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Development of a Microwave-induced Plasma Reactor Combined with Catalyst for Harmful Gas Treatment

Research Project

Project/Area Number 11650290
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 電力工学・電気機器工学
Research InstitutionOita University

Principal Investigator

KANAZAWA Seiji  Oita University, Department of Electrical and Electronic Engineering, Associate Professor, 工学部, 助教授 (70224574)

Co-Investigator(Kenkyū-buntansha) OHKUBO Toshikazu  Oita University, Department of Electrical and Electronic Engineering, Professor, 工学部, 教授 (00094061)
NOMOTO Yukiharu  Oita University, Department of Electrical and Electronic Engineering, Professor, 工学部, 教授 (90037953)
Project Period (FY) 1999 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥3,600,000 (Direct Cost: ¥3,600,000)
Fiscal Year 2000: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 1999: ¥2,900,000 (Direct Cost: ¥2,900,000)
KeywordsMicrowave discharge / Atmospheric pressure plasma / Plasma catalytic reaction / Photocatalyst / VOC
Research Abstract

Non-thermal plasma processing has been considered as one of the most effective methods for harmful gas treatment. However, the issues to be solved are the improvement of the energy efficiency and the control of undesirable by-products. To improve the energy efficiency, utilization of catalyst/adsorbent into plasmas was investigated. Microwave discharges are attractive for this purpose due to their property to have different plasma compared to the conventional non-thermal plasmas and due to their ability to heat a material such as a catalyst. In this study, a microwave induced plasma reactor was developed and used for decomposition of harmful gas. The reactor consists of a quartz glass tube which inserts in the waveguide vertically. To sustain the plasma at atmospheric pressure, a fine carbon rod covered by an alumina tube is set inside the quartz glass tube coaxially to act as a source of electrons. Especially, the combination of plasma with photocatalyst was studed. NO and toluene (C_6H_5CH_3) were chosen as test gases. As a results, the microwave plasma could be generated stably at atmospheric pressure with low microwave power (<10W). It was found that efficient decomposition of NO and toluene was possible using the microwave plasma process. The combination of the plasma and photocatalyst (TiO_2) was effective for improving efficiency at lower power consumption. The NO and toluene decomposition rates increase with increasing the specific energy density, while the energy efficiency decreases with increasing the specific energy density. However, decomposition efficiency nonmonotonically depends on the gas flow rate. The energy efficiency obtained was the same order with conventional non-thermal plasma processes such as dc corona and dielectric barrier discharges induced plasma processes.

