• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

RESEARCH ON HIGH T_C ORGANIC MAGNETS AND NON-FERMI LIQUID BEHAVIOR UNDER MULTIPLE EXTREME PHYSICAL CONDITIONS

Research Project

Project/Area Number 12305022
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionKYUSHU UNIVERSITY

Principal Investigator

TAKEDA Kazuyoshi  KYUSHU UNIVERSITY, Faculty of Engineering, Prof., 大学院・工学研究院, 教授 (10029548)

Co-Investigator(Kenkyū-buntansha) IDOGAKI Toshihiro  KYUSHU UNIVERSITY, Faculty of Engineering, Prof., 大学院・工学研究院, 教授 (40038013)
HITAKA Masako  KYUSHU UNIVERSITY, Faculty of Engineering, Assist., 大学院・工学研究院, 助手 (00264094)
KAWAE Tatsuya  KYUSHU UNIVERSITY, Faculty of Engineering, Assist.Prof., 大学院・工学研究院, 助教授 (30253503)
TANAKA Akinori  KYUSHU UNIVERSITY, Faculty of Engineering, Assist., 大学院・工学研究院, 助手 (80274512)
美藤 正樹  九州大学, 大学院・工学研究院, 助手 (60315108)
Project Period (FY) 2000 – 2003
Project Status Completed (Fiscal Year 2003)
Budget Amount *help
¥39,270,000 (Direct Cost: ¥38,100,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2003: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2002: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2001: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2000: ¥34,200,000 (Direct Cost: ¥34,200,000)
KeywordsElectronic Properties / High Pressure / High Magnetic Field / Low Temperature / Organic Magnets / Non-Fermi Liquid / Magnetic Behavior / Quantum Critical Point / 純有機磁性体 / 量子臨界
Research Abstract

The first realization of the genuine organic ferromagnet had to await the synthesis of b-p-NPNN in 1990. The mechanism of magnetic interactions and high ordering temperature has not been clear now. We have marked the highest value of the magnetic ordering temperature of some 70K with a weak-ferromagnetic organic radical cry stal(the ordering temperature is 36K at ambient pressure) by the application of the pressure up to 1.6GPa.
The Non-Fermi liquid behavior in the non-magnetic quadrupolar system has been found in the present study on(Pr-La)Pb3 system for the dilute limit of Pr.
On the contrary for the wide range of the Prconcentration, the glassy behavior of the quadrupolar moment has been observed with the characteristic 2-level model as the Anderson's glass theory.

Report

(5 results)
  • 2003 Annual Research Report   Final Research Report Summary
  • 2002 Annual Research Report
  • 2001 Annual Research Report
  • 2000 Annual Research Report
  • Research Products

    (34 results)

All Other

All Publications (34 results)

  • [Publications] M.Mito et al.: "Pressure effects on an organic radical ferromagnet : 2,5-difluorophenyl-α-nitronyl nitroxide"Physical Review B.. 67. 024427 1-024427 8 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Mukai et al.: "Heat Capacity Study of the Doping Effect of Paramagnetic Radicals on the Organic Spin-Peiels System : p-CyDOV Radical Crystal"J.Phys.Soc.Jpn. 72. 2312-2316 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] T.Kawae et al.: "Non-Fermi Liquid Behavior in Dilute Quadrupolar Pr_xLa_<1-x>Pb_3 with x< 0.05"J.Phys.Soc.Jpn. 72. 2141-2144 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] K.Takeda et al.: "Pressure Effects of a Genuine Organic Crystalline Ferromagnet Dupeyredioxyl"Polyhedron. 22. 2287-2291 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] A.Tanaka et al.: "Stability of Ferromagnetism in the Hubberd Model on the Kagome Lattice"Phys.Rev.Letters. 90. 067204-1-067204-4 (2003)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Mito, H.Deguchi, T.Tanimoto, T.Kawae, S.Nakatsuji, H.Morimoto, H.Anzai, H.Nakano, Y.Murakami, K.Takeda: "Pressure effects on an organic radical ferromagnet : 2,5-difluorophenyl-a-nitronyl nitoroxide"Physical Review. Vol.67. 024427 1-024427 8 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Kazuo MUKAI, Masanobu YANAGIMOTO, Shyuichi TANAKA, Masaki MITO, Tatsuya KAWAE, Kazuyoshi TAKEDA: "Heat Capacity Study of the Doping Effect of Paramagnetic Radicals on the Organic Spin-Peiels System(p-CyDOV Radical Crystal)"J.Phys.Soc.Jpn.. Vol.72. 2312-2316 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Tatsuya KAWAE, Tatsuharu YAMAMOTO, Kenji YURUE, Naoyuki TATEIWA, Kazuyoshi TAKEDA, Tetsuo KITAI: "Non-Fermi Liquid Behavior in Dilute Quadrupolar System PrxLa1-xPb3 with x<0.05"J.Phys.Soc.Jpn.. Vol.72. 2141-2144 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Kazuyoshi TAKEDA, Masaki MITO, Keiichiro KINOSHTTA, Miguel A.NOVAK, Jean Louis THOLENCE, Andre RASSAT: "Pressure Effects of a Genuine Organic Crystalline Ferromagnet Dupeyredioxyl"Polyhedron. Vol22. 2287-2291 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] Akinori TANAKA, Hiromitsu UEDA: "Stability of Ferromagnetism in the Hubbart Model on the Kagome Lattice"Physical Review Letters. Vol.80, No.6. 067204 (2003)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2003 Final Research Report Summary
  • [Publications] M.Mito et al.: "Pressure Effects on an S=1 Haldane Compound Ni(C_5H_<14>N_2)_2N_3(PF_6)"J.Phys.Soc.Jpn. 72・2. 399-404 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Kawae et al.: "Specific Heat and Electrical Resistivity Measurements in Pr_<0.03>La_<0.99>Pb_3"Physica B. 329-333. 493-494 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Mukai et al.: "Heat Capacity Study of the Doping Effect of Paramagnetic Radicals On the Organic Spin-Peiels System (P-CyDOV Radical Crystal)"J.Phys.Soc.Jpn. 72. 2312-2316 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] M.Mito et al.: "Pressure effects on an organic ferromagneti 2,5-difluoro-phenyl-a-nitronyl nitroxide"Phys.Rev.B. 67. 024427-1-024427-8 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Kawae: "Non-Fermi Liquid Behavior in Dilute Quardrupolar System Pr_xLa_<1-x>Pb_3"J.Phys.Soc.Jpn. 72. 2141-2144 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] K.Takeda: "Pressure Effects of a Genuim Organic Crystalline Ferromagnet Dupere"Polyhedron. 122. 2287-2291 (2003)

