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Investigation of free volume in polymer by using synchronized irradiation technique of pulsed positron beam and laser

Research Project

Project/Area Number 11680516
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionOsaka University

Principal Investigator

HONDA Yoshihide  Osaka University, ISIR, Research Associate, 産業科学研究所, 助手 (40209333)

Co-Investigator(Kenkyū-buntansha) YOSHIDA Yoichi  Osaka University, ISIR, Associate Professor, 産業科学研究所, 助教授 (50210729)
NISHIJIMA Shigehiro  Osaka University, Graduate school of engineering, Professor, 大学院・工学研究所, 教授 (00156069)
TAGAWA Seiichi  Osaka University, ISIR, Professor, 産業科学研究所, 教授 (80011203)
Project Period (FY) 1999 – 2001
Project Status Completed (Fiscal Year 2001)
Budget Amount *help
¥3,700,000 (Direct Cost: ¥3,700,000)
Fiscal Year 2001: ¥200,000 (Direct Cost: ¥200,000)
Fiscal Year 2000: ¥800,000 (Direct Cost: ¥800,000)
Fiscal Year 1999: ¥2,700,000 (Direct Cost: ¥2,700,000)
KeywordsPositron / Positronium / Synchronization / Multiple irradiation / Pulsed positron beam / Electron linear accelerator
Research Abstract

To investigate the interactions between positronium and the materials using laser-synchronized system, we have developed two kinds of short pulsed positron beams based on L-band and S-band electron linear accelerators (linacs) which are characterized by high density and high count rate.
A new facility based on L-band linac (maximum energy: 38 MeV, pulse width: 20 ps) was designed and constructed for the purpose of the investigation of the status of positronium in the materials by exciting positronium with ultra short pulsed laser. In the experiments, the number of positrons coming from the target with the energy corresponding to the applied voltage was about 2500 per pulse and the pulse width was about 20 ns (FWHM) by measuring annihilation gamma rays. These values were rather low compared with the computational estimation. This results could be mainly ascribed to improper positioning of the positron beam because of bright electron image.
The several phenomena such as excitation of the specialized molecules and vibration, can be introduced by laser irradiation and the lifetime of the positronium is influenced through the interactions. We also developed another new short pulsed positron beam facility based on S-band linac for the use of this kind of experiment. The pulse width of this positron beam could be attained about 370 ps. Using this positron beam, we started the measurement of positron lifetime in several materials with regular structure such as LB films and several derivatives, to investigate the interactions mentioned above. The experiments with laser excitation will be started soon.

Report

(4 results)
  • 2001 Annual Research Report   Final Research Report Summary
  • 2000 Annual Research Report
  • 1999 Annual Research Report
  • Research Products

    (14 results)

All Other

All Publications (14 results)

  • [Publications] Y.Honda, et al.: "Development of a new positron beam for coincident studies with laser excitation"Material Science Forum. 363-365. 667-669 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M.Tashiro, et al.: "Development of a pulsing system with the linac based slow positron beam"Material Science Forum. 363-365. 664-666 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M.Tashiro, et al.: "Development of a short-pulsed slow positron beam for application to polymer films"Radiation Physics and Chemistry. 60. 529-533 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M.Tashiro, et al.: "Study of interfaces in polymer bilayers using slow positron beam"Applied Surface Science. (to be published).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Tashiro, et al.: "Study of interfaces in polymer bilayers using slow positron beam"Applied Surface Science. (To be published).

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y. Honda, et al.: "Development of a new positron beam for coincident studies with laser excitation"Material Science Forum. 363-365. 667-669 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Tashiro, et al.: "Development of a pulsing system with the linac based slow positron beam"Material Science Forum. 363-365. 664-666 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] M. Tashiro, et al.: "Development of a short-pulsed slow positron beam for application to polymer films"Radiation Physics and Chemistry. 60. 529-533 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2001 Final Research Report Summary
  • [Publications] Y.Honda, et al.: "Development of a new positron beam for coincident studies with laser excitation"Material Science Forum. 363-365. 667-669 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Tashiro, et al.: "Development of a pulsing system with the linac based slow positron beam"Material Science Forum. 363-365. 664-666 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Tashiro, et al.: "Development of a pulsing system with the linac based slow positron beam"Radiation Physics and Chemistry. 60. 529-533 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Tashiro, et al.: "Study of interfaces in polymer bilayers using slow positron beam"Applied Surface Science. (to be published).

    • Related Report
      2001 Annual Research Report
  • [Publications] Y.Honda, et al.: "Development of a new positron beam for coincident studies with laser excitation"Material Science Forum . (to be published).

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Tashiro, et al.: "Development of a pulsing system with the lianc based slow positron beam"Material Science Forum . (to be published).

    • Related Report
      2000 Annual Research Report

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Published: 1999-04-01   Modified: 2016-04-21  

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