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Development of Spin-Tunneling Junctions with Large Magnetoresistance Using Half-Metallic Oxide Ferromagnets

Research Project

Project/Area Number 11650320
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionJapan Advanced Institute of Science and Technology

Principal Investigator

GOMI Manabu  School of Materials Science, Japan Advanced Institute of Science and Technology Associate Professor, 材料科学研究科, 助教授 (80126276)

Project Period (FY) 1999 – 2000
Project Status Completed (Fiscal Year 2000)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2000: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 1999: ¥3,000,000 (Direct Cost: ¥3,000,000)
KeywordsSpin Tunneling Junction / Magnetic Oxide Thin Film / Giant Magnetoresistance / Pulsed Laser Deposition / Magnetite Thin Film / Surface Magnetism / Low Temperature Growth / Half-Metallic Oxide Ferromagnet / トンネル磁気抵抗 / 反位相境界 / パルスレーザ堆積 / ダブルプロブスカイト酸化物
Research Abstract

Optimum fabrication conditions of the junctions and influence of surface magnetic of the ferromagnetic oxides on tunneling magnetoresistance have been investigated in order to achieve large magnetoresistance effect in tunneling junctions using transition metal oxides with half metallic nature. The results are summarized as follows :
1.Thin films of Fe_3O_4 and MgO with high quality were grown by pulsed laser deposition (PLD) at low temperature. The insulating MgO layer was required to be grown at lower temperature than 200℃ even at oxigen pressure of 1 x 10^<-5> Torr in order to prevent the Fe_3O_4 surface from oxidizing in a fabrication process of junction. Thin films of Sr_2FeMoO_6 with half metallic nature which is a promising candidate of ferromagnetic electrode were successfully grown at 500℃, lower than the reported growth temperature.
2.Optimum PLD-growth conditions for MgO insulating layers were determined. Analysis of current-voltage characteristics of Fe_3O_4/MgO/Au junction structures fabricated under the optimum conditions showed that the junctions with MgO insulating layer as thin as 1 nm have good tunneling quality.
3.Tunneling magnetoresistane (TMR) due to the magnetization of the Fe_3O_4 electrodes aligned in anti-parallel was observed in a Co_<0.4>Fe_<2.6>O_4/Fe_3O_4/MgO/Fe_3O_4 junction, though the TMR change was as low as -0.5 %. The magnetic field dependence of TMR showed that the low TMR may be associated with the superparamagnetic behavior of the surface magnetization of Fe_3O_4 electrode layers.
4.The Fe_3O_4/NiO/MgO/NiO/Fe_3O_4 junction structures with double insulating layers of non-magnetic MgO - magnetic NiO were fabricated. However, the expected junction properties were not obtained due to some issues caused by large junction area and NiO layers as thin as 1 nm. The advanced process fabricating the fine structure such as photolithography will be required to overcome these problems.

