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BLUK SENSITIVE HIGH RESOLUTION PHOTOEMISSION AND MICROSPECTROSCOPY

Research Project

Project/Area Number 12304015
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅰ(光物性・半導体・誘電体)
Research InstitutionOSAKA UNIVERSITY

Principal Investigator

SUGA Sigemasa  OSAKA UNIVERSITY, GRADUATE SCHOOL OF ENGINEERING SCIENCE, PROFESSOR, 基礎工学研究科, 教授 (40107438)

Co-Investigator(Kenkyū-buntansha) SEKIYAMA Akira  OSAKA UNIVERSITY, GRADUATE SCHOOL OF ENGINEERING SCIENCE, ASSISTANT PROFESSOR, 基礎工学研究科, 助手 (40294160)
IMADA Shin  OSAKA UNIVERSITY, GRADUATE SCHOOL OF ENGINEERING SCIENCE, ASSOCIATE PROFESSOR, 基礎工学研究科, 助教授 (90240837)
Project Period (FY) 2000 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥38,710,000 (Direct Cost: ¥31,900,000、Indirect Cost: ¥6,810,000)
Fiscal Year 2003: ¥9,620,000 (Direct Cost: ¥7,400,000、Indirect Cost: ¥2,220,000)
Fiscal Year 2002: ¥9,620,000 (Direct Cost: ¥7,400,000、Indirect Cost: ¥2,220,000)
Fiscal Year 2001: ¥10,270,000 (Direct Cost: ¥7,900,000、Indirect Cost: ¥2,370,000)
Fiscal Year 2000: ¥9,200,000 (Direct Cost: ¥9,200,000)
Keywordssoft x-ray / photoelectron / hulk / ARPES / Fermi Swtau / spin polarized STM / photoelectron emission / microscope / バンドマッピング / 高分解能 / 軟X線光分子光 / 超高分解能 / バルク敏感光電子分光 / 強相関電子系 / スピン・電荷分離 / コヒーレント成分 / 光電子分光 / 放射光 / バルク電子状態 / 表面電子状態 / ミクロ領域
Research Abstract

In many transition metal compounds and alloys, which are attracting attention from practical of view, the Coulomb repulsive force between electrons (so called electron correlation : U) is large and makes the system either an insulator or a metal depending upon its relative magnitude to the electron transfer energy t. On the surface of solids, the number of the nearest neighbor atoms is much reduced than in the bulk. So the electron correlation effect represented by U/t becomes very important on the surface. The photoemission spectroscopy, which is now an inevitable tool to study electronic structures of correlated electron systems, is a rather surface sensitive technique because of the short mean free path of the photoelectrons with the minimum of 3 to 5A in the region of 20-120cV. If the kinetic energy becomes more than a few hundred eV, however, the mean free path becomes larger than 10A. Then the relative weight of the surface contribution is much reduced. We have succeeded in the angle resolved photoemission spectroscopy in the soft X-ray region for the first time and found clear differences of the Fermi surface shapes from surface sensitive low energy ARPES in the cases of Sr_2Ruo_4 and LA_<2-x>Sr_xCuO_4.
As for the microspectroscopy, we have succeeded in photoelectron emission microscopy by use of the circularly polarized light at BL25SU of SPring-8. We have further succeeded in the spin polarized scanning tunneling microscopy on the Fe island system on W(001).

Report

(5 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • Research Products

    (36 results)

All Other

All Publications (36 results)

  • [Publications] Akira Sekiyama: "Bulk 4f Electron States of Ce-Based Heavy Fermion System Proved by High-resolution Resonance Photoemission"J.Phys.Soc.Jpn.. 69. 2771-2774 (2000)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Shigemasa Suga: "High Resolution Soft X-ray Bulk Sensitive Photoemission from Strongly Correlated Systems"J.Electr.Spectrosc.Rel Phenom.. 114-116. 659-658 (2001)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Shin Imada: "Magnetic Microspectroscopy by a Combination of XMCD and PEEM"Surface Review and letters. 9. 877-881 (2002)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Atsushi Yamasaki: "Direct Observation of the Single-domain Limit of Fe Nanomagnets by Spin-polarized Scanning tunneling Spectroscopy"Phys.Rev.Lett.. 91. 127201-1-127201-2 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Atsushi Higashiya: "Resonant Inelastic X-ray Scattering (RIXS) of SrCuO_2"Solid State Commun.. 130. 7-11 (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Akira Sekiyama: "High-energy Bulk Sensitive Angle-resolved Photoemission Study of Strongly Correlated Systems"J.Electr.Spectrosc.Rel Phenom.. (in press). (2004)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Akira Sekiyama: "Bulk 4f Electron States of Ce-Based Heavy Fermion System Proved by High-resolution Resonance Photoemission"J. Phys: Soc. Jpn.. 69. 2771-2774 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Shigemasa Suga: "High Resolution Soft X-ray Bulk Sensitive Photoemission from Strongly Correlated Systems"J.Electr. Spectrosc : Rel Phenom.. 114-116. 658-659 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Shin Imada: "Magnetic Microspectroscopy by a Combination of XMCD and PEEM"Surface Review and Letters. 9. 877-881 (2002)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Atsushi Yamasaki: "Direct Observation of the Single-domain Limit of Fe Nanomagnets by Spin-polarized Scanning tunneling Spectroscopy"Phys. Rev. Lett.. 91. 127201-1-127201-2 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Atsushi Higashiya: "Resonant Inelastic X-rah Scattering (RIXS) of SrCuO2"Solid State Commun. 130. 7-11 (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Akira Sekiyama, High-energy Bulk: "Sensitive Angle-resolved Photoemission Study of Strongly Correlated Systems"J. Electr. Spectrosc. Rel Phenom.. (in press). (2004)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Higashiya: "Resonant Inelastic X-ray Scattering (RIXS) of SrCuO_2"Solid State Commun.. (印刷中). (2004)