Report

(3 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] 丸尾大輔: "触媒反応アシスト型マイクロ波放電プラズマによる有害ガスの処理"電気学会放電研究会資料. ED-99-77. 5-8 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 金沢誠司: "マイクロ波を利用した有害ガス処理用プラズマの発生とトルエンの分解への応用"静電気学会講演論文集'99. 17aB3. 185-186 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa: "Decomposition of VOCs by Microwave Discharge Plasma at Atmospheric Pressure"Proc.of the 17th Symposium on Plasma Processing. 443-446 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 金沢誠司: "大気圧マイクロ波放電プラズマによるトルエンの分解特性"平成12年電気学会全国大会講演論文集. 1-165. 213 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa: "Decomposition of Toluene by a Dielectric Barrier Discharge Reactor with a Catalyst Coating Electrode"Transactions of the Institute of Fluid-Flow Machinery. 107. 65-74 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa: "Decomposition of Toluene in Air by a Microwave Discharge Plasma Reactor"Proc.Second Asia-Pacific International Symposium on the Basic and Application of Plasma Technologys. (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] D.Li, S.Kanazawa, T.Ohkubo, Y.Nomoto: "Decomposition of Toluene by Silent Discharge Plasma with Photocatalyst, (in Japanese)"Proc.of 1999 Annuak Meeting of The Institute of Electrostatics Japan. 17a B1. 179-180 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Maruo, T.Ohkubo, Y.Nomoto: "Generation of Microwave-induced Plasma for Harmful Gas Treatment and its Application for Decomposition of Toluene, (in Japanese)"Proc.of 1999 Annuak Meeting of The Institute of Electrostatics Japan. 17a B3. 185-186 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] D.Maruo, S.Kanazawa, T.Ohkubo, Y.Nomoto: "Treatment of Harmful Gases by Microwave-Induced Plasma with Catalyst, (in Japanese)"Papers of Technical Meeting on Electrical Discharges. ED-99-77, IEE Japan. 5-8 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Maruo, T.Ohkubo, Y.Nomoto: "Decomposition of VOCs by Microwave Discharge Plasma at Atmospheric Pressure"Proc.of the 17th Symposium on Plasma Processing. 443-446 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Maruo, S.Akamine, T.Ohkubo, Y.Nomoto: "Decomposition of Toluene Using Microwave Discharge Plasma, (in Japanese)"2000 National Convention Record IEE Japan. 210. 1-165 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Li, S.Akamine, T.Ohkubo, Y.Nomoto: "Decomposition of Toluene by a Dielectric Barrier Discharge Reactor with a Catalyst Coating Electrode"Proceedings The First Polish-Japanese Hakone Group Symposium on Non-Thermal Plasma Processing of Water and Air. 55-58 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] D.Maruo, S.Kanazawa, T.Ohkubo, Y.Nomoto: "Effect of Reactor Diameter on Toluene Decomposition by Microwave Discharge Plasma at Atmospheric Pressure, (in Japanese)"Record of 2000 Joint Conference of Electrical and Electronics Engineers in Kyushu. 635. 269 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Li, S.Akamine, T.Ohkubo, Y.Nomoto: "Decomposition of Toluene by a Dielectric Barrier Discharge Reactor with a Catalyst Coating Electrode"Transactions of the Institute of Fluid-Flow Machinery. 107. 65-74 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] S.Kanazawa, D.Maruo, T.Ito, T.Ohkubo, Y.Nomoto: "Decomposition of Toluene in Air by a Microwave Discharge Plasma Reactor"Proc.Second Asia-Pacific International Symposium on the Basic and Application of Plasma Technology. (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 丸尾大輔: "大気圧マイクロ波放電プラズマによるトルエン分解に及ぼす放電管径の影響"平成12年度電気関係学会九州支部連合会大会論文集. 635. 269 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Kanazawa: "Decomposition of Toluene by a Dielectric Barrier Discharge Reactor with a Catalyst Coating Electrode"Transactions of the Institute of Fluid-Flow Machinery. 107. 65-74 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Kanazawa: "Decomposition of Toluene by a Dielectric Barrier Discharge Reactor with a Catalyst Coating Electrode"Proceedings The First Polish-Japanese Hakone Group Symposium on Non-Thermal Plasma Processing of Water and Air. 55-58 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Kanazawa: "Decomposition of Toluene in Air by a Microwave Discharge Plasma Reactor"Proc.Second Asia-Pacific International Symposium on the Basic and Application of Plasma Technologys. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] 丸尾大輔: "触媒反応アシスト型マイクロ波放電プラズマによる有害ガスの処理"電気学会放電研究会資料. ED-99-77. 5-8 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 金沢誠司: "マイクロ波を利用した有害ガス処理用プラズマの発生とトルエンの分解への応用"静電気学会講演論文集'99. 17aB3. 185-186 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] S.Kanazawa: "Decomposition of VOCs by Microwave Discharge Plasma at Atmospheric Pressure"Proc.of the 17th Symposium on Plasma Processing. 443-446 (2000)

    • Related Report
      1999 Annual Research Report
  • [Publications] 金沢誠司: "大気圧マイクロ波放電プラズマによるトルエンの分解特性"平成12年電気学会全国大会講演論文集. 1-165. 213 (2000)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2016-04-21  

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