Report

(3 results)
  • 2000 Annual Research Report   Final Research Report Summary
  • 1999 Annual Research Report
  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] T.Kiyomura: "PLD Growth of Stoichiometric Fe_3O_4 Thin Films for Spin Tunnmeling Devices"IEEE Trans.on Magn.. 35. 3046-3048 (1999)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] 五味学: "パルスレーザー堆積によるフェライト薄膜の低温成長"粉体および粉末冶金. 47. 723-729 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Kiyomura: "Electrical Properties of MgO Insulating Layers in Spin-Dependent Tunneling Junctions using Fe_3O_4"J.Appl.Phys.. 88. 4768-4771 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Kiyomura: "Structural and Magnetic Properties of Spinel Ferrite Epitaxial Films pulsed-Laser-Deposited at Low Temperature"Jpn.J.Appl.Phys.. 49. 118-122 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi: "Pulsed Laser Deposition of Magnetic Oxide Thin Films for Magnetic Tunneling Devices"J.Alloys and Compounds. (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi: "Spin-Dependent Transport in Tunneling Junctions Using Fe_3O_4"Ferrites : Proc.of The 8th Int.Conf.on Ferrites. (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi: "Magnetic and Electric Properties of Ordered Double-Perovskite Sr_2CrWO_6 Thin Films Grown by Molecular-Beam Epitaxy"Ferrites : Proc.of The 8th Int.Conf.on Ferrites. (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] H.Nogi: "Epitaxial Growth of Fe_3O_4 Thin Films by Alternate Adsorption of Iron Acetylacetonate and Oxygen"Ferrites : Proc.of The 8th Int.Conf.on Ferrites. (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Kiyomura, M.Gomi, Y.Maruo, and H.Toyoshima: "PLD Growth of Stoichiometric Fe_3O_4 Thin Films for Spin Tunneling Devices"IEEE Trans.on Magn.. 35 (5). 3046-3048 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi and T.Kiyomura: "Low Temprature Growth of Ferrite Thin Films by Pulsed Laser Deposition"Jpn.Soc.Powder and Powder Metallurgy. 47 (7). 723-729 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Kiyomura, Y.Maruo, and M.Gomi: "Electrical properties of MgO insulating layers in spin-dependent tunneling junctions using Fe_3O_4"J.Appl.Phys.. 88 (8). 4768-4771 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Kiyomura and M.Gomi: "Structural and Magnetic Properties of Spinel Ferrite Epitaxial Films Pulsed-Laser-Deposited at Low Temperature"Jpn.J.Appl.Phys.. 49 (1). 118-122 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi: "Pulsed Laser Deposition of Magnetic Oxide Thin Films for Magnetic Tunneling Devices"J.Alloys and Compounds. (to be published). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi, Y.Maruo, and R.Tamoto: "Spin-Dependent Transport in Tunneling Junctions Using Fe_3O_4"Ferrites : Proc.of The 8^<th> Int.Conf.On Ferrites.. (to be published). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] M.Gomi and S.Ichinose: "Magnetic and Electric Properties of Ordered Double-Perovskite Sr_2CrWO_b Thin Films Grown by Molecular-Beam Epitaxy"Ferrites : Proc.of The 8^<th> Int.Conf.On Ferrites. (to be published). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] H.Nogi, K.Kametani, and M.Gomi: "Epitaxial Growth of Fe_3O_4 Thin Films by Alternate Adsorption of Iron Acetylacetonate and Oxygen"Ferrites : Proc.of The 8^<th> Int.Conf.On Ferrites. (to be published). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2000 Final Research Report Summary
  • [Publications] T.Tiyomura: "Electrical properties of MgO insulating layers in spin-dependent tunneling junctions using Fe_3O_4"J.AppL.Phys.. 88・8. 4768-4771 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Gomi: "Spin-dependent transport in tunneling junctions using Fe_3O_4"Ferrites : Proc.of The 8th Int.Conf.on Ferrites. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Gomi: "Pulsed laser deposition of magnetic oxide thin films for magnetic tunneling devices"J.Alloys and Compounds. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Kiyomura: "Structural and magnetic properties of spinel ferrite epitaxial films pulsed-laser-deposited at low temperature"Jpn.J.Appl.Phys.. 40・1. 118-122 (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] H.Nogi: "Epitaxial growth of Fe_3O_4 thin films by alternate adsorption of iron-organic complex and oxygen"Ferrites : Proc.of The 8th Int.Conf.on Ferrites. (2001)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Kiyomura: "PLD Growth of Stoichiometric Fe_3O_4 Thin Films for Spin Tunneling Devices"IEEE Trans.on Magn.. 35・5. 3046-3048 (1999)

    • Related Report
      1999 Annual Research Report
  • [Publications] 五味 学: "パルスレーザー堆積によるフェライト薄膜の低温成長"粉体および粉末冶金. 47・7. (2000)

    • Related Report
      1999 Annual Research Report

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Published: 1999-04-01   Modified: 2016-04-21  

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