processes and Spectroscopy. Vol.14. 80-96 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "Femtosecond real-time probing of the ultrafast energy dissipation in the Hg (6^3P_1)-CO van der Waals interaction"J.Chem.Phys.. 113. 461-464 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "A high-resolution angle-resolved electron spectroscopy study of the 5dnp Rydberg series in Ba"J.Phys.B : At.Mol.Opt.Phys.. 32. 5223-5235 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] K.Ohmori: "Attosecond coherent control of the wave packet dynamics in the Hg-X van der Waals interaction"Spectral Line Shapes. Vol.11. in press. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] Kenji Ohmori: "Using optical collision to control the transition-region dynamics"Multiphoton Processes and Spectroscopy. Vol.13. 80-96 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Ohmori: "Femtosecond real-time probing of the ultrafast energy dissipation in the Hg(6^3P_1)-CO van der Waals interaction"J.Chem.Phys.. 113. 461-464 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] Kenji Ohmori: "Optical collision to control the transition-region dynamics"Multiphoton Processes and Spectroscopy. vol.13(in press). (2000)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2016-04-21  

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