    • Related Report
      2003 Annual Research Report
  • [Publications] J.-S.Kang: "Resonant photoemission spectroscopy study of impurity-induced melting in Cr- and Ru-doped Nd_<1/2>A_<1/2>MnO_3(A=Ca,Sr)"Phys.Rev.. B68. 012410-1-012410-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] R.-J.Jung: "Localized character of 4f electrons in CeRh_x(x=2,3) and CeNi_x(x=3,5)"Phys.Rev.Lett.. 91. 157601-1-157601-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Yamasaki: "Direct observation of the single-domain limit of Fe nanomagnets by spin-polarized scanning tunneling spectroscopy"Phys.Rev.Lett. 91. 127201-1-127201-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] E.-J.Cho: "Auger effect in high-resolution Ce 3d-edge resonance photoemission photoemission"Phys.Rev.. B67. 155107-1-155107-6 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] S.-K.Mo: "Prominent quasiparticle peak in the photoemission spectrum of the metallic phase of V_2O_3"Phys.Rev.Lett.. 90. 186403-1-186403-4 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] A.Irizawa: "Bulk-sensitive photoemission of Mn_5Si_3"Solid State Commun.. 124. 1-5 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] J.-S.Kang: "Resonanct Photoemission Spectroscopy of A_2FeMoO_6 Double Perovslkites (A=Sr, Ba)"Phys. Rev. B. 66. 113105-1-113105-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Soda: "High-resolution photoelectron spectroscopy of Heusler-type Fe_2VAl alloy"J. Syncrotron Radiation. 9. 233-236 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] H.Sato: "Electronic structure of YbXCu_4 (X=In, Cd, Mg) investigated by high-resolution photoemission"J. Syncrotron Radiation 9, pp.229-232 (2002). 9. 229-232 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] A.Yamasaki: "Orbital angular momentum and interpretation on band picture in Co-based Heusler alloys Co_2YSn(Y=Ti, Zr, and Nb)"Phys. Rev. B. 65. 104410-1-104410-6 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] T.Iwasaki: "High-Resolution Resonance Photoemission Study of CeMX(M=Pt, Pd ; X=P, As, Sb)"Phys. Rev. B. 65. 195109-1-195109-7 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] S.Suga: "Extremely high quality soft X-ray beam line BL25SU of SPring-8: instrumentation and research activities"Nucl.Instrum.Meth.. A467-468. 1388-1395 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Suga: "X・MCD at twin-helical undulator beam line BL25SU of SPring-8"J.Magn.Magn.Mater.. 233. 60-64 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] S.Suga: "High resolution soft x-ray bulk sensitive photoemission from strongly correlated systems"J.Electron Spectrosc.Rel.Phenom.. 114-116. 659-668 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] W.Kuch: "Element-selective mapping of magnetic moments in ultrathin magnetic films using photoemission microscope"Surf.Sci. 480. 153-162 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] R.Jung: "Temperature dependent bulk sensitive Ce 3d edge rscmant photoemission study of Ce Fe2 sensitive"J.Electron Spectrosc.Rel.Phenom.. 114-116. 693-698 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Sekiyama: "Bulk-sensitive high-resolution Ce 3d-4f resonance photoemission study of CeNiSn and CePdSn"J.Electron Spectrosc.Rel.Phenom.. 114. 699-703 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] A.Sekiyama: "Bulk 4f Electronic States of Ce-Based Heavy Fermion System Probed by High-Resolution Resonance Photoemission"J.Phys.Soc.Jpn. 69. 2771-2774 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Iwasaki: "Bulk and surface electronic structures of CePdX (X=As,Sb) studied by 3d-4f resonance photoemission"Phys.Rev.B. 61. 4621-4628 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Yang: "High-resolution Ce 3d-edge resonant photoemission study of CeNi_2"Phys.Rev.B. 61. R13329-13332 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Suga: "Angle-resolved, resonance-and inverse photoemission studies of transition metal intercalated TiS_2"Molecular Crystals and Liquid Crystals. 341. 9-14 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] S.Suga: "Electronic states of Sm_4As_3 and Sm_4Bi_3 studied with photoemission spectroscopy"Physica B. 281・282. 158-160 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] W.Kuch: "Magnetic circular dichroism microspectroscopy at the spin reorientation transition in Ni(001)film"Phys.Rev.B. 62. 3824-3833 (2000)

    • Related Report
      2000 Annual Research Report

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Published: 2000-04-01   Modified: 2020-05-15  

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