    • Related Report
      2003 Annual Research Report
  • [Publications] T.Kawae et al.: "La impurity effect on quadrupolar ordering Pi-Pb_3"Phys. Rev. B. 65. 0102409-1-0102409-4 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Mito: "Pressure effects on an S=1/2 Heisenberg two-leg ladder antiferromagnet Cu_2(C_5H_<12>N_2)_2 Cl_<14>"Phys. Rev. B. 65. 104405-1-104405-7 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Takeda, M.Mito: "Disappearance of Bulk Ferromagnelism of Iron at High Pressure above 9 GPa"J. Phys. Soc. Jpn. 71. 729-731 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] M.Zukovic: "Histogram Monte Carlo Simulation of the Geometricall Frustrated XY Antiferromagnet with Biquadratic Ex."Phys. Rev.. 65. 144410-1-14441-8 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Zenmyo: "Proton NMR Study of Random Mixture Fe_<1-x>M_<nx>Cl_2 2H_2O with Competing Anisotropic Exchange Interaction"J. Phys. Soc. Jpn. 71. 1740-1745 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Tanaka: "Long Range Order in the Ground State of the Spin System with Crbital Degeneracy"Phys. Rev. B. 66. 134426-1-134426-13 (2002)

    • Related Report
      2002 Annual Research Report
  • [Publications] K.Takeda, et al.: "Magnetic Correlations in the S=5/2 Quadratic Lattice Heisenberg Antiforromagnet Mn(HCOO)_2・2(ND_2)_2CO"Phys.Rev.B. 63. 24425-24428 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Tanaka, et al.: "Long-range order in the ground state of the bilinear-biguadratic exchange model"J.Phyo.A. 34. 8767-8780 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] D.Shiomi, et al.: "Single-Component Molecule-Based Ferrimagnets"J.Am.Chem.Soc.. 123. 11823-11824 (2001)

    • Related Report
      2001 Annual Research Report
  • [Publications] T.Kawae, et al.: "La impurity effects on guadrupolar ordering in PrPb_3"Phys.Rev.B. 65. 102409 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] M.Mito et al.: "Pressure effects on an S=1/2 Heisenberg two-leg ladder antiferromagnet Cu_2(C5H_<12>N_2)_2Cl_4"Phys.Rev.B. 65(in press). 104405 (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Takeda et al.: "Disappearance of Bulk Ferromagnetism of Iron at High Pressures abova 9GPa"J.Phys.Soc.Jpn.. 71(No.3)(in press). (2002)

    • Related Report
      2001 Annual Research Report
  • [Publications] K.Takeda et al.: "Exchange interactions in pressure-induced ferromagnetic transition of a genuine organic crystal"Physica B. 284-288. 1491-1492 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Mito et al.: "Pressure-Induced Enhancement of Tc in a Genuine Organic Bulk-Ferromagnet"Physica B. 284-288. 1493-1494 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] T.Kawae et al.: "Magnetic Phase Diagram of RrCO_2Si_2 with Long Period Commensurate Structure"J.Phys,Soc.Jpn.. 69. 586-591 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] M.Mito et al.: "Pressure Effect of an S=1 Haldane Compound"J.Phys.Soc.Jpn.. 69. 1498-1502 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Takeda et al.: "Site Dilution Study of a Square Lattice Heisenberg Antiferromagnet with S=5/2 Covering the Percolation"J.Phys.Soc.Jpn.. 69. 3696-3703 (2000)

    • Related Report
      2000 Annual Research Report
  • [Publications] K.Takeda et al.: "Magnetic correlations in the S=5/2 quadratic lattice Heisenberg antiferromagnet Mn(HCOU)_22(ND_2)_2CO"Phys.Rev.B. 63. 24425-24428 (2001)

    • Related Report
      2000 Annual Research Report

URL: 

Published: 2000-04-01   Modified: 2016-04-21  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi